Facile manufacture of porous organic framework membranes for precombustion CO(2) capture

The development of new membranes with high H(2) separation performance under industrially relevant conditions (high temperatures and pressures) is of primary importance. For instance, these membranes may facilitate the implementation of energy-efficient precombustion CO(2) capture or reduce energy i...

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Detalles Bibliográficos
Autores principales: Shan, Meixia, Liu, Xinlei, Wang, Xuerui, Yarulina, Irina, Seoane, Beatriz, Kapteijn, Freek, Gascon, Jorge
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Association for the Advancement of Science 2018
Materias:
Research Articles
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6155097/
https://www.ncbi.nlm.nih.gov/pubmed/30255154
http://dx.doi.org/10.1126/sciadv.aau1698
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author Shan, Meixia
Liu, Xinlei
Wang, Xuerui
Yarulina, Irina
Seoane, Beatriz
Kapteijn, Freek
Gascon, Jorge
author_facet Shan, Meixia
Liu, Xinlei
Wang, Xuerui
Yarulina, Irina
Seoane, Beatriz
Kapteijn, Freek
Gascon, Jorge
author_sort Shan, Meixia
collection PubMed
description The development of new membranes with high H(2) separation performance under industrially relevant conditions (high temperatures and pressures) is of primary importance. For instance, these membranes may facilitate the implementation of energy-efficient precombustion CO(2) capture or reduce energy intensity in other industrial processes such as ammonia synthesis. We report a facile synthetic protocol based on interfacial polymerization for the fabrication of supported benzimidazole-linked polymer membranes that display an unprecedented H(2)/CO(2) selectivity (up to 40) at 423 K together with high-pressure resistance and long-term stability (>800 hours in the presence of water vapor).
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spelling pubmed-61550972018-09-25 Facile manufacture of porous organic framework membranes for precombustion CO(2) capture Shan, Meixia Liu, Xinlei Wang, Xuerui Yarulina, Irina Seoane, Beatriz Kapteijn, Freek Gascon, Jorge Sci Adv Research Articles The development of new membranes with high H(2) separation performance under industrially relevant conditions (high temperatures and pressures) is of primary importance. For instance, these membranes may facilitate the implementation of energy-efficient precombustion CO(2) capture or reduce energy intensity in other industrial processes such as ammonia synthesis. We report a facile synthetic protocol based on interfacial polymerization for the fabrication of supported benzimidazole-linked polymer membranes that display an unprecedented H(2)/CO(2) selectivity (up to 40) at 423 K together with high-pressure resistance and long-term stability (>800 hours in the presence of water vapor). American Association for the Advancement of Science 2018-09-21 /pmc/articles/PMC6155097/ /pubmed/30255154 http://dx.doi.org/10.1126/sciadv.aau1698 Text en Copyright © 2018 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution NonCommercial License 4.0 (CC BY-NC). http://creativecommons.org/licenses/by-nc/4.0/ This is an open-access article distributed under the terms of the Creative Commons Attribution-NonCommercial license (http://creativecommons.org/licenses/by-nc/4.0/) , which permits use, distribution, and reproduction in any medium, so long as the resultant use is not for commercial advantage and provided the original work is properly cited.
spellingShingle Research Articles
Shan, Meixia
Liu, Xinlei
Wang, Xuerui
Yarulina, Irina
Seoane, Beatriz
Kapteijn, Freek
Gascon, Jorge
Facile manufacture of porous organic framework membranes for precombustion CO(2) capture
title Facile manufacture of porous organic framework membranes for precombustion CO(2) capture
title_full Facile manufacture of porous organic framework membranes for precombustion CO(2) capture
title_fullStr Facile manufacture of porous organic framework membranes for precombustion CO(2) capture
title_full_unstemmed Facile manufacture of porous organic framework membranes for precombustion CO(2) capture
title_short Facile manufacture of porous organic framework membranes for precombustion CO(2) capture
title_sort facile manufacture of porous organic framework membranes for precombustion co(2) capture
topic Research Articles
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6155097/
https://www.ncbi.nlm.nih.gov/pubmed/30255154
http://dx.doi.org/10.1126/sciadv.aau1698
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