Increasing the activity of copper exchanged mordenite in the direct isothermal conversion of methane to methanol by Pt and Pd doping

PtCu- and PdCu–mordenite allow for isothermal reaction at 200 °C for the stepwise methane to methanol conversion with comparably high yields. In contrast to traditional Cu-zeolites, these materials are more reactive under isothermal conditions than after high temperature activation.

Detalles Bibliográficos
Autores principales: Tomkins, P., Mansouri, A., L. Sushkevich, V., van der Wal, L. I., Bozbag, S. E., Krumeich, F., Ranocchiari, M., van Bokhoven, J. A.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Royal Society of Chemistry 2018
Materias:
Chemistry
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6330690/
https://www.ncbi.nlm.nih.gov/pubmed/30713628
http://dx.doi.org/10.1039/c8sc02795a
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author Tomkins, P.
Mansouri, A.
L. Sushkevich, V.
van der Wal, L. I.
Bozbag, S. E.
Krumeich, F.
Ranocchiari, M.
van Bokhoven, J. A.
author_facet Tomkins, P.
Mansouri, A.
L. Sushkevich, V.
van der Wal, L. I.
Bozbag, S. E.
Krumeich, F.
Ranocchiari, M.
van Bokhoven, J. A.
author_sort Tomkins, P.
collection PubMed
description PtCu- and PdCu–mordenite allow for isothermal reaction at 200 °C for the stepwise methane to methanol conversion with comparably high yields. In contrast to traditional Cu-zeolites, these materials are more reactive under isothermal conditions than after high temperature activation.
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spelling pubmed-63306902019-02-01 Increasing the activity of copper exchanged mordenite in the direct isothermal conversion of methane to methanol by Pt and Pd doping Tomkins, P. Mansouri, A. L. Sushkevich, V. van der Wal, L. I. Bozbag, S. E. Krumeich, F. Ranocchiari, M. van Bokhoven, J. A. Chem Sci Chemistry PtCu- and PdCu–mordenite allow for isothermal reaction at 200 °C for the stepwise methane to methanol conversion with comparably high yields. In contrast to traditional Cu-zeolites, these materials are more reactive under isothermal conditions than after high temperature activation. Royal Society of Chemistry 2018-10-03 /pmc/articles/PMC6330690/ /pubmed/30713628 http://dx.doi.org/10.1039/c8sc02795a Text en This journal is © The Royal Society of Chemistry 2019 http://creativecommons.org/licenses/by/3.0/ This article is freely available. This article is licensed under a Creative Commons Attribution 3.0 Unported Licence (CC BY 3.0)
spellingShingle Chemistry
Tomkins, P.
Mansouri, A.
L. Sushkevich, V.
van der Wal, L. I.
Bozbag, S. E.
Krumeich, F.
Ranocchiari, M.
van Bokhoven, J. A.
Increasing the activity of copper exchanged mordenite in the direct isothermal conversion of methane to methanol by Pt and Pd doping
title Increasing the activity of copper exchanged mordenite in the direct isothermal conversion of methane to methanol by Pt and Pd doping
title_full Increasing the activity of copper exchanged mordenite in the direct isothermal conversion of methane to methanol by Pt and Pd doping
title_fullStr Increasing the activity of copper exchanged mordenite in the direct isothermal conversion of methane to methanol by Pt and Pd doping
title_full_unstemmed Increasing the activity of copper exchanged mordenite in the direct isothermal conversion of methane to methanol by Pt and Pd doping
title_short Increasing the activity of copper exchanged mordenite in the direct isothermal conversion of methane to methanol by Pt and Pd doping
title_sort increasing the activity of copper exchanged mordenite in the direct isothermal conversion of methane to methanol by pt and pd doping
topic Chemistry
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6330690/
https://www.ncbi.nlm.nih.gov/pubmed/30713628
http://dx.doi.org/10.1039/c8sc02795a
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