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Breaking the scaling relationship via thermally stable Pt/Cu single atom alloys for catalytic dehydrogenation

Noble-metal alloys are widely used as heterogeneous catalysts. However, due to the existence of scaling properties of adsorption energies on transition metal surfaces, the enhancement of catalytic activity is frequently accompanied by side reactions leading to a reduction in selectivity for the targ...

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Autores principales: Sun, Guodong, Zhao, Zhi-Jian, Mu, Rentao, Zha, Shenjun, Li, Lulu, Chen, Sai, Zang, Ketao, Luo, Jun, Li, Zhenglong, Purdy, Stephen C., Kropf, A. Jeremy, Miller, Jeffrey T., Zeng, Liang, Gong, Jinlong
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2018
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6203812/
https://www.ncbi.nlm.nih.gov/pubmed/30367052
http://dx.doi.org/10.1038/s41467-018-06967-8
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author Sun, Guodong
Zhao, Zhi-Jian
Mu, Rentao
Zha, Shenjun
Li, Lulu
Chen, Sai
Zang, Ketao
Luo, Jun
Li, Zhenglong
Purdy, Stephen C.
Kropf, A. Jeremy
Miller, Jeffrey T.
Zeng, Liang
Gong, Jinlong
author_facet Sun, Guodong
Zhao, Zhi-Jian
Mu, Rentao
Zha, Shenjun
Li, Lulu
Chen, Sai
Zang, Ketao
Luo, Jun
Li, Zhenglong
Purdy, Stephen C.
Kropf, A. Jeremy
Miller, Jeffrey T.
Zeng, Liang
Gong, Jinlong
author_sort Sun, Guodong
collection PubMed
description Noble-metal alloys are widely used as heterogeneous catalysts. However, due to the existence of scaling properties of adsorption energies on transition metal surfaces, the enhancement of catalytic activity is frequently accompanied by side reactions leading to a reduction in selectivity for the target product. Herein, we describe an approach to breaking the scaling relationship for propane dehydrogenation, an industrially important reaction, by assembling single atom alloys (SAAs), to achieve simultaneous enhancement of propylene selectivity and propane conversion. We synthesize γ-alumina-supported platinum/copper SAA catalysts by incipient wetness co-impregnation method with a high copper to platinum ratio. Single platinum atoms dispersed on copper nanoparticles dramatically enhance the desorption of surface-bounded propylene and prohibit its further dehydrogenation, resulting in high propylene selectivity (~90%). Unlike previous reported SAA applications at low temperatures (<400 °C), Pt/Cu SAA shows excellent stability of more than 120 h of operation under atmospheric pressure at 520 °C.
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spelling pubmed-62038122018-10-29 Breaking the scaling relationship via thermally stable Pt/Cu single atom alloys for catalytic dehydrogenation Sun, Guodong Zhao, Zhi-Jian Mu, Rentao Zha, Shenjun Li, Lulu Chen, Sai Zang, Ketao Luo, Jun Li, Zhenglong Purdy, Stephen C. Kropf, A. Jeremy Miller, Jeffrey T. Zeng, Liang Gong, Jinlong Nat Commun Article Noble-metal alloys are widely used as heterogeneous catalysts. However, due to the existence of scaling properties of adsorption energies on transition metal surfaces, the enhancement of catalytic activity is frequently accompanied by side reactions leading to a reduction in selectivity for the target product. Herein, we describe an approach to breaking the scaling relationship for propane dehydrogenation, an industrially important reaction, by assembling single atom alloys (SAAs), to achieve simultaneous enhancement of propylene selectivity and propane conversion. We synthesize γ-alumina-supported platinum/copper SAA catalysts by incipient wetness co-impregnation method with a high copper to platinum ratio. Single platinum atoms dispersed on copper nanoparticles dramatically enhance the desorption of surface-bounded propylene and prohibit its further dehydrogenation, resulting in high propylene selectivity (~90%). Unlike previous reported SAA applications at low temperatures (<400 °C), Pt/Cu SAA shows excellent stability of more than 120 h of operation under atmospheric pressure at 520 °C. Nature Publishing Group UK 2018-10-26 /pmc/articles/PMC6203812/ /pubmed/30367052 http://dx.doi.org/10.1038/s41467-018-06967-8 Text en © The Author(s) 2018 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Sun, Guodong
Zhao, Zhi-Jian
Mu, Rentao
Zha, Shenjun
Li, Lulu
Chen, Sai
Zang, Ketao
Luo, Jun
Li, Zhenglong
Purdy, Stephen C.
Kropf, A. Jeremy
Miller, Jeffrey T.
Zeng, Liang
Gong, Jinlong
Breaking the scaling relationship via thermally stable Pt/Cu single atom alloys for catalytic dehydrogenation
title Breaking the scaling relationship via thermally stable Pt/Cu single atom alloys for catalytic dehydrogenation
title_full Breaking the scaling relationship via thermally stable Pt/Cu single atom alloys for catalytic dehydrogenation
title_fullStr Breaking the scaling relationship via thermally stable Pt/Cu single atom alloys for catalytic dehydrogenation
title_full_unstemmed Breaking the scaling relationship via thermally stable Pt/Cu single atom alloys for catalytic dehydrogenation
title_short Breaking the scaling relationship via thermally stable Pt/Cu single atom alloys for catalytic dehydrogenation
title_sort breaking the scaling relationship via thermally stable pt/cu single atom alloys for catalytic dehydrogenation
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6203812/
https://www.ncbi.nlm.nih.gov/pubmed/30367052
http://dx.doi.org/10.1038/s41467-018-06967-8
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