Pore-tuning to boost the electrocatalytic activity of polymeric micelle-templated mesoporous Pd nanoparticles

Understanding how mesoporous noble metal architectures affect electrocatalytic performance is very important for the rational design and preparation of high-performance electrocatalysts. Herein, by using polymeric micelle-assembled structures as templates, mesoporous Pd nanoparticles with tunable po...

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Autores principales: Li, Cuiling, Iqbal, Muhammad, Jiang, Bo, Wang, Zhongli, Kim, Jeonghun, Nanjundan, Ashok Kumar, Whitten, Andrew E., Wood, Kathleen, Yamauchi, Yusuke
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Royal Society of Chemistry 2019
Materias:
Chemistry
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6457336/
https://www.ncbi.nlm.nih.gov/pubmed/31015946
http://dx.doi.org/10.1039/c8sc03911a
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author Li, Cuiling
Iqbal, Muhammad
Jiang, Bo
Wang, Zhongli
Kim, Jeonghun
Nanjundan, Ashok Kumar
Whitten, Andrew E.
Wood, Kathleen
Yamauchi, Yusuke
author_facet Li, Cuiling
Iqbal, Muhammad
Jiang, Bo
Wang, Zhongli
Kim, Jeonghun
Nanjundan, Ashok Kumar
Whitten, Andrew E.
Wood, Kathleen
Yamauchi, Yusuke
author_sort Li, Cuiling
collection PubMed
description Understanding how mesoporous noble metal architectures affect electrocatalytic performance is very important for the rational design and preparation of high-performance electrocatalysts. Herein, by using polymeric micelle-assembled structures as templates, mesoporous Pd nanoparticles with tunable porous constructions are synthesized by simply tuning the solvent compositions. The effect of porous Pd nanoparticles on the electrocatalytic performance is thoroughly studied. Their superior electrocatalytic activity can be attributed to the mass transport efficiency and open porous structures.
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spelling pubmed-64573362019-04-23 Pore-tuning to boost the electrocatalytic activity of polymeric micelle-templated mesoporous Pd nanoparticles Li, Cuiling Iqbal, Muhammad Jiang, Bo Wang, Zhongli Kim, Jeonghun Nanjundan, Ashok Kumar Whitten, Andrew E. Wood, Kathleen Yamauchi, Yusuke Chem Sci Chemistry Understanding how mesoporous noble metal architectures affect electrocatalytic performance is very important for the rational design and preparation of high-performance electrocatalysts. Herein, by using polymeric micelle-assembled structures as templates, mesoporous Pd nanoparticles with tunable porous constructions are synthesized by simply tuning the solvent compositions. The effect of porous Pd nanoparticles on the electrocatalytic performance is thoroughly studied. Their superior electrocatalytic activity can be attributed to the mass transport efficiency and open porous structures. Royal Society of Chemistry 2019-03-12 /pmc/articles/PMC6457336/ /pubmed/31015946 http://dx.doi.org/10.1039/c8sc03911a Text en This journal is © The Royal Society of Chemistry 2019 http://creativecommons.org/licenses/by/3.0/ This article is freely available. This article is licensed under a Creative Commons Attribution 3.0 Unported Licence (CC BY 3.0)
spellingShingle Chemistry
Li, Cuiling
Iqbal, Muhammad
Jiang, Bo
Wang, Zhongli
Kim, Jeonghun
Nanjundan, Ashok Kumar
Whitten, Andrew E.
Wood, Kathleen
Yamauchi, Yusuke
Pore-tuning to boost the electrocatalytic activity of polymeric micelle-templated mesoporous Pd nanoparticles
title Pore-tuning to boost the electrocatalytic activity of polymeric micelle-templated mesoporous Pd nanoparticles
title_full Pore-tuning to boost the electrocatalytic activity of polymeric micelle-templated mesoporous Pd nanoparticles
title_fullStr Pore-tuning to boost the electrocatalytic activity of polymeric micelle-templated mesoporous Pd nanoparticles
title_full_unstemmed Pore-tuning to boost the electrocatalytic activity of polymeric micelle-templated mesoporous Pd nanoparticles
title_short Pore-tuning to boost the electrocatalytic activity of polymeric micelle-templated mesoporous Pd nanoparticles
title_sort pore-tuning to boost the electrocatalytic activity of polymeric micelle-templated mesoporous pd nanoparticles
topic Chemistry
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6457336/
https://www.ncbi.nlm.nih.gov/pubmed/31015946
http://dx.doi.org/10.1039/c8sc03911a
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