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Tamm Plasmons Directionally Enhance Rare-Earth Nanophosphor Emission
[Image: see text] Rare-earth-based phosphors are the materials on which current solid-state lighting technology is built. However, their large crystal size impedes the tuning, optimization, or manipulation of emitted light that can be achieved by their integration in nanophotonic architectures. Here...
Autores principales: | , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American Chemical Society
2019
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Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6488127/ https://www.ncbi.nlm.nih.gov/pubmed/31049366 http://dx.doi.org/10.1021/acsphotonics.8b01407 |
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author | Geng, Dongling Cabello-Olmo, Elena Lozano, Gabriel Míguez, Hernán |
author_facet | Geng, Dongling Cabello-Olmo, Elena Lozano, Gabriel Míguez, Hernán |
author_sort | Geng, Dongling |
collection | PubMed |
description | [Image: see text] Rare-earth-based phosphors are the materials on which current solid-state lighting technology is built. However, their large crystal size impedes the tuning, optimization, or manipulation of emitted light that can be achieved by their integration in nanophotonic architectures. Herein we demonstrate a hybrid plasmonic–photonic architecture capable of both channeling in a specific direction and enhancing by eight times the emission radiated by a macroscopically wide layer of nanophosphors. In order to do so, a slab of rare-earth-based nanocrystals is inserted between a dielectric multilayer and a metal film, following a rational design that optimizes the coupling of nanophosphor emission to collective modes sustained by the metal–dielectric system. Our approach is advantageous for the optimization of solid-state lighting systems. |
format | Online Article Text |
id | pubmed-6488127 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2019 |
publisher | American Chemical Society |
record_format | MEDLINE/PubMed |
spelling | pubmed-64881272019-04-30 Tamm Plasmons Directionally Enhance Rare-Earth Nanophosphor Emission Geng, Dongling Cabello-Olmo, Elena Lozano, Gabriel Míguez, Hernán ACS Photonics [Image: see text] Rare-earth-based phosphors are the materials on which current solid-state lighting technology is built. However, their large crystal size impedes the tuning, optimization, or manipulation of emitted light that can be achieved by their integration in nanophotonic architectures. Herein we demonstrate a hybrid plasmonic–photonic architecture capable of both channeling in a specific direction and enhancing by eight times the emission radiated by a macroscopically wide layer of nanophosphors. In order to do so, a slab of rare-earth-based nanocrystals is inserted between a dielectric multilayer and a metal film, following a rational design that optimizes the coupling of nanophosphor emission to collective modes sustained by the metal–dielectric system. Our approach is advantageous for the optimization of solid-state lighting systems. American Chemical Society 2019-02-14 2019-03-20 /pmc/articles/PMC6488127/ /pubmed/31049366 http://dx.doi.org/10.1021/acsphotonics.8b01407 Text en Copyright © 2019 American Chemical Society This is an open access article published under an ACS AuthorChoice License (http://pubs.acs.org/page/policy/authorchoice_termsofuse.html) , which permits copying and redistribution of the article or any adaptations for non-commercial purposes. |
spellingShingle | Geng, Dongling Cabello-Olmo, Elena Lozano, Gabriel Míguez, Hernán Tamm Plasmons Directionally Enhance Rare-Earth Nanophosphor Emission |
title | Tamm Plasmons Directionally Enhance Rare-Earth Nanophosphor
Emission |
title_full | Tamm Plasmons Directionally Enhance Rare-Earth Nanophosphor
Emission |
title_fullStr | Tamm Plasmons Directionally Enhance Rare-Earth Nanophosphor
Emission |
title_full_unstemmed | Tamm Plasmons Directionally Enhance Rare-Earth Nanophosphor
Emission |
title_short | Tamm Plasmons Directionally Enhance Rare-Earth Nanophosphor
Emission |
title_sort | tamm plasmons directionally enhance rare-earth nanophosphor
emission |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6488127/ https://www.ncbi.nlm.nih.gov/pubmed/31049366 http://dx.doi.org/10.1021/acsphotonics.8b01407 |
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