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High sensitivity variable-temperature infrared nanoscopy of conducting oxide interfaces

Probing the local transport properties of two-dimensional electron systems (2DES) confined at buried interfaces requires a non-invasive technique with a high spatial resolution operating in a broad temperature range. In this paper, we investigate the scattering-type scanning near field optical micro...

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Autores principales: Luo, Weiwei, Boselli, Margherita, Poumirol, Jean-Marie, Ardizzone, Ivan, Teyssier, Jérémie, van der Marel, Dirk, Gariglio, Stefano, Triscone, Jean-Marc, Kuzmenko, Alexey B.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2019
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6591405/
https://www.ncbi.nlm.nih.gov/pubmed/31235858
http://dx.doi.org/10.1038/s41467-019-10672-5
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author Luo, Weiwei
Boselli, Margherita
Poumirol, Jean-Marie
Ardizzone, Ivan
Teyssier, Jérémie
van der Marel, Dirk
Gariglio, Stefano
Triscone, Jean-Marc
Kuzmenko, Alexey B.
author_facet Luo, Weiwei
Boselli, Margherita
Poumirol, Jean-Marie
Ardizzone, Ivan
Teyssier, Jérémie
van der Marel, Dirk
Gariglio, Stefano
Triscone, Jean-Marc
Kuzmenko, Alexey B.
author_sort Luo, Weiwei
collection PubMed
description Probing the local transport properties of two-dimensional electron systems (2DES) confined at buried interfaces requires a non-invasive technique with a high spatial resolution operating in a broad temperature range. In this paper, we investigate the scattering-type scanning near field optical microscopy as a tool for studying the conducting LaAlO(3)/SrTiO(3) interface from room temperature down to 6 K. We show that the near-field optical signal, in particular its phase component, is highly sensitive to the transport properties of the electron system present at the interface. Our modeling reveals that such sensitivity originates from the interaction of the AFM tip with coupled plasmon–phonon modes with a small penetration depth. The model allows us to quantitatively correlate changes in the optical signal with the variation of the 2DES transport properties induced by cooling and by electrostatic gating. To probe the spatial resolution of the technique, we image conducting nano-channels written in insulating heterostructures with a voltage-biased tip of an atomic force microscope.
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spelling pubmed-65914052019-06-26 High sensitivity variable-temperature infrared nanoscopy of conducting oxide interfaces Luo, Weiwei Boselli, Margherita Poumirol, Jean-Marie Ardizzone, Ivan Teyssier, Jérémie van der Marel, Dirk Gariglio, Stefano Triscone, Jean-Marc Kuzmenko, Alexey B. Nat Commun Article Probing the local transport properties of two-dimensional electron systems (2DES) confined at buried interfaces requires a non-invasive technique with a high spatial resolution operating in a broad temperature range. In this paper, we investigate the scattering-type scanning near field optical microscopy as a tool for studying the conducting LaAlO(3)/SrTiO(3) interface from room temperature down to 6 K. We show that the near-field optical signal, in particular its phase component, is highly sensitive to the transport properties of the electron system present at the interface. Our modeling reveals that such sensitivity originates from the interaction of the AFM tip with coupled plasmon–phonon modes with a small penetration depth. The model allows us to quantitatively correlate changes in the optical signal with the variation of the 2DES transport properties induced by cooling and by electrostatic gating. To probe the spatial resolution of the technique, we image conducting nano-channels written in insulating heterostructures with a voltage-biased tip of an atomic force microscope. Nature Publishing Group UK 2019-06-24 /pmc/articles/PMC6591405/ /pubmed/31235858 http://dx.doi.org/10.1038/s41467-019-10672-5 Text en © The Author(s) 2019 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Luo, Weiwei
Boselli, Margherita
Poumirol, Jean-Marie
Ardizzone, Ivan
Teyssier, Jérémie
van der Marel, Dirk
Gariglio, Stefano
Triscone, Jean-Marc
Kuzmenko, Alexey B.
High sensitivity variable-temperature infrared nanoscopy of conducting oxide interfaces
title High sensitivity variable-temperature infrared nanoscopy of conducting oxide interfaces
title_full High sensitivity variable-temperature infrared nanoscopy of conducting oxide interfaces
title_fullStr High sensitivity variable-temperature infrared nanoscopy of conducting oxide interfaces
title_full_unstemmed High sensitivity variable-temperature infrared nanoscopy of conducting oxide interfaces
title_short High sensitivity variable-temperature infrared nanoscopy of conducting oxide interfaces
title_sort high sensitivity variable-temperature infrared nanoscopy of conducting oxide interfaces
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6591405/
https://www.ncbi.nlm.nih.gov/pubmed/31235858
http://dx.doi.org/10.1038/s41467-019-10672-5
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