Cargando…

Improved recovery time and sensitivity to H(2) and NH(3) at room temperature with SnO(x) vertical nanopillars on ITO

Nanostructured SnO(2) is a promising material for the scalable production of portable gas sensors. To fully exploit their potential, these gas sensors need a faster recovery rate and higher sensitivity at room temperature than the current state of the art. Here we demonstrate a chemiresistive gas se...

Descripción completa

Detalles Bibliográficos
Autores principales: D’Arsié, L., Alijani, V., Brunelli, S. T. Suran, Rigoni, F., Di Santo, G., Caputo, M., Panighel, M., Freddi, S., Sangaletti, L., Goldoni, A.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2018
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6030158/
https://www.ncbi.nlm.nih.gov/pubmed/29968779
http://dx.doi.org/10.1038/s41598-018-28298-w
_version_ 1783337088763035648
author D’Arsié, L.
Alijani, V.
Brunelli, S. T. Suran
Rigoni, F.
Di Santo, G.
Caputo, M.
Panighel, M.
Freddi, S.
Sangaletti, L.
Goldoni, A.
author_facet D’Arsié, L.
Alijani, V.
Brunelli, S. T. Suran
Rigoni, F.
Di Santo, G.
Caputo, M.
Panighel, M.
Freddi, S.
Sangaletti, L.
Goldoni, A.
author_sort D’Arsié, L.
collection PubMed
description Nanostructured SnO(2) is a promising material for the scalable production of portable gas sensors. To fully exploit their potential, these gas sensors need a faster recovery rate and higher sensitivity at room temperature than the current state of the art. Here we demonstrate a chemiresistive gas sensor based on vertical SnO(x) nanopillars, capable of sensing < 5 ppm of H(2) at room temperature and 10 ppt at 230 °C. We test the sample both in vacuum and in air and observe an exceptional improvement in the performance compared to commercially available gas sensors. In particular, the recovery time for sensing NH(3) at room temperature is more than one order of magnitude faster than a commercial SnO(2) sensor. The sensor shows an unique combination of high sensitivity and fast recovery time, matching the requirements on materials expected to foster widespread use of portable and affordable gas sensors.
format Online
Article
Text
id pubmed-6030158
institution National Center for Biotechnology Information
language English
publishDate 2018
publisher Nature Publishing Group UK
record_format MEDLINE/PubMed
spelling pubmed-60301582018-07-11 Improved recovery time and sensitivity to H(2) and NH(3) at room temperature with SnO(x) vertical nanopillars on ITO D’Arsié, L. Alijani, V. Brunelli, S. T. Suran Rigoni, F. Di Santo, G. Caputo, M. Panighel, M. Freddi, S. Sangaletti, L. Goldoni, A. Sci Rep Article Nanostructured SnO(2) is a promising material for the scalable production of portable gas sensors. To fully exploit their potential, these gas sensors need a faster recovery rate and higher sensitivity at room temperature than the current state of the art. Here we demonstrate a chemiresistive gas sensor based on vertical SnO(x) nanopillars, capable of sensing < 5 ppm of H(2) at room temperature and 10 ppt at 230 °C. We test the sample both in vacuum and in air and observe an exceptional improvement in the performance compared to commercially available gas sensors. In particular, the recovery time for sensing NH(3) at room temperature is more than one order of magnitude faster than a commercial SnO(2) sensor. The sensor shows an unique combination of high sensitivity and fast recovery time, matching the requirements on materials expected to foster widespread use of portable and affordable gas sensors. Nature Publishing Group UK 2018-07-03 /pmc/articles/PMC6030158/ /pubmed/29968779 http://dx.doi.org/10.1038/s41598-018-28298-w Text en © The Author(s) 2018 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
D’Arsié, L.
Alijani, V.
Brunelli, S. T. Suran
Rigoni, F.
Di Santo, G.
Caputo, M.
Panighel, M.
Freddi, S.
Sangaletti, L.
Goldoni, A.
Improved recovery time and sensitivity to H(2) and NH(3) at room temperature with SnO(x) vertical nanopillars on ITO
title Improved recovery time and sensitivity to H(2) and NH(3) at room temperature with SnO(x) vertical nanopillars on ITO
title_full Improved recovery time and sensitivity to H(2) and NH(3) at room temperature with SnO(x) vertical nanopillars on ITO
title_fullStr Improved recovery time and sensitivity to H(2) and NH(3) at room temperature with SnO(x) vertical nanopillars on ITO
title_full_unstemmed Improved recovery time and sensitivity to H(2) and NH(3) at room temperature with SnO(x) vertical nanopillars on ITO
title_short Improved recovery time and sensitivity to H(2) and NH(3) at room temperature with SnO(x) vertical nanopillars on ITO
title_sort improved recovery time and sensitivity to h(2) and nh(3) at room temperature with sno(x) vertical nanopillars on ito
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6030158/
https://www.ncbi.nlm.nih.gov/pubmed/29968779
http://dx.doi.org/10.1038/s41598-018-28298-w
work_keys_str_mv AT darsiel improvedrecoverytimeandsensitivitytoh2andnh3atroomtemperaturewithsnoxverticalnanopillarsonito
AT alijaniv improvedrecoverytimeandsensitivitytoh2andnh3atroomtemperaturewithsnoxverticalnanopillarsonito
AT brunellistsuran improvedrecoverytimeandsensitivitytoh2andnh3atroomtemperaturewithsnoxverticalnanopillarsonito
AT rigonif improvedrecoverytimeandsensitivitytoh2andnh3atroomtemperaturewithsnoxverticalnanopillarsonito
AT disantog improvedrecoverytimeandsensitivitytoh2andnh3atroomtemperaturewithsnoxverticalnanopillarsonito
AT caputom improvedrecoverytimeandsensitivitytoh2andnh3atroomtemperaturewithsnoxverticalnanopillarsonito
AT panighelm improvedrecoverytimeandsensitivitytoh2andnh3atroomtemperaturewithsnoxverticalnanopillarsonito
AT freddis improvedrecoverytimeandsensitivitytoh2andnh3atroomtemperaturewithsnoxverticalnanopillarsonito
AT sangalettil improvedrecoverytimeandsensitivitytoh2andnh3atroomtemperaturewithsnoxverticalnanopillarsonito
AT goldonia improvedrecoverytimeandsensitivitytoh2andnh3atroomtemperaturewithsnoxverticalnanopillarsonito