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Sea Spray Aerosol: Where Marine Biology Meets Atmospheric Chemistry

[Image: see text] Atmospheric aerosols have long been known to alter climate by scattering incoming solar radiation and acting as seeds for cloud formation. These processes have vast implications for controlling the chemistry of our environment and the Earth’s climate. Sea spray aerosol (SSA) is emi...

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Autores principales: Schiffer, Jamie M., Mael, Liora E., Prather, Kimberly A., Amaro, Rommie E., Grassian, Vicki H.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2018
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6311946/
https://www.ncbi.nlm.nih.gov/pubmed/30648145
http://dx.doi.org/10.1021/acscentsci.8b00674
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author Schiffer, Jamie M.
Mael, Liora E.
Prather, Kimberly A.
Amaro, Rommie E.
Grassian, Vicki H.
author_facet Schiffer, Jamie M.
Mael, Liora E.
Prather, Kimberly A.
Amaro, Rommie E.
Grassian, Vicki H.
author_sort Schiffer, Jamie M.
collection PubMed
description [Image: see text] Atmospheric aerosols have long been known to alter climate by scattering incoming solar radiation and acting as seeds for cloud formation. These processes have vast implications for controlling the chemistry of our environment and the Earth’s climate. Sea spray aerosol (SSA) is emitted over nearly three-quarters of our planet, yet precisely how SSA impacts Earth’s radiation budget remains highly uncertain. Over the past several decades, studies have shown that SSA particles are far more complex than just sea salt. Ocean biological and physical processes produce individual SSA particles containing a diverse array of biological species including proteins, enzymes, bacteria, and viruses and a diverse array of organic compounds including fatty acids and sugars. Thus, a new frontier of research is emerging at the nexus of chemistry, biology, and atmospheric science. In this Outlook article, we discuss how current and future aerosol chemistry research demands a tight coupling between experimental (observational and laboratory studies) and computational (simulation-based) methods. This integration of approaches will enable the systematic interrogation of the complexity within individual SSA particles at a level that will enable prediction of the physicochemical properties of real-world SSA, ultimately illuminating the detailed mechanisms of how the constituents within individual SSA impact climate.
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spelling pubmed-63119462019-01-15 Sea Spray Aerosol: Where Marine Biology Meets Atmospheric Chemistry Schiffer, Jamie M. Mael, Liora E. Prather, Kimberly A. Amaro, Rommie E. Grassian, Vicki H. ACS Cent Sci [Image: see text] Atmospheric aerosols have long been known to alter climate by scattering incoming solar radiation and acting as seeds for cloud formation. These processes have vast implications for controlling the chemistry of our environment and the Earth’s climate. Sea spray aerosol (SSA) is emitted over nearly three-quarters of our planet, yet precisely how SSA impacts Earth’s radiation budget remains highly uncertain. Over the past several decades, studies have shown that SSA particles are far more complex than just sea salt. Ocean biological and physical processes produce individual SSA particles containing a diverse array of biological species including proteins, enzymes, bacteria, and viruses and a diverse array of organic compounds including fatty acids and sugars. Thus, a new frontier of research is emerging at the nexus of chemistry, biology, and atmospheric science. In this Outlook article, we discuss how current and future aerosol chemistry research demands a tight coupling between experimental (observational and laboratory studies) and computational (simulation-based) methods. This integration of approaches will enable the systematic interrogation of the complexity within individual SSA particles at a level that will enable prediction of the physicochemical properties of real-world SSA, ultimately illuminating the detailed mechanisms of how the constituents within individual SSA impact climate. American Chemical Society 2018-12-14 2018-12-26 /pmc/articles/PMC6311946/ /pubmed/30648145 http://dx.doi.org/10.1021/acscentsci.8b00674 Text en Copyright © 2018 American Chemical Society This is an open access article published under an ACS AuthorChoice License (http://pubs.acs.org/page/policy/authorchoice_termsofuse.html) , which permits copying and redistribution of the article or any adaptations for non-commercial purposes.
spellingShingle Schiffer, Jamie M.
Mael, Liora E.
Prather, Kimberly A.
Amaro, Rommie E.
Grassian, Vicki H.
Sea Spray Aerosol: Where Marine Biology Meets Atmospheric Chemistry
title Sea Spray Aerosol: Where Marine Biology Meets Atmospheric Chemistry
title_full Sea Spray Aerosol: Where Marine Biology Meets Atmospheric Chemistry
title_fullStr Sea Spray Aerosol: Where Marine Biology Meets Atmospheric Chemistry
title_full_unstemmed Sea Spray Aerosol: Where Marine Biology Meets Atmospheric Chemistry
title_short Sea Spray Aerosol: Where Marine Biology Meets Atmospheric Chemistry
title_sort sea spray aerosol: where marine biology meets atmospheric chemistry
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6311946/
https://www.ncbi.nlm.nih.gov/pubmed/30648145
http://dx.doi.org/10.1021/acscentsci.8b00674
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