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Forced Magnetostrictions and Magnetizations of Ni(2+x)MnGa(1−x) at Its Curie Temperature

Experimental investigations into the field dependence of magnetization and the relationship between magnetization and magnetostriction in Ni(2+x)MnGa(1−x) (x = 0.00, 0.02, 0.04) alloy ferromagnets were performed following the self-consistent renormalization (SCR) spin fluctuation theory of itinerant...

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Autores principales: Sakon, Takuo, Hayashi, Yuhi, Li, Dexin, Honda, Fuminori, Oomi, Gendo, Narumi, Yasuo, Hagiwara, Masayuki, Kanomata, Takeshi, Eto, Tetsujiro
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2018
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6266816/
https://www.ncbi.nlm.nih.gov/pubmed/30373290
http://dx.doi.org/10.3390/ma11112115
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author Sakon, Takuo
Hayashi, Yuhi
Li, Dexin
Honda, Fuminori
Oomi, Gendo
Narumi, Yasuo
Hagiwara, Masayuki
Kanomata, Takeshi
Eto, Tetsujiro
author_facet Sakon, Takuo
Hayashi, Yuhi
Li, Dexin
Honda, Fuminori
Oomi, Gendo
Narumi, Yasuo
Hagiwara, Masayuki
Kanomata, Takeshi
Eto, Tetsujiro
author_sort Sakon, Takuo
collection PubMed
description Experimental investigations into the field dependence of magnetization and the relationship between magnetization and magnetostriction in Ni(2+x)MnGa(1−x) (x = 0.00, 0.02, 0.04) alloy ferromagnets were performed following the self-consistent renormalization (SCR) spin fluctuation theory of itinerant ferromagnetism. In this study, we investigated the magnetization of and magnetostriction on Ni(2+x)MnGa(1−x) (x = 0.02, 0.04) to check whether these relations held when the ratio of Ni to Ga and, the valence electron concentration per atom, e/a were varied. When the ratio of Ni to Ga was varied, e/a increased with increasing x. The magnetization results for x = 0.02 (e/a = 7.535) and 0.04 (e/a = 7.570) suggest that the critical index δ of H ∝ M(δ) is around 5.0 at the Curie temperature T(C), which is the critical temperature of the ferromagnetic–paramagnetic transition. This result confirms Takahashi’s spin fluctuation theory and the experimental results of Ni(2)MnGa. The spontaneous magnetization p(S) slightly decreased with increasing x. For x = 0.00, the spin fluctuation parameter in k-space (momentum space; T(A)) and that in energy space (T(0)) were obtained. The relationship between p(eff)/p(S) and T(C)/T(0) can also be explained by Takahashi’s theory, where p(eff) indicates the effective magnetic moments. We created a generalized Rhodes-Wohlfarth plot of p(eff)/p(S) versus T(C)/T(0) for other ferromagnets. The plot indicates that the relationship between p(eff)/p(S) and T(0)/T(C) follows Takahashi’s theory. We also measured the magnetostriction for Ni(2+x)MnGa(1−x) (x = 0.02, 0.04). As a result, at T(C), the plot of the magnetostriction (ΔL/L) versus M(4) shows proportionality and crosses the origin. These magnetization and magnetostriction results were analyzed in terms of Takahashi’s SCR spin fluctuation theory. We investigated the magnetostriction at the premartensite phase, which is the precursor state to the martensitic transition. In Ni(2)MnGa system alloys, the maximum value of magnetostriction is almost proportional to the e/a.
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spelling pubmed-62668162018-12-17 Forced Magnetostrictions and Magnetizations of Ni(2+x)MnGa(1−x) at Its Curie Temperature Sakon, Takuo Hayashi, Yuhi Li, Dexin Honda, Fuminori Oomi, Gendo Narumi, Yasuo Hagiwara, Masayuki Kanomata, Takeshi Eto, Tetsujiro Materials (Basel) Article Experimental investigations into the field dependence of magnetization and the relationship between magnetization and magnetostriction in Ni(2+x)MnGa(1−x) (x = 0.00, 0.02, 0.04) alloy ferromagnets were performed following the self-consistent renormalization (SCR) spin fluctuation theory of itinerant ferromagnetism. In this study, we investigated the magnetization of and magnetostriction on Ni(2+x)MnGa(1−x) (x = 0.02, 0.04) to check whether these relations held when the ratio of Ni to Ga and, the valence electron concentration per atom, e/a were varied. When the ratio of Ni to Ga was varied, e/a increased with increasing x. The magnetization results for x = 0.02 (e/a = 7.535) and 0.04 (e/a = 7.570) suggest that the critical index δ of H ∝ M(δ) is around 5.0 at the Curie temperature T(C), which is the critical temperature of the ferromagnetic–paramagnetic transition. This result confirms Takahashi’s spin fluctuation theory and the experimental results of Ni(2)MnGa. The spontaneous magnetization p(S) slightly decreased with increasing x. For x = 0.00, the spin fluctuation parameter in k-space (momentum space; T(A)) and that in energy space (T(0)) were obtained. The relationship between p(eff)/p(S) and T(C)/T(0) can also be explained by Takahashi’s theory, where p(eff) indicates the effective magnetic moments. We created a generalized Rhodes-Wohlfarth plot of p(eff)/p(S) versus T(C)/T(0) for other ferromagnets. The plot indicates that the relationship between p(eff)/p(S) and T(0)/T(C) follows Takahashi’s theory. We also measured the magnetostriction for Ni(2+x)MnGa(1−x) (x = 0.02, 0.04). As a result, at T(C), the plot of the magnetostriction (ΔL/L) versus M(4) shows proportionality and crosses the origin. These magnetization and magnetostriction results were analyzed in terms of Takahashi’s SCR spin fluctuation theory. We investigated the magnetostriction at the premartensite phase, which is the precursor state to the martensitic transition. In Ni(2)MnGa system alloys, the maximum value of magnetostriction is almost proportional to the e/a. MDPI 2018-10-28 /pmc/articles/PMC6266816/ /pubmed/30373290 http://dx.doi.org/10.3390/ma11112115 Text en © 2018 by the authors. Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (http://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Sakon, Takuo
Hayashi, Yuhi
Li, Dexin
Honda, Fuminori
Oomi, Gendo
Narumi, Yasuo
Hagiwara, Masayuki
Kanomata, Takeshi
Eto, Tetsujiro
Forced Magnetostrictions and Magnetizations of Ni(2+x)MnGa(1−x) at Its Curie Temperature
title Forced Magnetostrictions and Magnetizations of Ni(2+x)MnGa(1−x) at Its Curie Temperature
title_full Forced Magnetostrictions and Magnetizations of Ni(2+x)MnGa(1−x) at Its Curie Temperature
title_fullStr Forced Magnetostrictions and Magnetizations of Ni(2+x)MnGa(1−x) at Its Curie Temperature
title_full_unstemmed Forced Magnetostrictions and Magnetizations of Ni(2+x)MnGa(1−x) at Its Curie Temperature
title_short Forced Magnetostrictions and Magnetizations of Ni(2+x)MnGa(1−x) at Its Curie Temperature
title_sort forced magnetostrictions and magnetizations of ni(2+x)mnga(1−x) at its curie temperature
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6266816/
https://www.ncbi.nlm.nih.gov/pubmed/30373290
http://dx.doi.org/10.3390/ma11112115
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