Cargando…
Odd electron wave packets from cycloidal ultrashort laser fields
Polarization-tailored bichromatic femtosecond laser fields with cycloidal polarization profiles have emerged as a powerful tool for coherent control of quantum processes. We present an optical scheme to create and manipulate three-dimensional free electron wave packets with arbitrary rotational symm...
Autores principales: | , , , |
---|---|
Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group UK
2019
|
Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6368582/ https://www.ncbi.nlm.nih.gov/pubmed/30737394 http://dx.doi.org/10.1038/s41467-019-08601-7 |
_version_ | 1783394010481557504 |
---|---|
author | Kerbstadt, S. Eickhoff, K. Bayer, T. Wollenhaupt, M. |
author_facet | Kerbstadt, S. Eickhoff, K. Bayer, T. Wollenhaupt, M. |
author_sort | Kerbstadt, S. |
collection | PubMed |
description | Polarization-tailored bichromatic femtosecond laser fields with cycloidal polarization profiles have emerged as a powerful tool for coherent control of quantum processes. We present an optical scheme to create and manipulate three-dimensional free electron wave packets with arbitrary rotational symmetry by combining advanced supercontinuum pulse shaping with high resolution photoelectron tomography. Here we use carrier-envelope phase-stable polarization-tailored bichromatic (3ω:4ω) counter- and corotating femtosecond laser pulses to generate 7-fold rotational symmetric and asymmetric photoelectron momentum distributions by multiphoton ionization of sodium atoms. To elucidate the physical mechanisms, we investigate the interplay between the symmetry properties of the driving field and the resulting electron wave packets by varying the optical field parameters. Our results show that the symmetry properties of electron wave packets are not fully determined by the field symmetry, but completely described by multipath quantum interference of states with different angular momenta. |
format | Online Article Text |
id | pubmed-6368582 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2019 |
publisher | Nature Publishing Group UK |
record_format | MEDLINE/PubMed |
spelling | pubmed-63685822019-02-11 Odd electron wave packets from cycloidal ultrashort laser fields Kerbstadt, S. Eickhoff, K. Bayer, T. Wollenhaupt, M. Nat Commun Article Polarization-tailored bichromatic femtosecond laser fields with cycloidal polarization profiles have emerged as a powerful tool for coherent control of quantum processes. We present an optical scheme to create and manipulate three-dimensional free electron wave packets with arbitrary rotational symmetry by combining advanced supercontinuum pulse shaping with high resolution photoelectron tomography. Here we use carrier-envelope phase-stable polarization-tailored bichromatic (3ω:4ω) counter- and corotating femtosecond laser pulses to generate 7-fold rotational symmetric and asymmetric photoelectron momentum distributions by multiphoton ionization of sodium atoms. To elucidate the physical mechanisms, we investigate the interplay between the symmetry properties of the driving field and the resulting electron wave packets by varying the optical field parameters. Our results show that the symmetry properties of electron wave packets are not fully determined by the field symmetry, but completely described by multipath quantum interference of states with different angular momenta. Nature Publishing Group UK 2019-02-08 /pmc/articles/PMC6368582/ /pubmed/30737394 http://dx.doi.org/10.1038/s41467-019-08601-7 Text en © The Author(s) 2019 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/. |
spellingShingle | Article Kerbstadt, S. Eickhoff, K. Bayer, T. Wollenhaupt, M. Odd electron wave packets from cycloidal ultrashort laser fields |
title | Odd electron wave packets from cycloidal ultrashort laser fields |
title_full | Odd electron wave packets from cycloidal ultrashort laser fields |
title_fullStr | Odd electron wave packets from cycloidal ultrashort laser fields |
title_full_unstemmed | Odd electron wave packets from cycloidal ultrashort laser fields |
title_short | Odd electron wave packets from cycloidal ultrashort laser fields |
title_sort | odd electron wave packets from cycloidal ultrashort laser fields |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6368582/ https://www.ncbi.nlm.nih.gov/pubmed/30737394 http://dx.doi.org/10.1038/s41467-019-08601-7 |
work_keys_str_mv | AT kerbstadts oddelectronwavepacketsfromcycloidalultrashortlaserfields AT eickhoffk oddelectronwavepacketsfromcycloidalultrashortlaserfields AT bayert oddelectronwavepacketsfromcycloidalultrashortlaserfields AT wollenhauptm oddelectronwavepacketsfromcycloidalultrashortlaserfields |