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Rapid Production of Mn(3)O(4)/rGO as an Efficient Electrode Material for Supercapacitor by Flame Plasma

Benefiting from good ion accessibility and high electrical conductivity, graphene-based material as electrodes show promising electrochemical performance in energy storage systems. In this study, a novel strategy is devised to prepare binder-free Mn(3)O(4)-reduced graphene oxide (Mn(3)O(4)/rGO) elec...

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Detalles Bibliográficos
Autores principales: Zhou, Yang, Guo, Lei, Shi, Wei, Zou, Xuefeng, Xiang, Bin, Xing, Shaohua
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2018
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6025293/
https://www.ncbi.nlm.nih.gov/pubmed/29795008
http://dx.doi.org/10.3390/ma11060881
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author Zhou, Yang
Guo, Lei
Shi, Wei
Zou, Xuefeng
Xiang, Bin
Xing, Shaohua
author_facet Zhou, Yang
Guo, Lei
Shi, Wei
Zou, Xuefeng
Xiang, Bin
Xing, Shaohua
author_sort Zhou, Yang
collection PubMed
description Benefiting from good ion accessibility and high electrical conductivity, graphene-based material as electrodes show promising electrochemical performance in energy storage systems. In this study, a novel strategy is devised to prepare binder-free Mn(3)O(4)-reduced graphene oxide (Mn(3)O(4)/rGO) electrodes. Well-dispersed and homogeneous Mn(3)O(4) nanosheets are grown on graphene layers through a facile chemical co-precipitation process and subsequent flame procedure. This obtained Mn(3)O(4)/rGO nanostructures exhibit excellent gravimetric specific capacitance of 342.5 F g(−1) at current density of 1 A g(−1) and remarkable cycling stability of 85.47% capacitance retention under 10,000 extreme charge/discharge cycles at large current density. Furthermore, an asymmetric supercapacitor assembled using Mn(3)O(4)/rGO and activated graphene (AG) delivers a high energy density of 27.41 Wh kg(−1) and a maximum power density of 8 kW kg(−1). The material synthesis strategy presented in this study is facile, rapid and simple, which would give an insight into potential strategies for large-scale applications of metal oxide/graphene and hold tremendous promise for power storage applications.
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spelling pubmed-60252932018-07-09 Rapid Production of Mn(3)O(4)/rGO as an Efficient Electrode Material for Supercapacitor by Flame Plasma Zhou, Yang Guo, Lei Shi, Wei Zou, Xuefeng Xiang, Bin Xing, Shaohua Materials (Basel) Article Benefiting from good ion accessibility and high electrical conductivity, graphene-based material as electrodes show promising electrochemical performance in energy storage systems. In this study, a novel strategy is devised to prepare binder-free Mn(3)O(4)-reduced graphene oxide (Mn(3)O(4)/rGO) electrodes. Well-dispersed and homogeneous Mn(3)O(4) nanosheets are grown on graphene layers through a facile chemical co-precipitation process and subsequent flame procedure. This obtained Mn(3)O(4)/rGO nanostructures exhibit excellent gravimetric specific capacitance of 342.5 F g(−1) at current density of 1 A g(−1) and remarkable cycling stability of 85.47% capacitance retention under 10,000 extreme charge/discharge cycles at large current density. Furthermore, an asymmetric supercapacitor assembled using Mn(3)O(4)/rGO and activated graphene (AG) delivers a high energy density of 27.41 Wh kg(−1) and a maximum power density of 8 kW kg(−1). The material synthesis strategy presented in this study is facile, rapid and simple, which would give an insight into potential strategies for large-scale applications of metal oxide/graphene and hold tremendous promise for power storage applications. MDPI 2018-05-24 /pmc/articles/PMC6025293/ /pubmed/29795008 http://dx.doi.org/10.3390/ma11060881 Text en © 2018 by the authors. Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (http://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Zhou, Yang
Guo, Lei
Shi, Wei
Zou, Xuefeng
Xiang, Bin
Xing, Shaohua
Rapid Production of Mn(3)O(4)/rGO as an Efficient Electrode Material for Supercapacitor by Flame Plasma
title Rapid Production of Mn(3)O(4)/rGO as an Efficient Electrode Material for Supercapacitor by Flame Plasma
title_full Rapid Production of Mn(3)O(4)/rGO as an Efficient Electrode Material for Supercapacitor by Flame Plasma
title_fullStr Rapid Production of Mn(3)O(4)/rGO as an Efficient Electrode Material for Supercapacitor by Flame Plasma
title_full_unstemmed Rapid Production of Mn(3)O(4)/rGO as an Efficient Electrode Material for Supercapacitor by Flame Plasma
title_short Rapid Production of Mn(3)O(4)/rGO as an Efficient Electrode Material for Supercapacitor by Flame Plasma
title_sort rapid production of mn(3)o(4)/rgo as an efficient electrode material for supercapacitor by flame plasma
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6025293/
https://www.ncbi.nlm.nih.gov/pubmed/29795008
http://dx.doi.org/10.3390/ma11060881
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