Cargando…

High sensitivity organic inorganic hybrid X-ray detectors with direct transduction and broadband response

X-ray detectors are critical to healthcare diagnostics, cancer therapy and homeland security, with many potential uses limited by system cost and/or detector dimensions. Current X-ray detector sensitivities are limited by the bulk X-ray attenuation of the materials and consequently necessitate thick...

Descripción completa

Detalles Bibliográficos
Autores principales: Thirimanne, H. M., Jayawardena, K. D. G. I., Parnell, A. J., Bandara, R. M. I., Karalasingam, A., Pani, S., Huerdler, J. E., Lidzey, D. G., Tedde, S. F., Nisbet, A., Mills, C. A., Silva, S. R. P.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2018
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6062530/
https://www.ncbi.nlm.nih.gov/pubmed/30050037
http://dx.doi.org/10.1038/s41467-018-05301-6
_version_ 1783342387752337408
author Thirimanne, H. M.
Jayawardena, K. D. G. I.
Parnell, A. J.
Bandara, R. M. I.
Karalasingam, A.
Pani, S.
Huerdler, J. E.
Lidzey, D. G.
Tedde, S. F.
Nisbet, A.
Mills, C. A.
Silva, S. R. P.
author_facet Thirimanne, H. M.
Jayawardena, K. D. G. I.
Parnell, A. J.
Bandara, R. M. I.
Karalasingam, A.
Pani, S.
Huerdler, J. E.
Lidzey, D. G.
Tedde, S. F.
Nisbet, A.
Mills, C. A.
Silva, S. R. P.
author_sort Thirimanne, H. M.
collection PubMed
description X-ray detectors are critical to healthcare diagnostics, cancer therapy and homeland security, with many potential uses limited by system cost and/or detector dimensions. Current X-ray detector sensitivities are limited by the bulk X-ray attenuation of the materials and consequently necessitate thick crystals (~1 mm–1 cm), resulting in rigid structures, high operational voltages and high cost. Here we present a disruptive, flexible, low cost, broadband, and high sensitivity direct X-ray transduction technology produced by embedding high atomic number bismuth oxide nanoparticles in an organic bulk heterojunction. These hybrid detectors demonstrate sensitivities of 1712 µC mGy(−1) cm(−3) for “soft” X-rays and ~30 and 58 µC mGy(−1) cm(−3) under 6 and 15 MV “hard” X-rays generated from a medical linear accelerator; strongly competing with the current solid state detectors, all achieved at low bias voltages (−10 V) and low power, enabling detector operation powered by coin cell batteries.
format Online
Article
Text
id pubmed-6062530
institution National Center for Biotechnology Information
language English
publishDate 2018
publisher Nature Publishing Group UK
record_format MEDLINE/PubMed
spelling pubmed-60625302018-07-30 High sensitivity organic inorganic hybrid X-ray detectors with direct transduction and broadband response Thirimanne, H. M. Jayawardena, K. D. G. I. Parnell, A. J. Bandara, R. M. I. Karalasingam, A. Pani, S. Huerdler, J. E. Lidzey, D. G. Tedde, S. F. Nisbet, A. Mills, C. A. Silva, S. R. P. Nat Commun Article X-ray detectors are critical to healthcare diagnostics, cancer therapy and homeland security, with many potential uses limited by system cost and/or detector dimensions. Current X-ray detector sensitivities are limited by the bulk X-ray attenuation of the materials and consequently necessitate thick crystals (~1 mm–1 cm), resulting in rigid structures, high operational voltages and high cost. Here we present a disruptive, flexible, low cost, broadband, and high sensitivity direct X-ray transduction technology produced by embedding high atomic number bismuth oxide nanoparticles in an organic bulk heterojunction. These hybrid detectors demonstrate sensitivities of 1712 µC mGy(−1) cm(−3) for “soft” X-rays and ~30 and 58 µC mGy(−1) cm(−3) under 6 and 15 MV “hard” X-rays generated from a medical linear accelerator; strongly competing with the current solid state detectors, all achieved at low bias voltages (−10 V) and low power, enabling detector operation powered by coin cell batteries. Nature Publishing Group UK 2018-07-26 /pmc/articles/PMC6062530/ /pubmed/30050037 http://dx.doi.org/10.1038/s41467-018-05301-6 Text en © The Author(s) 2018 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Thirimanne, H. M.
Jayawardena, K. D. G. I.
Parnell, A. J.
Bandara, R. M. I.
Karalasingam, A.
Pani, S.
Huerdler, J. E.
Lidzey, D. G.
Tedde, S. F.
Nisbet, A.
Mills, C. A.
Silva, S. R. P.
High sensitivity organic inorganic hybrid X-ray detectors with direct transduction and broadband response
title High sensitivity organic inorganic hybrid X-ray detectors with direct transduction and broadband response
title_full High sensitivity organic inorganic hybrid X-ray detectors with direct transduction and broadband response
title_fullStr High sensitivity organic inorganic hybrid X-ray detectors with direct transduction and broadband response
title_full_unstemmed High sensitivity organic inorganic hybrid X-ray detectors with direct transduction and broadband response
title_short High sensitivity organic inorganic hybrid X-ray detectors with direct transduction and broadband response
title_sort high sensitivity organic inorganic hybrid x-ray detectors with direct transduction and broadband response
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6062530/
https://www.ncbi.nlm.nih.gov/pubmed/30050037
http://dx.doi.org/10.1038/s41467-018-05301-6
work_keys_str_mv AT thirimannehm highsensitivityorganicinorganichybridxraydetectorswithdirecttransductionandbroadbandresponse
AT jayawardenakdgi highsensitivityorganicinorganichybridxraydetectorswithdirecttransductionandbroadbandresponse
AT parnellaj highsensitivityorganicinorganichybridxraydetectorswithdirecttransductionandbroadbandresponse
AT bandararmi highsensitivityorganicinorganichybridxraydetectorswithdirecttransductionandbroadbandresponse
AT karalasingama highsensitivityorganicinorganichybridxraydetectorswithdirecttransductionandbroadbandresponse
AT panis highsensitivityorganicinorganichybridxraydetectorswithdirecttransductionandbroadbandresponse
AT huerdlerje highsensitivityorganicinorganichybridxraydetectorswithdirecttransductionandbroadbandresponse
AT lidzeydg highsensitivityorganicinorganichybridxraydetectorswithdirecttransductionandbroadbandresponse
AT teddesf highsensitivityorganicinorganichybridxraydetectorswithdirecttransductionandbroadbandresponse
AT nisbeta highsensitivityorganicinorganichybridxraydetectorswithdirecttransductionandbroadbandresponse
AT millsca highsensitivityorganicinorganichybridxraydetectorswithdirecttransductionandbroadbandresponse
AT silvasrp highsensitivityorganicinorganichybridxraydetectorswithdirecttransductionandbroadbandresponse