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Tailoring carbon nanotubes optical properties through chirality-wise silicon ring resonators

Semiconducting single walled carbon nanotubes (s-SWNT) have an immense potential for the development of active optoelectronic functionalities in ultra-compact hybrid photonic circuits. Specifically, s-SWNT have been identified as a very promising solution to implement light sources in the silicon ph...

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Autores principales: Durán-Valdeiglesias, Elena, Zhang, Weiwei, Alonso-Ramos, Carlos, Serna, Samuel, Le Roux, Xavier, Maris-Morini, Delphine, Caselli, Niccolò, Biccari, Francesco, Gurioli, Massimo, Filoramo, Arianna, Cassan, Eric, Vivien, Laurent
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2018
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6062534/
https://www.ncbi.nlm.nih.gov/pubmed/30050165
http://dx.doi.org/10.1038/s41598-018-29300-1
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author Durán-Valdeiglesias, Elena
Zhang, Weiwei
Alonso-Ramos, Carlos
Serna, Samuel
Le Roux, Xavier
Maris-Morini, Delphine
Caselli, Niccolò
Biccari, Francesco
Gurioli, Massimo
Filoramo, Arianna
Cassan, Eric
Vivien, Laurent
author_facet Durán-Valdeiglesias, Elena
Zhang, Weiwei
Alonso-Ramos, Carlos
Serna, Samuel
Le Roux, Xavier
Maris-Morini, Delphine
Caselli, Niccolò
Biccari, Francesco
Gurioli, Massimo
Filoramo, Arianna
Cassan, Eric
Vivien, Laurent
author_sort Durán-Valdeiglesias, Elena
collection PubMed
description Semiconducting single walled carbon nanotubes (s-SWNT) have an immense potential for the development of active optoelectronic functionalities in ultra-compact hybrid photonic circuits. Specifically, s-SWNT have been identified as a very promising solution to implement light sources in the silicon photonics platform. Still, two major challenges remain to fully exploit the potential of this hybrid technology: the limited interaction between s-SWNTs and Si waveguides and the low quantum efficiency of s-SWNTs emission. Silicon micro-ring resonators have the potential capability to overcome these limitations, by providing enhanced light s-SWNT interaction through resonant light recirculation. Here, we demonstrate that Si ring resonators provide SWNT chirality-wise photoluminescence resonance enhancement, releasing a new degree of freedom to tailor s-SWNT optical properties. Specifically, we show that judicious design of the micro-ring geometry allows selectively promoting the emission enhancement of either (8,6) or (8,7) SWNT chiralities present in a high-purity polymer-sorted s-SWNT solution. In addition, we present an analysis of nanometric-sized silicon-on-insulator waveguides that predicts stronger light s-SWNT interaction for transverse-magnetic (TM) modes than for conventionally used transverse-electric (TE) modes.
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spelling pubmed-60625342018-07-31 Tailoring carbon nanotubes optical properties through chirality-wise silicon ring resonators Durán-Valdeiglesias, Elena Zhang, Weiwei Alonso-Ramos, Carlos Serna, Samuel Le Roux, Xavier Maris-Morini, Delphine Caselli, Niccolò Biccari, Francesco Gurioli, Massimo Filoramo, Arianna Cassan, Eric Vivien, Laurent Sci Rep Article Semiconducting single walled carbon nanotubes (s-SWNT) have an immense potential for the development of active optoelectronic functionalities in ultra-compact hybrid photonic circuits. Specifically, s-SWNT have been identified as a very promising solution to implement light sources in the silicon photonics platform. Still, two major challenges remain to fully exploit the potential of this hybrid technology: the limited interaction between s-SWNTs and Si waveguides and the low quantum efficiency of s-SWNTs emission. Silicon micro-ring resonators have the potential capability to overcome these limitations, by providing enhanced light s-SWNT interaction through resonant light recirculation. Here, we demonstrate that Si ring resonators provide SWNT chirality-wise photoluminescence resonance enhancement, releasing a new degree of freedom to tailor s-SWNT optical properties. Specifically, we show that judicious design of the micro-ring geometry allows selectively promoting the emission enhancement of either (8,6) or (8,7) SWNT chiralities present in a high-purity polymer-sorted s-SWNT solution. In addition, we present an analysis of nanometric-sized silicon-on-insulator waveguides that predicts stronger light s-SWNT interaction for transverse-magnetic (TM) modes than for conventionally used transverse-electric (TE) modes. Nature Publishing Group UK 2018-07-26 /pmc/articles/PMC6062534/ /pubmed/30050165 http://dx.doi.org/10.1038/s41598-018-29300-1 Text en © The Author(s) 2018 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Durán-Valdeiglesias, Elena
Zhang, Weiwei
Alonso-Ramos, Carlos
Serna, Samuel
Le Roux, Xavier
Maris-Morini, Delphine
Caselli, Niccolò
Biccari, Francesco
Gurioli, Massimo
Filoramo, Arianna
Cassan, Eric
Vivien, Laurent
Tailoring carbon nanotubes optical properties through chirality-wise silicon ring resonators
title Tailoring carbon nanotubes optical properties through chirality-wise silicon ring resonators
title_full Tailoring carbon nanotubes optical properties through chirality-wise silicon ring resonators
title_fullStr Tailoring carbon nanotubes optical properties through chirality-wise silicon ring resonators
title_full_unstemmed Tailoring carbon nanotubes optical properties through chirality-wise silicon ring resonators
title_short Tailoring carbon nanotubes optical properties through chirality-wise silicon ring resonators
title_sort tailoring carbon nanotubes optical properties through chirality-wise silicon ring resonators
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6062534/
https://www.ncbi.nlm.nih.gov/pubmed/30050165
http://dx.doi.org/10.1038/s41598-018-29300-1
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