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Tamm Plasmons Directionally Enhance Rare-Earth Nanophosphor Emission

[Image: see text] Rare-earth-based phosphors are the materials on which current solid-state lighting technology is built. However, their large crystal size impedes the tuning, optimization, or manipulation of emitted light that can be achieved by their integration in nanophotonic architectures. Here...

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Autores principales: Geng, Dongling, Cabello-Olmo, Elena, Lozano, Gabriel, Míguez, Hernán
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2019
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6488127/
https://www.ncbi.nlm.nih.gov/pubmed/31049366
http://dx.doi.org/10.1021/acsphotonics.8b01407
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author Geng, Dongling
Cabello-Olmo, Elena
Lozano, Gabriel
Míguez, Hernán
author_facet Geng, Dongling
Cabello-Olmo, Elena
Lozano, Gabriel
Míguez, Hernán
author_sort Geng, Dongling
collection PubMed
description [Image: see text] Rare-earth-based phosphors are the materials on which current solid-state lighting technology is built. However, their large crystal size impedes the tuning, optimization, or manipulation of emitted light that can be achieved by their integration in nanophotonic architectures. Herein we demonstrate a hybrid plasmonic–photonic architecture capable of both channeling in a specific direction and enhancing by eight times the emission radiated by a macroscopically wide layer of nanophosphors. In order to do so, a slab of rare-earth-based nanocrystals is inserted between a dielectric multilayer and a metal film, following a rational design that optimizes the coupling of nanophosphor emission to collective modes sustained by the metal–dielectric system. Our approach is advantageous for the optimization of solid-state lighting systems.
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spelling pubmed-64881272019-04-30 Tamm Plasmons Directionally Enhance Rare-Earth Nanophosphor Emission Geng, Dongling Cabello-Olmo, Elena Lozano, Gabriel Míguez, Hernán ACS Photonics [Image: see text] Rare-earth-based phosphors are the materials on which current solid-state lighting technology is built. However, their large crystal size impedes the tuning, optimization, or manipulation of emitted light that can be achieved by their integration in nanophotonic architectures. Herein we demonstrate a hybrid plasmonic–photonic architecture capable of both channeling in a specific direction and enhancing by eight times the emission radiated by a macroscopically wide layer of nanophosphors. In order to do so, a slab of rare-earth-based nanocrystals is inserted between a dielectric multilayer and a metal film, following a rational design that optimizes the coupling of nanophosphor emission to collective modes sustained by the metal–dielectric system. Our approach is advantageous for the optimization of solid-state lighting systems. American Chemical Society 2019-02-14 2019-03-20 /pmc/articles/PMC6488127/ /pubmed/31049366 http://dx.doi.org/10.1021/acsphotonics.8b01407 Text en Copyright © 2019 American Chemical Society This is an open access article published under an ACS AuthorChoice License (http://pubs.acs.org/page/policy/authorchoice_termsofuse.html) , which permits copying and redistribution of the article or any adaptations for non-commercial purposes.
spellingShingle Geng, Dongling
Cabello-Olmo, Elena
Lozano, Gabriel
Míguez, Hernán
Tamm Plasmons Directionally Enhance Rare-Earth Nanophosphor Emission
title Tamm Plasmons Directionally Enhance Rare-Earth Nanophosphor Emission
title_full Tamm Plasmons Directionally Enhance Rare-Earth Nanophosphor Emission
title_fullStr Tamm Plasmons Directionally Enhance Rare-Earth Nanophosphor Emission
title_full_unstemmed Tamm Plasmons Directionally Enhance Rare-Earth Nanophosphor Emission
title_short Tamm Plasmons Directionally Enhance Rare-Earth Nanophosphor Emission
title_sort tamm plasmons directionally enhance rare-earth nanophosphor emission
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6488127/
https://www.ncbi.nlm.nih.gov/pubmed/31049366
http://dx.doi.org/10.1021/acsphotonics.8b01407
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