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Recrystallization as the governing mechanism of ion track formation
Response of dielectric crystals: MgO, Al(2)O(3) and Y(3)Al(5)O(12) (YAG) to irradiation with 167 MeV Xe ions decelerating in the electronic stopping regime is studied. Comprehensive simulations demonstrated that despite similar ion energy losses and the initial excitation kinetics of the electronic...
Autores principales: | , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group UK
2019
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6405954/ https://www.ncbi.nlm.nih.gov/pubmed/30846734 http://dx.doi.org/10.1038/s41598-019-40239-9 |
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author | Rymzhanov, R. A. Medvedev, N. O’Connell, J. H. Janse van Vuuren, A. Skuratov, V. A. Volkov, A. E. |
author_facet | Rymzhanov, R. A. Medvedev, N. O’Connell, J. H. Janse van Vuuren, A. Skuratov, V. A. Volkov, A. E. |
author_sort | Rymzhanov, R. A. |
collection | PubMed |
description | Response of dielectric crystals: MgO, Al(2)O(3) and Y(3)Al(5)O(12) (YAG) to irradiation with 167 MeV Xe ions decelerating in the electronic stopping regime is studied. Comprehensive simulations demonstrated that despite similar ion energy losses and the initial excitation kinetics of the electronic systems and lattices, significant differences occur among final structures of ion tracks in these materials, supported by experiments. No ion tracks appeared in MgO, whereas discontinuous distorted crystalline tracks of ~2 nm in diameter were observed in Al(2)O(3) and continuous amorphous tracks were detected in YAG. These track structures in Al(2)O(3) and YAG were confirmed by high resolution TEM data. The simulations enabled us to identify recrystallization as the dominant mechanism governing formation of detected tracks in these oxides. We analyzed effects of the viscosity in molten state, lattice structure and difference in the kinetics of metallic and oxygen sublattices at the crystallization surface on damage recovery in tracks. |
format | Online Article Text |
id | pubmed-6405954 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2019 |
publisher | Nature Publishing Group UK |
record_format | MEDLINE/PubMed |
spelling | pubmed-64059542019-03-12 Recrystallization as the governing mechanism of ion track formation Rymzhanov, R. A. Medvedev, N. O’Connell, J. H. Janse van Vuuren, A. Skuratov, V. A. Volkov, A. E. Sci Rep Article Response of dielectric crystals: MgO, Al(2)O(3) and Y(3)Al(5)O(12) (YAG) to irradiation with 167 MeV Xe ions decelerating in the electronic stopping regime is studied. Comprehensive simulations demonstrated that despite similar ion energy losses and the initial excitation kinetics of the electronic systems and lattices, significant differences occur among final structures of ion tracks in these materials, supported by experiments. No ion tracks appeared in MgO, whereas discontinuous distorted crystalline tracks of ~2 nm in diameter were observed in Al(2)O(3) and continuous amorphous tracks were detected in YAG. These track structures in Al(2)O(3) and YAG were confirmed by high resolution TEM data. The simulations enabled us to identify recrystallization as the dominant mechanism governing formation of detected tracks in these oxides. We analyzed effects of the viscosity in molten state, lattice structure and difference in the kinetics of metallic and oxygen sublattices at the crystallization surface on damage recovery in tracks. Nature Publishing Group UK 2019-03-07 /pmc/articles/PMC6405954/ /pubmed/30846734 http://dx.doi.org/10.1038/s41598-019-40239-9 Text en © The Author(s) 2019 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/. |
spellingShingle | Article Rymzhanov, R. A. Medvedev, N. O’Connell, J. H. Janse van Vuuren, A. Skuratov, V. A. Volkov, A. E. Recrystallization as the governing mechanism of ion track formation |
title | Recrystallization as the governing mechanism of ion track formation |
title_full | Recrystallization as the governing mechanism of ion track formation |
title_fullStr | Recrystallization as the governing mechanism of ion track formation |
title_full_unstemmed | Recrystallization as the governing mechanism of ion track formation |
title_short | Recrystallization as the governing mechanism of ion track formation |
title_sort | recrystallization as the governing mechanism of ion track formation |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6405954/ https://www.ncbi.nlm.nih.gov/pubmed/30846734 http://dx.doi.org/10.1038/s41598-019-40239-9 |
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