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Odd electron wave packets from cycloidal ultrashort laser fields

Polarization-tailored bichromatic femtosecond laser fields with cycloidal polarization profiles have emerged as a powerful tool for coherent control of quantum processes. We present an optical scheme to create and manipulate three-dimensional free electron wave packets with arbitrary rotational symm...

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Detalles Bibliográficos
Autores principales: Kerbstadt, S., Eickhoff, K., Bayer, T., Wollenhaupt, M.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2019
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6368582/
https://www.ncbi.nlm.nih.gov/pubmed/30737394
http://dx.doi.org/10.1038/s41467-019-08601-7
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author Kerbstadt, S.
Eickhoff, K.
Bayer, T.
Wollenhaupt, M.
author_facet Kerbstadt, S.
Eickhoff, K.
Bayer, T.
Wollenhaupt, M.
author_sort Kerbstadt, S.
collection PubMed
description Polarization-tailored bichromatic femtosecond laser fields with cycloidal polarization profiles have emerged as a powerful tool for coherent control of quantum processes. We present an optical scheme to create and manipulate three-dimensional free electron wave packets with arbitrary rotational symmetry by combining advanced supercontinuum pulse shaping with high resolution photoelectron tomography. Here we use carrier-envelope phase-stable polarization-tailored bichromatic (3ω:4ω) counter- and corotating femtosecond laser pulses to generate 7-fold rotational symmetric and asymmetric photoelectron momentum distributions by multiphoton ionization of sodium atoms. To elucidate the physical mechanisms, we investigate the interplay between the symmetry properties of the driving field and the resulting electron wave packets by varying the optical field parameters. Our results show that the symmetry properties of electron wave packets are not fully determined by the field symmetry, but completely described by multipath quantum interference of states with different angular momenta.
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spelling pubmed-63685822019-02-11 Odd electron wave packets from cycloidal ultrashort laser fields Kerbstadt, S. Eickhoff, K. Bayer, T. Wollenhaupt, M. Nat Commun Article Polarization-tailored bichromatic femtosecond laser fields with cycloidal polarization profiles have emerged as a powerful tool for coherent control of quantum processes. We present an optical scheme to create and manipulate three-dimensional free electron wave packets with arbitrary rotational symmetry by combining advanced supercontinuum pulse shaping with high resolution photoelectron tomography. Here we use carrier-envelope phase-stable polarization-tailored bichromatic (3ω:4ω) counter- and corotating femtosecond laser pulses to generate 7-fold rotational symmetric and asymmetric photoelectron momentum distributions by multiphoton ionization of sodium atoms. To elucidate the physical mechanisms, we investigate the interplay between the symmetry properties of the driving field and the resulting electron wave packets by varying the optical field parameters. Our results show that the symmetry properties of electron wave packets are not fully determined by the field symmetry, but completely described by multipath quantum interference of states with different angular momenta. Nature Publishing Group UK 2019-02-08 /pmc/articles/PMC6368582/ /pubmed/30737394 http://dx.doi.org/10.1038/s41467-019-08601-7 Text en © The Author(s) 2019 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Kerbstadt, S.
Eickhoff, K.
Bayer, T.
Wollenhaupt, M.
Odd electron wave packets from cycloidal ultrashort laser fields
title Odd electron wave packets from cycloidal ultrashort laser fields
title_full Odd electron wave packets from cycloidal ultrashort laser fields
title_fullStr Odd electron wave packets from cycloidal ultrashort laser fields
title_full_unstemmed Odd electron wave packets from cycloidal ultrashort laser fields
title_short Odd electron wave packets from cycloidal ultrashort laser fields
title_sort odd electron wave packets from cycloidal ultrashort laser fields
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6368582/
https://www.ncbi.nlm.nih.gov/pubmed/30737394
http://dx.doi.org/10.1038/s41467-019-08601-7
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