Cargando…
A general printing approach for scalable growth of perovskite single-crystal films
Perovskite single-crystal films, which exhibit exceptionally low trap density and nearly perfect translational symmetry, are believed to achieve the highest performance of perovskite-based optoelectronic devices. However, fabrication of these perovskite single-crystal films is quite difficult becaus...
Autores principales: | , , , , |
---|---|
Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American Association for the Advancement of Science
2018
|
Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6025903/ https://www.ncbi.nlm.nih.gov/pubmed/29963635 http://dx.doi.org/10.1126/sciadv.aat2390 |
Sumario: | Perovskite single-crystal films, which exhibit exceptionally low trap density and nearly perfect translational symmetry, are believed to achieve the highest performance of perovskite-based optoelectronic devices. However, fabrication of these perovskite single-crystal films is quite difficult because of the uncontrollable nucleation caused by the rapid reaction of two perovskite precursors. We report a facile seed printing approach to selectively create millimeter-sized perovskite single-crystal films with controlled thickness and high yield. We show that perovskite single-crystal films can be perfectly transferred to almost arbitrary substrates through the printing process. The as-grown perovskite single-crystal films have excellent crystalline quality and morphology. We further demonstrate that perovskite single-crystal films can be directly printed for scalable fabrication of photodetectors and effective image sensors. This strategy allows high-yield fabrication of large perovskite single-crystal films for functional devices and may extend to other solution-processed materials for wide applications. |
---|