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Dielectric Response of Quantum Critical Ferroelectric as a Function of Pressure

In this work we report for the first time measurements of the dielectric loss of single-crystal SrTiO(3) under the application of hydrostatic pressure up to 20 kbar and temperatures down to 200 mK which allow us to comment on the evolution of new fundamental material properties and their relationshi...

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Autores principales: Coak, M. J., Haines, C. R. S., Liu, C., Jarvis, D. M., Littlewood, P. B., Saxena, S. S.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2018
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6175889/
https://www.ncbi.nlm.nih.gov/pubmed/30297803
http://dx.doi.org/10.1038/s41598-018-33320-2
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author Coak, M. J.
Haines, C. R. S.
Liu, C.
Jarvis, D. M.
Littlewood, P. B.
Saxena, S. S.
author_facet Coak, M. J.
Haines, C. R. S.
Liu, C.
Jarvis, D. M.
Littlewood, P. B.
Saxena, S. S.
author_sort Coak, M. J.
collection PubMed
description In this work we report for the first time measurements of the dielectric loss of single-crystal SrTiO(3) under the application of hydrostatic pressure up to 20 kbar and temperatures down to 200 mK which allow us to comment on the evolution of new fundamental material properties and their relationship with the recently discovered quantum critical phenomena in this material. The well known 18 K peak or shoulder was no longer observed after pressure was applied, even after subsequently removing it, suggesting it is associated with the twin walls formed at the 110 K cubic-tetragonal transition. The family of familiar peaks were all seen to increase in temperature linearly with pressure and the height of the 9.4 K peak was drastically suppressed by even the smallest pressures. This peak is discussed in the context of a postulated ferroelectric quantum critical point in SrTiO(3) and the behaviour of its size linked to the position of this point on the recently established phase diagram.
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spelling pubmed-61758892018-10-12 Dielectric Response of Quantum Critical Ferroelectric as a Function of Pressure Coak, M. J. Haines, C. R. S. Liu, C. Jarvis, D. M. Littlewood, P. B. Saxena, S. S. Sci Rep Article In this work we report for the first time measurements of the dielectric loss of single-crystal SrTiO(3) under the application of hydrostatic pressure up to 20 kbar and temperatures down to 200 mK which allow us to comment on the evolution of new fundamental material properties and their relationship with the recently discovered quantum critical phenomena in this material. The well known 18 K peak or shoulder was no longer observed after pressure was applied, even after subsequently removing it, suggesting it is associated with the twin walls formed at the 110 K cubic-tetragonal transition. The family of familiar peaks were all seen to increase in temperature linearly with pressure and the height of the 9.4 K peak was drastically suppressed by even the smallest pressures. This peak is discussed in the context of a postulated ferroelectric quantum critical point in SrTiO(3) and the behaviour of its size linked to the position of this point on the recently established phase diagram. Nature Publishing Group UK 2018-10-08 /pmc/articles/PMC6175889/ /pubmed/30297803 http://dx.doi.org/10.1038/s41598-018-33320-2 Text en © The Author(s) 2018 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Coak, M. J.
Haines, C. R. S.
Liu, C.
Jarvis, D. M.
Littlewood, P. B.
Saxena, S. S.
Dielectric Response of Quantum Critical Ferroelectric as a Function of Pressure
title Dielectric Response of Quantum Critical Ferroelectric as a Function of Pressure
title_full Dielectric Response of Quantum Critical Ferroelectric as a Function of Pressure
title_fullStr Dielectric Response of Quantum Critical Ferroelectric as a Function of Pressure
title_full_unstemmed Dielectric Response of Quantum Critical Ferroelectric as a Function of Pressure
title_short Dielectric Response of Quantum Critical Ferroelectric as a Function of Pressure
title_sort dielectric response of quantum critical ferroelectric as a function of pressure
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6175889/
https://www.ncbi.nlm.nih.gov/pubmed/30297803
http://dx.doi.org/10.1038/s41598-018-33320-2
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