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An eco-friendly synthesized mesoporous-silica particle combined with WSe(2)-graphene-TiO(2) by self-assembled method for photocatalytic dye decomposition and hydrogen production

To address the limitations of titanium dioxide (TiO(2)) and expand the applicability of the photocatalytic activity of TiO(2),WSe(2) and silica, an eco-friendly, self-assembled method for combining a silica precursor with a WSe(2)-graphene-TiO(2) composite with cetyltrimethylammonium bromide (CTAB)...

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Detalles Bibliográficos
Autores principales: Zhu, Lei, Nguyen, Dinh Cung Tien, Woo, Jung-Hun, Zhang, Qinfang, Cho, Kwang Youn, Oh, Won-Chun
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2018
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6109040/
https://www.ncbi.nlm.nih.gov/pubmed/30143720
http://dx.doi.org/10.1038/s41598-018-31188-w
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author Zhu, Lei
Nguyen, Dinh Cung Tien
Woo, Jung-Hun
Zhang, Qinfang
Cho, Kwang Youn
Oh, Won-Chun
author_facet Zhu, Lei
Nguyen, Dinh Cung Tien
Woo, Jung-Hun
Zhang, Qinfang
Cho, Kwang Youn
Oh, Won-Chun
author_sort Zhu, Lei
collection PubMed
description To address the limitations of titanium dioxide (TiO(2)) and expand the applicability of the photocatalytic activity of TiO(2),WSe(2) and silica, an eco-friendly, self-assembled method for combining a silica precursor with a WSe(2)-graphene-TiO(2) composite with cetyltrimethylammonium bromide (CTAB) as surface active agents is proposed. Firstly, for the main target, the photocatalytic degradation of organic dye solutions with different initial pH levels and catalyst dosages under visible light irradiation was surveyed. The as-synthesized sample exhibited highly efficient photocatalytic effects for the treatment of the SO dye solution in the optimal conditions of this study, which included a solution with a pH level of 11 and 0.05-gram dosage of the catalyst. Secondly, previous photocatalytic hydrogen production studies reported markedly better outcomes with SiO(2)/WSe(2)-graphene-TiO(2) than with the binary WSe(2)-graphene and ternary WSe(2)-graphene-TiO(2) composites under ambient conditions with and without 20% methanol sacrificing reagents. The SiO(2)/WSe(2)-graphene-TiO(2) composite is promising to become a potential candidate for photocatalytic performance that performs excellently as well as offer an efficient heterosystem for hydrogen production.
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spelling pubmed-61090402018-08-31 An eco-friendly synthesized mesoporous-silica particle combined with WSe(2)-graphene-TiO(2) by self-assembled method for photocatalytic dye decomposition and hydrogen production Zhu, Lei Nguyen, Dinh Cung Tien Woo, Jung-Hun Zhang, Qinfang Cho, Kwang Youn Oh, Won-Chun Sci Rep Article To address the limitations of titanium dioxide (TiO(2)) and expand the applicability of the photocatalytic activity of TiO(2),WSe(2) and silica, an eco-friendly, self-assembled method for combining a silica precursor with a WSe(2)-graphene-TiO(2) composite with cetyltrimethylammonium bromide (CTAB) as surface active agents is proposed. Firstly, for the main target, the photocatalytic degradation of organic dye solutions with different initial pH levels and catalyst dosages under visible light irradiation was surveyed. The as-synthesized sample exhibited highly efficient photocatalytic effects for the treatment of the SO dye solution in the optimal conditions of this study, which included a solution with a pH level of 11 and 0.05-gram dosage of the catalyst. Secondly, previous photocatalytic hydrogen production studies reported markedly better outcomes with SiO(2)/WSe(2)-graphene-TiO(2) than with the binary WSe(2)-graphene and ternary WSe(2)-graphene-TiO(2) composites under ambient conditions with and without 20% methanol sacrificing reagents. The SiO(2)/WSe(2)-graphene-TiO(2) composite is promising to become a potential candidate for photocatalytic performance that performs excellently as well as offer an efficient heterosystem for hydrogen production. Nature Publishing Group UK 2018-08-24 /pmc/articles/PMC6109040/ /pubmed/30143720 http://dx.doi.org/10.1038/s41598-018-31188-w Text en © The Author(s) 2018 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Zhu, Lei
Nguyen, Dinh Cung Tien
Woo, Jung-Hun
Zhang, Qinfang
Cho, Kwang Youn
Oh, Won-Chun
An eco-friendly synthesized mesoporous-silica particle combined with WSe(2)-graphene-TiO(2) by self-assembled method for photocatalytic dye decomposition and hydrogen production
title An eco-friendly synthesized mesoporous-silica particle combined with WSe(2)-graphene-TiO(2) by self-assembled method for photocatalytic dye decomposition and hydrogen production
title_full An eco-friendly synthesized mesoporous-silica particle combined with WSe(2)-graphene-TiO(2) by self-assembled method for photocatalytic dye decomposition and hydrogen production
title_fullStr An eco-friendly synthesized mesoporous-silica particle combined with WSe(2)-graphene-TiO(2) by self-assembled method for photocatalytic dye decomposition and hydrogen production
title_full_unstemmed An eco-friendly synthesized mesoporous-silica particle combined with WSe(2)-graphene-TiO(2) by self-assembled method for photocatalytic dye decomposition and hydrogen production
title_short An eco-friendly synthesized mesoporous-silica particle combined with WSe(2)-graphene-TiO(2) by self-assembled method for photocatalytic dye decomposition and hydrogen production
title_sort eco-friendly synthesized mesoporous-silica particle combined with wse(2)-graphene-tio(2) by self-assembled method for photocatalytic dye decomposition and hydrogen production
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6109040/
https://www.ncbi.nlm.nih.gov/pubmed/30143720
http://dx.doi.org/10.1038/s41598-018-31188-w
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