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3D strain-induced superconductivity in La(2)CuO(4+δ) using a simple vertically aligned nanocomposite approach

A long-term goal for superconductors is to increase the superconducting transition temperature, T(C). In cuprates, T(C) depends strongly on the out-of-plane Cu-apical oxygen distance and the in-plane Cu-O distance, but there has been little attention paid to tuning them independently. Here, in simpl...

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Autores principales: Choi, Eun-Mi, Di Bernardo, Angelo, Zhu, Bonan, Lu, Ping, Alpern, Hen, Zhang, Kelvin H. L., Shapira, Tamar, Feighan, John, Sun, Xing, Robinson, Jason, Paltiel, Yossi, Millo, Oded, Wang, Haiyan, Jia, Quanxi, MacManus-Driscoll, Judith L.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Association for the Advancement of Science 2019
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6486216/
https://www.ncbi.nlm.nih.gov/pubmed/31032414
http://dx.doi.org/10.1126/sciadv.aav5532
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author Choi, Eun-Mi
Di Bernardo, Angelo
Zhu, Bonan
Lu, Ping
Alpern, Hen
Zhang, Kelvin H. L.
Shapira, Tamar
Feighan, John
Sun, Xing
Robinson, Jason
Paltiel, Yossi
Millo, Oded
Wang, Haiyan
Jia, Quanxi
MacManus-Driscoll, Judith L.
author_facet Choi, Eun-Mi
Di Bernardo, Angelo
Zhu, Bonan
Lu, Ping
Alpern, Hen
Zhang, Kelvin H. L.
Shapira, Tamar
Feighan, John
Sun, Xing
Robinson, Jason
Paltiel, Yossi
Millo, Oded
Wang, Haiyan
Jia, Quanxi
MacManus-Driscoll, Judith L.
author_sort Choi, Eun-Mi
collection PubMed
description A long-term goal for superconductors is to increase the superconducting transition temperature, T(C). In cuprates, T(C) depends strongly on the out-of-plane Cu-apical oxygen distance and the in-plane Cu-O distance, but there has been little attention paid to tuning them independently. Here, in simply grown, self-assembled, vertically aligned nanocomposite thin films of La(2)CuO(4+δ) + LaCuO(3), by strongly increasing out-of-plane distances without reducing in-plane distances (three-dimensional strain engineering), we achieve superconductivity up to 50 K in the vertical interface regions, spaced ~50 nm apart. No additional process to supply excess oxygen, e.g., by ozone or high-pressure oxygen annealing, was required, as is normally the case for plain La(2)CuO(4+δ) films. Our proof-of-concept work represents an entirely new approach to increasing T(C) in cuprates or other superconductors.
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spelling pubmed-64862162019-04-27 3D strain-induced superconductivity in La(2)CuO(4+δ) using a simple vertically aligned nanocomposite approach Choi, Eun-Mi Di Bernardo, Angelo Zhu, Bonan Lu, Ping Alpern, Hen Zhang, Kelvin H. L. Shapira, Tamar Feighan, John Sun, Xing Robinson, Jason Paltiel, Yossi Millo, Oded Wang, Haiyan Jia, Quanxi MacManus-Driscoll, Judith L. Sci Adv Research Articles A long-term goal for superconductors is to increase the superconducting transition temperature, T(C). In cuprates, T(C) depends strongly on the out-of-plane Cu-apical oxygen distance and the in-plane Cu-O distance, but there has been little attention paid to tuning them independently. Here, in simply grown, self-assembled, vertically aligned nanocomposite thin films of La(2)CuO(4+δ) + LaCuO(3), by strongly increasing out-of-plane distances without reducing in-plane distances (three-dimensional strain engineering), we achieve superconductivity up to 50 K in the vertical interface regions, spaced ~50 nm apart. No additional process to supply excess oxygen, e.g., by ozone or high-pressure oxygen annealing, was required, as is normally the case for plain La(2)CuO(4+δ) films. Our proof-of-concept work represents an entirely new approach to increasing T(C) in cuprates or other superconductors. American Association for the Advancement of Science 2019-04-26 /pmc/articles/PMC6486216/ /pubmed/31032414 http://dx.doi.org/10.1126/sciadv.aav5532 Text en Copyright © 2019 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution License 4.0 (CC BY). http://creativecommons.org/licenses/by/4.0/ This is an open-access article distributed under the terms of the Creative Commons Attribution license (http://creativecommons.org/licenses/by/4.0/) , which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited.
spellingShingle Research Articles
Choi, Eun-Mi
Di Bernardo, Angelo
Zhu, Bonan
Lu, Ping
Alpern, Hen
Zhang, Kelvin H. L.
Shapira, Tamar
Feighan, John
Sun, Xing
Robinson, Jason
Paltiel, Yossi
Millo, Oded
Wang, Haiyan
Jia, Quanxi
MacManus-Driscoll, Judith L.
3D strain-induced superconductivity in La(2)CuO(4+δ) using a simple vertically aligned nanocomposite approach
title 3D strain-induced superconductivity in La(2)CuO(4+δ) using a simple vertically aligned nanocomposite approach
title_full 3D strain-induced superconductivity in La(2)CuO(4+δ) using a simple vertically aligned nanocomposite approach
title_fullStr 3D strain-induced superconductivity in La(2)CuO(4+δ) using a simple vertically aligned nanocomposite approach
title_full_unstemmed 3D strain-induced superconductivity in La(2)CuO(4+δ) using a simple vertically aligned nanocomposite approach
title_short 3D strain-induced superconductivity in La(2)CuO(4+δ) using a simple vertically aligned nanocomposite approach
title_sort 3d strain-induced superconductivity in la(2)cuo(4+δ) using a simple vertically aligned nanocomposite approach
topic Research Articles
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6486216/
https://www.ncbi.nlm.nih.gov/pubmed/31032414
http://dx.doi.org/10.1126/sciadv.aav5532
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