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Recrystallization as the governing mechanism of ion track formation

Response of dielectric crystals: MgO, Al(2)O(3) and Y(3)Al(5)O(12) (YAG) to irradiation with 167 MeV Xe ions decelerating in the electronic stopping regime is studied. Comprehensive simulations demonstrated that despite similar ion energy losses and the initial excitation kinetics of the electronic...

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Autores principales: Rymzhanov, R. A., Medvedev, N., O’Connell, J. H., Janse van Vuuren, A., Skuratov, V. A., Volkov, A. E.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2019
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6405954/
https://www.ncbi.nlm.nih.gov/pubmed/30846734
http://dx.doi.org/10.1038/s41598-019-40239-9
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author Rymzhanov, R. A.
Medvedev, N.
O’Connell, J. H.
Janse van Vuuren, A.
Skuratov, V. A.
Volkov, A. E.
author_facet Rymzhanov, R. A.
Medvedev, N.
O’Connell, J. H.
Janse van Vuuren, A.
Skuratov, V. A.
Volkov, A. E.
author_sort Rymzhanov, R. A.
collection PubMed
description Response of dielectric crystals: MgO, Al(2)O(3) and Y(3)Al(5)O(12) (YAG) to irradiation with 167 MeV Xe ions decelerating in the electronic stopping regime is studied. Comprehensive simulations demonstrated that despite similar ion energy losses and the initial excitation kinetics of the electronic systems and lattices, significant differences occur among final structures of ion tracks in these materials, supported by experiments. No ion tracks appeared in MgO, whereas discontinuous distorted crystalline tracks of ~2 nm in diameter were observed in Al(2)O(3) and continuous amorphous tracks were detected in YAG. These track structures in Al(2)O(3) and YAG were confirmed by high resolution TEM data. The simulations enabled us to identify recrystallization as the dominant mechanism governing formation of detected tracks in these oxides. We analyzed effects of the viscosity in molten state, lattice structure and difference in the kinetics of metallic and oxygen sublattices at the crystallization surface on damage recovery in tracks.
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spelling pubmed-64059542019-03-12 Recrystallization as the governing mechanism of ion track formation Rymzhanov, R. A. Medvedev, N. O’Connell, J. H. Janse van Vuuren, A. Skuratov, V. A. Volkov, A. E. Sci Rep Article Response of dielectric crystals: MgO, Al(2)O(3) and Y(3)Al(5)O(12) (YAG) to irradiation with 167 MeV Xe ions decelerating in the electronic stopping regime is studied. Comprehensive simulations demonstrated that despite similar ion energy losses and the initial excitation kinetics of the electronic systems and lattices, significant differences occur among final structures of ion tracks in these materials, supported by experiments. No ion tracks appeared in MgO, whereas discontinuous distorted crystalline tracks of ~2 nm in diameter were observed in Al(2)O(3) and continuous amorphous tracks were detected in YAG. These track structures in Al(2)O(3) and YAG were confirmed by high resolution TEM data. The simulations enabled us to identify recrystallization as the dominant mechanism governing formation of detected tracks in these oxides. We analyzed effects of the viscosity in molten state, lattice structure and difference in the kinetics of metallic and oxygen sublattices at the crystallization surface on damage recovery in tracks. Nature Publishing Group UK 2019-03-07 /pmc/articles/PMC6405954/ /pubmed/30846734 http://dx.doi.org/10.1038/s41598-019-40239-9 Text en © The Author(s) 2019 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Rymzhanov, R. A.
Medvedev, N.
O’Connell, J. H.
Janse van Vuuren, A.
Skuratov, V. A.
Volkov, A. E.
Recrystallization as the governing mechanism of ion track formation
title Recrystallization as the governing mechanism of ion track formation
title_full Recrystallization as the governing mechanism of ion track formation
title_fullStr Recrystallization as the governing mechanism of ion track formation
title_full_unstemmed Recrystallization as the governing mechanism of ion track formation
title_short Recrystallization as the governing mechanism of ion track formation
title_sort recrystallization as the governing mechanism of ion track formation
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6405954/
https://www.ncbi.nlm.nih.gov/pubmed/30846734
http://dx.doi.org/10.1038/s41598-019-40239-9
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