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The nature of spin excitations in the one-third magnetization plateau phase of Ba(3)CoSb(2)O(9)

Magnetization plateaus in quantum magnets—where bosonic quasiparticles crystallize into emergent spin superlattices—are spectacular yet simple examples of collective quantum phenomena escaping classical description. While magnetization plateaus have been observed in a number of spin-1/2 antiferromag...

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Autores principales: Kamiya, Y., Ge, L., Hong, Tao, Qiu, Y., Quintero-Castro, D. L., Lu, Z., Cao, H. B., Matsuda, M., Choi, E. S., Batista, C. D., Mourigal, M., Zhou, H. D., Ma, J.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2018
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6039502/
https://www.ncbi.nlm.nih.gov/pubmed/29991805
http://dx.doi.org/10.1038/s41467-018-04914-1
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author Kamiya, Y.
Ge, L.
Hong, Tao
Qiu, Y.
Quintero-Castro, D. L.
Lu, Z.
Cao, H. B.
Matsuda, M.
Choi, E. S.
Batista, C. D.
Mourigal, M.
Zhou, H. D.
Ma, J.
author_facet Kamiya, Y.
Ge, L.
Hong, Tao
Qiu, Y.
Quintero-Castro, D. L.
Lu, Z.
Cao, H. B.
Matsuda, M.
Choi, E. S.
Batista, C. D.
Mourigal, M.
Zhou, H. D.
Ma, J.
author_sort Kamiya, Y.
collection PubMed
description Magnetization plateaus in quantum magnets—where bosonic quasiparticles crystallize into emergent spin superlattices—are spectacular yet simple examples of collective quantum phenomena escaping classical description. While magnetization plateaus have been observed in a number of spin-1/2 antiferromagnets, the description of their magnetic excitations remains an open theoretical and experimental challenge. Here, we investigate the dynamical properties of the triangular-lattice spin-1/2 antiferromagnet Ba(3)CoSb(2)O(9) in its one-third magnetization plateau phase using a combination of nonlinear spin-wave theory and neutron scattering measurements. The agreement between our theoretical treatment and the experimental data demonstrates that magnons behave semiclassically in the plateau in spite of the purely quantum origin of the underlying magnetic structure. This allows for a quantitative determination of Ba(3)CoSb(2)O(9) exchange parameters. We discuss the implication of our results to the deviations from semiclassical behavior observed in zero-field spin dynamics of the same material and conclude they must have an intrinsic origin.
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spelling pubmed-60395022018-07-12 The nature of spin excitations in the one-third magnetization plateau phase of Ba(3)CoSb(2)O(9) Kamiya, Y. Ge, L. Hong, Tao Qiu, Y. Quintero-Castro, D. L. Lu, Z. Cao, H. B. Matsuda, M. Choi, E. S. Batista, C. D. Mourigal, M. Zhou, H. D. Ma, J. Nat Commun Article Magnetization plateaus in quantum magnets—where bosonic quasiparticles crystallize into emergent spin superlattices—are spectacular yet simple examples of collective quantum phenomena escaping classical description. While magnetization plateaus have been observed in a number of spin-1/2 antiferromagnets, the description of their magnetic excitations remains an open theoretical and experimental challenge. Here, we investigate the dynamical properties of the triangular-lattice spin-1/2 antiferromagnet Ba(3)CoSb(2)O(9) in its one-third magnetization plateau phase using a combination of nonlinear spin-wave theory and neutron scattering measurements. The agreement between our theoretical treatment and the experimental data demonstrates that magnons behave semiclassically in the plateau in spite of the purely quantum origin of the underlying magnetic structure. This allows for a quantitative determination of Ba(3)CoSb(2)O(9) exchange parameters. We discuss the implication of our results to the deviations from semiclassical behavior observed in zero-field spin dynamics of the same material and conclude they must have an intrinsic origin. Nature Publishing Group UK 2018-07-10 /pmc/articles/PMC6039502/ /pubmed/29991805 http://dx.doi.org/10.1038/s41467-018-04914-1 Text en © The Author(s) 2018 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Kamiya, Y.
Ge, L.
Hong, Tao
Qiu, Y.
Quintero-Castro, D. L.
Lu, Z.
Cao, H. B.
Matsuda, M.
Choi, E. S.
Batista, C. D.
Mourigal, M.
Zhou, H. D.
Ma, J.
The nature of spin excitations in the one-third magnetization plateau phase of Ba(3)CoSb(2)O(9)
title The nature of spin excitations in the one-third magnetization plateau phase of Ba(3)CoSb(2)O(9)
title_full The nature of spin excitations in the one-third magnetization plateau phase of Ba(3)CoSb(2)O(9)
title_fullStr The nature of spin excitations in the one-third magnetization plateau phase of Ba(3)CoSb(2)O(9)
title_full_unstemmed The nature of spin excitations in the one-third magnetization plateau phase of Ba(3)CoSb(2)O(9)
title_short The nature of spin excitations in the one-third magnetization plateau phase of Ba(3)CoSb(2)O(9)
title_sort nature of spin excitations in the one-third magnetization plateau phase of ba(3)cosb(2)o(9)
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6039502/
https://www.ncbi.nlm.nih.gov/pubmed/29991805
http://dx.doi.org/10.1038/s41467-018-04914-1
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