Simple Synthesis of High Specific Surface Carbon Nitride for Adsorption-Enhanced Photocatalytic Performance

ABSTRACT: TMC-incorporated carbon nitride (CN) with hexagonal and quadrangle honeycomb-like structure and having periodic lattice defects linked by –CONH– bond was synthesized through combining the high calcination with the chemical condensation of melamine and 1,3,5-benzenetricarbonyl trichloride....

Descripción completa

Detalles Bibliográficos
Autores principales: Wang, Jie, Li, Meisheng, Qian, Ming, Zhou, Shouyong, Xue, Ailian, Zhang, Lili, Zhao, Yijiang, Xing, Weihong
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Springer US 2018
Materias:
Nano Express
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6104408/
https://www.ncbi.nlm.nih.gov/pubmed/30136161
http://dx.doi.org/10.1186/s11671-018-2654-7
_version_ 1783349481539895296
author Wang, Jie
Li, Meisheng
Qian, Ming
Zhou, Shouyong
Xue, Ailian
Zhang, Lili
Zhao, Yijiang
Xing, Weihong
author_facet Wang, Jie
Li, Meisheng
Qian, Ming
Zhou, Shouyong
Xue, Ailian
Zhang, Lili
Zhao, Yijiang
Xing, Weihong
author_sort Wang, Jie
collection PubMed
description ABSTRACT: TMC-incorporated carbon nitride (CN) with hexagonal and quadrangle honeycomb-like structure and having periodic lattice defects linked by –CONH– bond was synthesized through combining the high calcination with the chemical condensation of melamine and 1,3,5-benzenetricarbonyl trichloride. The obtained CN has a tri-s-triazine ring and benzene ring skeleton, which makes it have excellent mechanical and thermal stability. The BET specific surface area was enhanced to about 125.6 m(2)/g, and the mean pore size is about 3.43 nm. This CN exhibited an excellent adsorption-enhanced photocatalytic performance. GRAPHICAL ABSTRACT: [Image: see text] ELECTRONIC SUPPLEMENTARY MATERIAL: The online version of this article (10.1186/s11671-018-2654-7) contains supplementary material, which is available to authorized users.
format Online
Article
Text
id pubmed-6104408
institution National Center for Biotechnology Information
language English
publishDate 2018
publisher Springer US
record_format MEDLINE/PubMed
spelling pubmed-61044082018-09-11 Simple Synthesis of High Specific Surface Carbon Nitride for Adsorption-Enhanced Photocatalytic Performance Wang, Jie Li, Meisheng Qian, Ming Zhou, Shouyong Xue, Ailian Zhang, Lili Zhao, Yijiang Xing, Weihong Nanoscale Res Lett Nano Express ABSTRACT: TMC-incorporated carbon nitride (CN) with hexagonal and quadrangle honeycomb-like structure and having periodic lattice defects linked by –CONH– bond was synthesized through combining the high calcination with the chemical condensation of melamine and 1,3,5-benzenetricarbonyl trichloride. The obtained CN has a tri-s-triazine ring and benzene ring skeleton, which makes it have excellent mechanical and thermal stability. The BET specific surface area was enhanced to about 125.6 m(2)/g, and the mean pore size is about 3.43 nm. This CN exhibited an excellent adsorption-enhanced photocatalytic performance. GRAPHICAL ABSTRACT: [Image: see text] ELECTRONIC SUPPLEMENTARY MATERIAL: The online version of this article (10.1186/s11671-018-2654-7) contains supplementary material, which is available to authorized users. Springer US 2018-08-22 /pmc/articles/PMC6104408/ /pubmed/30136161 http://dx.doi.org/10.1186/s11671-018-2654-7 Text en © The Author(s). 2018 Open AccessThis article is distributed under the terms of the Creative Commons Attribution 4.0 International License (http://creativecommons.org/licenses/by/4.0/), which permits unrestricted use, distribution, and reproduction in any medium, provided you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made.
spellingShingle Nano Express
Wang, Jie
Li, Meisheng
Qian, Ming
Zhou, Shouyong
Xue, Ailian
Zhang, Lili
Zhao, Yijiang
Xing, Weihong
Simple Synthesis of High Specific Surface Carbon Nitride for Adsorption-Enhanced Photocatalytic Performance
title Simple Synthesis of High Specific Surface Carbon Nitride for Adsorption-Enhanced Photocatalytic Performance
title_full Simple Synthesis of High Specific Surface Carbon Nitride for Adsorption-Enhanced Photocatalytic Performance
title_fullStr Simple Synthesis of High Specific Surface Carbon Nitride for Adsorption-Enhanced Photocatalytic Performance
title_full_unstemmed Simple Synthesis of High Specific Surface Carbon Nitride for Adsorption-Enhanced Photocatalytic Performance
title_short Simple Synthesis of High Specific Surface Carbon Nitride for Adsorption-Enhanced Photocatalytic Performance
title_sort simple synthesis of high specific surface carbon nitride for adsorption-enhanced photocatalytic performance
topic Nano Express
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6104408/
https://www.ncbi.nlm.nih.gov/pubmed/30136161
http://dx.doi.org/10.1186/s11671-018-2654-7
work_keys_str_mv AT wangjie simplesynthesisofhighspecificsurfacecarbonnitrideforadsorptionenhancedphotocatalyticperformance
AT limeisheng simplesynthesisofhighspecificsurfacecarbonnitrideforadsorptionenhancedphotocatalyticperformance
AT qianming simplesynthesisofhighspecificsurfacecarbonnitrideforadsorptionenhancedphotocatalyticperformance
AT zhoushouyong simplesynthesisofhighspecificsurfacecarbonnitrideforadsorptionenhancedphotocatalyticperformance
AT xueailian simplesynthesisofhighspecificsurfacecarbonnitrideforadsorptionenhancedphotocatalyticperformance
AT zhanglili simplesynthesisofhighspecificsurfacecarbonnitrideforadsorptionenhancedphotocatalyticperformance
AT zhaoyijiang simplesynthesisofhighspecificsurfacecarbonnitrideforadsorptionenhancedphotocatalyticperformance
AT xingweihong simplesynthesisofhighspecificsurfacecarbonnitrideforadsorptionenhancedphotocatalyticperformance

Ejemplares similares