Cargando…
Observation of bosonic condensation in a hybrid monolayer MoSe(2)-GaAs microcavity
Bosonic condensation belongs to the most intriguing phenomena in physics, and was mostly reserved for experiments with ultra-cold quantum gases. More recently, it became accessible in exciton-based solid-state systems at elevated temperatures. Here, we demonstrate bosonic condensation driven by exci...
Autores principales: | , , , , , , , , , , , , , , , |
---|---|
Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group UK
2018
|
Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6095855/ https://www.ncbi.nlm.nih.gov/pubmed/30115908 http://dx.doi.org/10.1038/s41467-018-05532-7 |
_version_ | 1783347994942242816 |
---|---|
author | Waldherr, Max Lundt, Nils Klaas, Martin Betzold, Simon Wurdack, Matthias Baumann, Vasilij Estrecho, Eliezer Nalitov, Anton Cherotchenko, Evgenia Cai, Hui Ostrovskaya, Elena A. Kavokin, Alexey V. Tongay, Sefaattin Klembt, Sebastian Höfling, Sven Schneider, Christian |
author_facet | Waldherr, Max Lundt, Nils Klaas, Martin Betzold, Simon Wurdack, Matthias Baumann, Vasilij Estrecho, Eliezer Nalitov, Anton Cherotchenko, Evgenia Cai, Hui Ostrovskaya, Elena A. Kavokin, Alexey V. Tongay, Sefaattin Klembt, Sebastian Höfling, Sven Schneider, Christian |
author_sort | Waldherr, Max |
collection | PubMed |
description | Bosonic condensation belongs to the most intriguing phenomena in physics, and was mostly reserved for experiments with ultra-cold quantum gases. More recently, it became accessible in exciton-based solid-state systems at elevated temperatures. Here, we demonstrate bosonic condensation driven by excitons hosted in an atomically thin layer of MoSe(2), strongly coupled to light in a solid-state resonator. The structure is operated in the regime of collective strong coupling between a Tamm-plasmon resonance, GaAs quantum well excitons, and two-dimensional excitons confined in the monolayer crystal. Polariton condensation in a monolayer crystal manifests by a superlinear increase of emission intensity from the hybrid polariton mode, its density-dependent blueshift, and a dramatic collapse of the emission linewidth, a hallmark of temporal coherence. Importantly, we observe a significant spin-polarization in the injected polariton condensate, a fingerprint for spin-valley locking in monolayer excitons. Our results pave the way towards highly nonlinear, coherent valleytronic devices and light sources. |
format | Online Article Text |
id | pubmed-6095855 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2018 |
publisher | Nature Publishing Group UK |
record_format | MEDLINE/PubMed |
spelling | pubmed-60958552018-08-20 Observation of bosonic condensation in a hybrid monolayer MoSe(2)-GaAs microcavity Waldherr, Max Lundt, Nils Klaas, Martin Betzold, Simon Wurdack, Matthias Baumann, Vasilij Estrecho, Eliezer Nalitov, Anton Cherotchenko, Evgenia Cai, Hui Ostrovskaya, Elena A. Kavokin, Alexey V. Tongay, Sefaattin Klembt, Sebastian Höfling, Sven Schneider, Christian Nat Commun Article Bosonic condensation belongs to the most intriguing phenomena in physics, and was mostly reserved for experiments with ultra-cold quantum gases. More recently, it became accessible in exciton-based solid-state systems at elevated temperatures. Here, we demonstrate bosonic condensation driven by excitons hosted in an atomically thin layer of MoSe(2), strongly coupled to light in a solid-state resonator. The structure is operated in the regime of collective strong coupling between a Tamm-plasmon resonance, GaAs quantum well excitons, and two-dimensional excitons confined in the monolayer crystal. Polariton condensation in a monolayer crystal manifests by a superlinear increase of emission intensity from the hybrid polariton mode, its density-dependent blueshift, and a dramatic collapse of the emission linewidth, a hallmark of temporal coherence. Importantly, we observe a significant spin-polarization in the injected polariton condensate, a fingerprint for spin-valley locking in monolayer excitons. Our results pave the way towards highly nonlinear, coherent valleytronic devices and light sources. Nature Publishing Group UK 2018-08-16 /pmc/articles/PMC6095855/ /pubmed/30115908 http://dx.doi.org/10.1038/s41467-018-05532-7 Text en © The Author(s) 2018 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/. |
spellingShingle | Article Waldherr, Max Lundt, Nils Klaas, Martin Betzold, Simon Wurdack, Matthias Baumann, Vasilij Estrecho, Eliezer Nalitov, Anton Cherotchenko, Evgenia Cai, Hui Ostrovskaya, Elena A. Kavokin, Alexey V. Tongay, Sefaattin Klembt, Sebastian Höfling, Sven Schneider, Christian Observation of bosonic condensation in a hybrid monolayer MoSe(2)-GaAs microcavity |
title | Observation of bosonic condensation in a hybrid monolayer MoSe(2)-GaAs microcavity |
title_full | Observation of bosonic condensation in a hybrid monolayer MoSe(2)-GaAs microcavity |
title_fullStr | Observation of bosonic condensation in a hybrid monolayer MoSe(2)-GaAs microcavity |
title_full_unstemmed | Observation of bosonic condensation in a hybrid monolayer MoSe(2)-GaAs microcavity |
title_short | Observation of bosonic condensation in a hybrid monolayer MoSe(2)-GaAs microcavity |
title_sort | observation of bosonic condensation in a hybrid monolayer mose(2)-gaas microcavity |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6095855/ https://www.ncbi.nlm.nih.gov/pubmed/30115908 http://dx.doi.org/10.1038/s41467-018-05532-7 |
work_keys_str_mv | AT waldherrmax observationofbosoniccondensationinahybridmonolayermose2gaasmicrocavity AT lundtnils observationofbosoniccondensationinahybridmonolayermose2gaasmicrocavity AT klaasmartin observationofbosoniccondensationinahybridmonolayermose2gaasmicrocavity AT betzoldsimon observationofbosoniccondensationinahybridmonolayermose2gaasmicrocavity AT wurdackmatthias observationofbosoniccondensationinahybridmonolayermose2gaasmicrocavity AT baumannvasilij observationofbosoniccondensationinahybridmonolayermose2gaasmicrocavity AT estrechoeliezer observationofbosoniccondensationinahybridmonolayermose2gaasmicrocavity AT nalitovanton observationofbosoniccondensationinahybridmonolayermose2gaasmicrocavity AT cherotchenkoevgenia observationofbosoniccondensationinahybridmonolayermose2gaasmicrocavity AT caihui observationofbosoniccondensationinahybridmonolayermose2gaasmicrocavity AT ostrovskayaelenaa observationofbosoniccondensationinahybridmonolayermose2gaasmicrocavity AT kavokinalexeyv observationofbosoniccondensationinahybridmonolayermose2gaasmicrocavity AT tongaysefaattin observationofbosoniccondensationinahybridmonolayermose2gaasmicrocavity AT klembtsebastian observationofbosoniccondensationinahybridmonolayermose2gaasmicrocavity AT hoflingsven observationofbosoniccondensationinahybridmonolayermose2gaasmicrocavity AT schneiderchristian observationofbosoniccondensationinahybridmonolayermose2gaasmicrocavity |