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Biexcitons in monolayer transition metal dichalcogenides tuned by magnetic fields

We present time-integrated four-wave mixing measurements on monolayer MoSe(2) in magnetic fields up to 25 T. The experimental data together with time-dependent density function theory calculations provide interesting insights into the biexciton formation and dynamics. In the presence of magnetic fie...

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Detalles Bibliográficos
Autores principales: Stevens, Christopher. E., Paul, Jagannath, Cox, Timothy, Sahoo, Prasana K., Gutiérrez, Humberto R., Turkowski, Volodymyr, Semenov, Dimitry, McGill, Steven A., Kapetanakis, Myron D., Perakis, Ilias E., Hilton, David J., Karaiskaj, Denis
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2018
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6137096/
https://www.ncbi.nlm.nih.gov/pubmed/30213976
http://dx.doi.org/10.1038/s41467-018-05643-1
Descripción
Sumario:We present time-integrated four-wave mixing measurements on monolayer MoSe(2) in magnetic fields up to 25 T. The experimental data together with time-dependent density function theory calculations provide interesting insights into the biexciton formation and dynamics. In the presence of magnetic fields the coherence at negative and positive time delays is dominated by intervalley biexcitons. We demonstrate that magnetic fields can serve as a control to enhance the biexciton formation and help search for more exotic states of matter, including the creation of multiple exciton complexes and excitonic condensates.