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An engineered GH1 β-glucosidase displays enhanced glucose tolerance and increased sugar release from lignocellulosic materials

β-glucosidases play a critical role among the enzymes in enzymatic cocktails designed for plant biomass deconstruction. By catalysing the breakdown of β-1, 4-glycosidic linkages, β-glucosidases produce free fermentable glucose and alleviate the inhibition of other cellulases by cellobiose during sac...

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Autores principales: Santos, Clelton A., Morais, Mariana A. B., Terrett, Oliver M., Lyczakowski, Jan J., Zanphorlin, Letícia M., Ferreira-Filho, Jaire A., Tonoli, Celisa C. C., Murakami, Mario T., Dupree, Paul, Souza, Anete P.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2019
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6426972/
https://www.ncbi.nlm.nih.gov/pubmed/30894609
http://dx.doi.org/10.1038/s41598-019-41300-3
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author Santos, Clelton A.
Morais, Mariana A. B.
Terrett, Oliver M.
Lyczakowski, Jan J.
Zanphorlin, Letícia M.
Ferreira-Filho, Jaire A.
Tonoli, Celisa C. C.
Murakami, Mario T.
Dupree, Paul
Souza, Anete P.
author_facet Santos, Clelton A.
Morais, Mariana A. B.
Terrett, Oliver M.
Lyczakowski, Jan J.
Zanphorlin, Letícia M.
Ferreira-Filho, Jaire A.
Tonoli, Celisa C. C.
Murakami, Mario T.
Dupree, Paul
Souza, Anete P.
author_sort Santos, Clelton A.
collection PubMed
description β-glucosidases play a critical role among the enzymes in enzymatic cocktails designed for plant biomass deconstruction. By catalysing the breakdown of β-1, 4-glycosidic linkages, β-glucosidases produce free fermentable glucose and alleviate the inhibition of other cellulases by cellobiose during saccharification. Despite this benefit, most characterised fungal β-glucosidases show weak activity at high glucose concentrations, limiting enzymatic hydrolysis of plant biomass in industrial settings. In this study, structural analyses combined with site-directed mutagenesis efficiently improved the functional properties of a GH1 β-glucosidase highly expressed by Trichoderma harzianum (ThBgl) under biomass degradation conditions. The tailored enzyme displayed high glucose tolerance levels, confirming that glucose tolerance can be achieved by the substitution of two amino acids that act as gatekeepers, changing active-site accessibility and preventing product inhibition. Furthermore, the enhanced efficiency of the engineered enzyme in terms of the amount of glucose released and ethanol yield was confirmed by saccharification and simultaneous saccharification and fermentation experiments using a wide range of plant biomass feedstocks. Our results not only experimentally confirm the structural basis of glucose tolerance in GH1 β-glucosidases but also demonstrate a strategy to improve technologies for bioethanol production based on enzymatic hydrolysis.
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spelling pubmed-64269722019-03-28 An engineered GH1 β-glucosidase displays enhanced glucose tolerance and increased sugar release from lignocellulosic materials Santos, Clelton A. Morais, Mariana A. B. Terrett, Oliver M. Lyczakowski, Jan J. Zanphorlin, Letícia M. Ferreira-Filho, Jaire A. Tonoli, Celisa C. C. Murakami, Mario T. Dupree, Paul Souza, Anete P. Sci Rep Article β-glucosidases play a critical role among the enzymes in enzymatic cocktails designed for plant biomass deconstruction. By catalysing the breakdown of β-1, 4-glycosidic linkages, β-glucosidases produce free fermentable glucose and alleviate the inhibition of other cellulases by cellobiose during saccharification. Despite this benefit, most characterised fungal β-glucosidases show weak activity at high glucose concentrations, limiting enzymatic hydrolysis of plant biomass in industrial settings. In this study, structural analyses combined with site-directed mutagenesis efficiently improved the functional properties of a GH1 β-glucosidase highly expressed by Trichoderma harzianum (ThBgl) under biomass degradation conditions. The tailored enzyme displayed high glucose tolerance levels, confirming that glucose tolerance can be achieved by the substitution of two amino acids that act as gatekeepers, changing active-site accessibility and preventing product inhibition. Furthermore, the enhanced efficiency of the engineered enzyme in terms of the amount of glucose released and ethanol yield was confirmed by saccharification and simultaneous saccharification and fermentation experiments using a wide range of plant biomass feedstocks. Our results not only experimentally confirm the structural basis of glucose tolerance in GH1 β-glucosidases but also demonstrate a strategy to improve technologies for bioethanol production based on enzymatic hydrolysis. Nature Publishing Group UK 2019-03-20 /pmc/articles/PMC6426972/ /pubmed/30894609 http://dx.doi.org/10.1038/s41598-019-41300-3 Text en © The Author(s) 2019 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Santos, Clelton A.
Morais, Mariana A. B.
Terrett, Oliver M.
Lyczakowski, Jan J.
Zanphorlin, Letícia M.
Ferreira-Filho, Jaire A.
Tonoli, Celisa C. C.
Murakami, Mario T.
Dupree, Paul
Souza, Anete P.
An engineered GH1 β-glucosidase displays enhanced glucose tolerance and increased sugar release from lignocellulosic materials
title An engineered GH1 β-glucosidase displays enhanced glucose tolerance and increased sugar release from lignocellulosic materials
title_full An engineered GH1 β-glucosidase displays enhanced glucose tolerance and increased sugar release from lignocellulosic materials
title_fullStr An engineered GH1 β-glucosidase displays enhanced glucose tolerance and increased sugar release from lignocellulosic materials
title_full_unstemmed An engineered GH1 β-glucosidase displays enhanced glucose tolerance and increased sugar release from lignocellulosic materials
title_short An engineered GH1 β-glucosidase displays enhanced glucose tolerance and increased sugar release from lignocellulosic materials
title_sort engineered gh1 β-glucosidase displays enhanced glucose tolerance and increased sugar release from lignocellulosic materials
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6426972/
https://www.ncbi.nlm.nih.gov/pubmed/30894609
http://dx.doi.org/10.1038/s41598-019-41300-3
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