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Improved catalytic combustion of methane using CuO nanobelts with predominantly (001) surfaces

Through computational calculations, CuO(001) has been identified as an active surface for methane oxidation. Experimental validation with CuO nanobelts comprised of predominantly (001) surfaces has been performed and it is confirmed that the performance of such nanobelts is much higher than normal n...

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Autores principales: Kong, Qingquan, Yin, Yichun, Xue, Bing, Jin, Yonggang, Feng, Wei, Chen, Zhi-Gang, Su, Shi, Sun, Chenghua
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Beilstein-Institut 2018
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6176823/
https://www.ncbi.nlm.nih.gov/pubmed/30345215
http://dx.doi.org/10.3762/bjnano.9.235
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author Kong, Qingquan
Yin, Yichun
Xue, Bing
Jin, Yonggang
Feng, Wei
Chen, Zhi-Gang
Su, Shi
Sun, Chenghua
author_facet Kong, Qingquan
Yin, Yichun
Xue, Bing
Jin, Yonggang
Feng, Wei
Chen, Zhi-Gang
Su, Shi
Sun, Chenghua
author_sort Kong, Qingquan
collection PubMed
description Through computational calculations, CuO(001) has been identified as an active surface for methane oxidation. Experimental validation with CuO nanobelts comprised of predominantly (001) surfaces has been performed and it is confirmed that the performance of such nanobelts is much higher than normal nanoparticles and nanowires. First principle calculations further clarified that two-coordinated oxygen plays a key role for methane adsorption and oxidation.
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spelling pubmed-61768232018-10-19 Improved catalytic combustion of methane using CuO nanobelts with predominantly (001) surfaces Kong, Qingquan Yin, Yichun Xue, Bing Jin, Yonggang Feng, Wei Chen, Zhi-Gang Su, Shi Sun, Chenghua Beilstein J Nanotechnol Full Research Paper Through computational calculations, CuO(001) has been identified as an active surface for methane oxidation. Experimental validation with CuO nanobelts comprised of predominantly (001) surfaces has been performed and it is confirmed that the performance of such nanobelts is much higher than normal nanoparticles and nanowires. First principle calculations further clarified that two-coordinated oxygen plays a key role for methane adsorption and oxidation. Beilstein-Institut 2018-09-24 /pmc/articles/PMC6176823/ /pubmed/30345215 http://dx.doi.org/10.3762/bjnano.9.235 Text en Copyright © 2018, Kong et al. https://creativecommons.org/licenses/by/4.0https://www.beilstein-journals.org/bjnano/termsThis is an Open Access article under the terms of the Creative Commons Attribution License (https://creativecommons.org/licenses/by/4.0). Please note that the reuse, redistribution and reproduction in particular requires that the authors and source are credited. The license is subject to the Beilstein Journal of Nanotechnology terms and conditions: (https://www.beilstein-journals.org/bjnano/terms)
spellingShingle Full Research Paper
Kong, Qingquan
Yin, Yichun
Xue, Bing
Jin, Yonggang
Feng, Wei
Chen, Zhi-Gang
Su, Shi
Sun, Chenghua
Improved catalytic combustion of methane using CuO nanobelts with predominantly (001) surfaces
title Improved catalytic combustion of methane using CuO nanobelts with predominantly (001) surfaces
title_full Improved catalytic combustion of methane using CuO nanobelts with predominantly (001) surfaces
title_fullStr Improved catalytic combustion of methane using CuO nanobelts with predominantly (001) surfaces
title_full_unstemmed Improved catalytic combustion of methane using CuO nanobelts with predominantly (001) surfaces
title_short Improved catalytic combustion of methane using CuO nanobelts with predominantly (001) surfaces
title_sort improved catalytic combustion of methane using cuo nanobelts with predominantly (001) surfaces
topic Full Research Paper
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6176823/
https://www.ncbi.nlm.nih.gov/pubmed/30345215
http://dx.doi.org/10.3762/bjnano.9.235
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