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Biexcitons in monolayer transition metal dichalcogenides tuned by magnetic fields

We present time-integrated four-wave mixing measurements on monolayer MoSe(2) in magnetic fields up to 25 T. The experimental data together with time-dependent density function theory calculations provide interesting insights into the biexciton formation and dynamics. In the presence of magnetic fie...

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Autores principales: Stevens, Christopher. E., Paul, Jagannath, Cox, Timothy, Sahoo, Prasana K., Gutiérrez, Humberto R., Turkowski, Volodymyr, Semenov, Dimitry, McGill, Steven A., Kapetanakis, Myron D., Perakis, Ilias E., Hilton, David J., Karaiskaj, Denis
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2018
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6137096/
https://www.ncbi.nlm.nih.gov/pubmed/30213976
http://dx.doi.org/10.1038/s41467-018-05643-1
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author Stevens, Christopher. E.
Paul, Jagannath
Cox, Timothy
Sahoo, Prasana K.
Gutiérrez, Humberto R.
Turkowski, Volodymyr
Semenov, Dimitry
McGill, Steven A.
Kapetanakis, Myron D.
Perakis, Ilias E.
Hilton, David J.
Karaiskaj, Denis
author_facet Stevens, Christopher. E.
Paul, Jagannath
Cox, Timothy
Sahoo, Prasana K.
Gutiérrez, Humberto R.
Turkowski, Volodymyr
Semenov, Dimitry
McGill, Steven A.
Kapetanakis, Myron D.
Perakis, Ilias E.
Hilton, David J.
Karaiskaj, Denis
author_sort Stevens, Christopher. E.
collection PubMed
description We present time-integrated four-wave mixing measurements on monolayer MoSe(2) in magnetic fields up to 25 T. The experimental data together with time-dependent density function theory calculations provide interesting insights into the biexciton formation and dynamics. In the presence of magnetic fields the coherence at negative and positive time delays is dominated by intervalley biexcitons. We demonstrate that magnetic fields can serve as a control to enhance the biexciton formation and help search for more exotic states of matter, including the creation of multiple exciton complexes and excitonic condensates.
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spelling pubmed-61370962018-09-17 Biexcitons in monolayer transition metal dichalcogenides tuned by magnetic fields Stevens, Christopher. E. Paul, Jagannath Cox, Timothy Sahoo, Prasana K. Gutiérrez, Humberto R. Turkowski, Volodymyr Semenov, Dimitry McGill, Steven A. Kapetanakis, Myron D. Perakis, Ilias E. Hilton, David J. Karaiskaj, Denis Nat Commun Article We present time-integrated four-wave mixing measurements on monolayer MoSe(2) in magnetic fields up to 25 T. The experimental data together with time-dependent density function theory calculations provide interesting insights into the biexciton formation and dynamics. In the presence of magnetic fields the coherence at negative and positive time delays is dominated by intervalley biexcitons. We demonstrate that magnetic fields can serve as a control to enhance the biexciton formation and help search for more exotic states of matter, including the creation of multiple exciton complexes and excitonic condensates. Nature Publishing Group UK 2018-09-13 /pmc/articles/PMC6137096/ /pubmed/30213976 http://dx.doi.org/10.1038/s41467-018-05643-1 Text en © The Author(s) 2018 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Stevens, Christopher. E.
Paul, Jagannath
Cox, Timothy
Sahoo, Prasana K.
Gutiérrez, Humberto R.
Turkowski, Volodymyr
Semenov, Dimitry
McGill, Steven A.
Kapetanakis, Myron D.
Perakis, Ilias E.
Hilton, David J.
Karaiskaj, Denis
Biexcitons in monolayer transition metal dichalcogenides tuned by magnetic fields
title Biexcitons in monolayer transition metal dichalcogenides tuned by magnetic fields
title_full Biexcitons in monolayer transition metal dichalcogenides tuned by magnetic fields
title_fullStr Biexcitons in monolayer transition metal dichalcogenides tuned by magnetic fields
title_full_unstemmed Biexcitons in monolayer transition metal dichalcogenides tuned by magnetic fields
title_short Biexcitons in monolayer transition metal dichalcogenides tuned by magnetic fields
title_sort biexcitons in monolayer transition metal dichalcogenides tuned by magnetic fields
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6137096/
https://www.ncbi.nlm.nih.gov/pubmed/30213976
http://dx.doi.org/10.1038/s41467-018-05643-1
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