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The nature of spin excitations in the one-third magnetization plateau phase of Ba(3)CoSb(2)O(9)
Magnetization plateaus in quantum magnets—where bosonic quasiparticles crystallize into emergent spin superlattices—are spectacular yet simple examples of collective quantum phenomena escaping classical description. While magnetization plateaus have been observed in a number of spin-1/2 antiferromag...
Autores principales: | , , , , , , , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group UK
2018
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6039502/ https://www.ncbi.nlm.nih.gov/pubmed/29991805 http://dx.doi.org/10.1038/s41467-018-04914-1 |
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author | Kamiya, Y. Ge, L. Hong, Tao Qiu, Y. Quintero-Castro, D. L. Lu, Z. Cao, H. B. Matsuda, M. Choi, E. S. Batista, C. D. Mourigal, M. Zhou, H. D. Ma, J. |
author_facet | Kamiya, Y. Ge, L. Hong, Tao Qiu, Y. Quintero-Castro, D. L. Lu, Z. Cao, H. B. Matsuda, M. Choi, E. S. Batista, C. D. Mourigal, M. Zhou, H. D. Ma, J. |
author_sort | Kamiya, Y. |
collection | PubMed |
description | Magnetization plateaus in quantum magnets—where bosonic quasiparticles crystallize into emergent spin superlattices—are spectacular yet simple examples of collective quantum phenomena escaping classical description. While magnetization plateaus have been observed in a number of spin-1/2 antiferromagnets, the description of their magnetic excitations remains an open theoretical and experimental challenge. Here, we investigate the dynamical properties of the triangular-lattice spin-1/2 antiferromagnet Ba(3)CoSb(2)O(9) in its one-third magnetization plateau phase using a combination of nonlinear spin-wave theory and neutron scattering measurements. The agreement between our theoretical treatment and the experimental data demonstrates that magnons behave semiclassically in the plateau in spite of the purely quantum origin of the underlying magnetic structure. This allows for a quantitative determination of Ba(3)CoSb(2)O(9) exchange parameters. We discuss the implication of our results to the deviations from semiclassical behavior observed in zero-field spin dynamics of the same material and conclude they must have an intrinsic origin. |
format | Online Article Text |
id | pubmed-6039502 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2018 |
publisher | Nature Publishing Group UK |
record_format | MEDLINE/PubMed |
spelling | pubmed-60395022018-07-12 The nature of spin excitations in the one-third magnetization plateau phase of Ba(3)CoSb(2)O(9) Kamiya, Y. Ge, L. Hong, Tao Qiu, Y. Quintero-Castro, D. L. Lu, Z. Cao, H. B. Matsuda, M. Choi, E. S. Batista, C. D. Mourigal, M. Zhou, H. D. Ma, J. Nat Commun Article Magnetization plateaus in quantum magnets—where bosonic quasiparticles crystallize into emergent spin superlattices—are spectacular yet simple examples of collective quantum phenomena escaping classical description. While magnetization plateaus have been observed in a number of spin-1/2 antiferromagnets, the description of their magnetic excitations remains an open theoretical and experimental challenge. Here, we investigate the dynamical properties of the triangular-lattice spin-1/2 antiferromagnet Ba(3)CoSb(2)O(9) in its one-third magnetization plateau phase using a combination of nonlinear spin-wave theory and neutron scattering measurements. The agreement between our theoretical treatment and the experimental data demonstrates that magnons behave semiclassically in the plateau in spite of the purely quantum origin of the underlying magnetic structure. This allows for a quantitative determination of Ba(3)CoSb(2)O(9) exchange parameters. We discuss the implication of our results to the deviations from semiclassical behavior observed in zero-field spin dynamics of the same material and conclude they must have an intrinsic origin. Nature Publishing Group UK 2018-07-10 /pmc/articles/PMC6039502/ /pubmed/29991805 http://dx.doi.org/10.1038/s41467-018-04914-1 Text en © The Author(s) 2018 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/. |
spellingShingle | Article Kamiya, Y. Ge, L. Hong, Tao Qiu, Y. Quintero-Castro, D. L. Lu, Z. Cao, H. B. Matsuda, M. Choi, E. S. Batista, C. D. Mourigal, M. Zhou, H. D. Ma, J. The nature of spin excitations in the one-third magnetization plateau phase of Ba(3)CoSb(2)O(9) |
title | The nature of spin excitations in the one-third magnetization plateau phase of Ba(3)CoSb(2)O(9) |
title_full | The nature of spin excitations in the one-third magnetization plateau phase of Ba(3)CoSb(2)O(9) |
title_fullStr | The nature of spin excitations in the one-third magnetization plateau phase of Ba(3)CoSb(2)O(9) |
title_full_unstemmed | The nature of spin excitations in the one-third magnetization plateau phase of Ba(3)CoSb(2)O(9) |
title_short | The nature of spin excitations in the one-third magnetization plateau phase of Ba(3)CoSb(2)O(9) |
title_sort | nature of spin excitations in the one-third magnetization plateau phase of ba(3)cosb(2)o(9) |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6039502/ https://www.ncbi.nlm.nih.gov/pubmed/29991805 http://dx.doi.org/10.1038/s41467-018-04914-1 |
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