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Biexcitons in monolayer transition metal dichalcogenides tuned by magnetic fields
We present time-integrated four-wave mixing measurements on monolayer MoSe(2) in magnetic fields up to 25 T. The experimental data together with time-dependent density function theory calculations provide interesting insights into the biexciton formation and dynamics. In the presence of magnetic fie...
Autores principales: | , , , , , , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group UK
2018
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6137096/ https://www.ncbi.nlm.nih.gov/pubmed/30213976 http://dx.doi.org/10.1038/s41467-018-05643-1 |
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author | Stevens, Christopher. E. Paul, Jagannath Cox, Timothy Sahoo, Prasana K. Gutiérrez, Humberto R. Turkowski, Volodymyr Semenov, Dimitry McGill, Steven A. Kapetanakis, Myron D. Perakis, Ilias E. Hilton, David J. Karaiskaj, Denis |
author_facet | Stevens, Christopher. E. Paul, Jagannath Cox, Timothy Sahoo, Prasana K. Gutiérrez, Humberto R. Turkowski, Volodymyr Semenov, Dimitry McGill, Steven A. Kapetanakis, Myron D. Perakis, Ilias E. Hilton, David J. Karaiskaj, Denis |
author_sort | Stevens, Christopher. E. |
collection | PubMed |
description | We present time-integrated four-wave mixing measurements on monolayer MoSe(2) in magnetic fields up to 25 T. The experimental data together with time-dependent density function theory calculations provide interesting insights into the biexciton formation and dynamics. In the presence of magnetic fields the coherence at negative and positive time delays is dominated by intervalley biexcitons. We demonstrate that magnetic fields can serve as a control to enhance the biexciton formation and help search for more exotic states of matter, including the creation of multiple exciton complexes and excitonic condensates. |
format | Online Article Text |
id | pubmed-6137096 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2018 |
publisher | Nature Publishing Group UK |
record_format | MEDLINE/PubMed |
spelling | pubmed-61370962018-09-17 Biexcitons in monolayer transition metal dichalcogenides tuned by magnetic fields Stevens, Christopher. E. Paul, Jagannath Cox, Timothy Sahoo, Prasana K. Gutiérrez, Humberto R. Turkowski, Volodymyr Semenov, Dimitry McGill, Steven A. Kapetanakis, Myron D. Perakis, Ilias E. Hilton, David J. Karaiskaj, Denis Nat Commun Article We present time-integrated four-wave mixing measurements on monolayer MoSe(2) in magnetic fields up to 25 T. The experimental data together with time-dependent density function theory calculations provide interesting insights into the biexciton formation and dynamics. In the presence of magnetic fields the coherence at negative and positive time delays is dominated by intervalley biexcitons. We demonstrate that magnetic fields can serve as a control to enhance the biexciton formation and help search for more exotic states of matter, including the creation of multiple exciton complexes and excitonic condensates. Nature Publishing Group UK 2018-09-13 /pmc/articles/PMC6137096/ /pubmed/30213976 http://dx.doi.org/10.1038/s41467-018-05643-1 Text en © The Author(s) 2018 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/. |
spellingShingle | Article Stevens, Christopher. E. Paul, Jagannath Cox, Timothy Sahoo, Prasana K. Gutiérrez, Humberto R. Turkowski, Volodymyr Semenov, Dimitry McGill, Steven A. Kapetanakis, Myron D. Perakis, Ilias E. Hilton, David J. Karaiskaj, Denis Biexcitons in monolayer transition metal dichalcogenides tuned by magnetic fields |
title | Biexcitons in monolayer transition metal dichalcogenides tuned by magnetic fields |
title_full | Biexcitons in monolayer transition metal dichalcogenides tuned by magnetic fields |
title_fullStr | Biexcitons in monolayer transition metal dichalcogenides tuned by magnetic fields |
title_full_unstemmed | Biexcitons in monolayer transition metal dichalcogenides tuned by magnetic fields |
title_short | Biexcitons in monolayer transition metal dichalcogenides tuned by magnetic fields |
title_sort | biexcitons in monolayer transition metal dichalcogenides tuned by magnetic fields |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6137096/ https://www.ncbi.nlm.nih.gov/pubmed/30213976 http://dx.doi.org/10.1038/s41467-018-05643-1 |
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