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Revising of the Purcell effect in periodic metal-dielectric structures: the role of absorption
Periodic metal-dielectric structures attract substantial interest since it was previously proposed that the spontaneous emission amplification rates (the Purcell factor) in such structures can reach enormous values up to 10(5). However, the role of absorption in real metals has not been thoroughly c...
Autores principales: | , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group UK
2019
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6610144/ https://www.ncbi.nlm.nih.gov/pubmed/31270385 http://dx.doi.org/10.1038/s41598-019-46071-5 |
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author | Morozov, Konstantin M. Ivanov, Konstantin A. de Sa Pereira, Daniel Menelaou, Christopher Monkman, Andrew P. Pozina, Galia Kaliteevski, Mikhail A. |
author_facet | Morozov, Konstantin M. Ivanov, Konstantin A. de Sa Pereira, Daniel Menelaou, Christopher Monkman, Andrew P. Pozina, Galia Kaliteevski, Mikhail A. |
author_sort | Morozov, Konstantin M. |
collection | PubMed |
description | Periodic metal-dielectric structures attract substantial interest since it was previously proposed that the spontaneous emission amplification rates (the Purcell factor) in such structures can reach enormous values up to 10(5). However, the role of absorption in real metals has not been thoroughly considered. We provide a theoretical analysis showing that absorption leads to diminishing values of Purcell factor. We also suggest that using emitting organic compounds such as CBP (4,4-Bis(N-carbazolyl)-1,1-biphenyl) can lead to a moderate increase of about an order of magnitude in the Purcell factor. Defining the experimentally measured Purcell factor as a ratio between the excited state lifetimes in bare CBP and in periodic structure, this increase in the fabricated periodic structure is demonstrated through a 4–8 times decrease in excited state radiative lifetime compared to a bare organic material in a wide emission spectrum. |
format | Online Article Text |
id | pubmed-6610144 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2019 |
publisher | Nature Publishing Group UK |
record_format | MEDLINE/PubMed |
spelling | pubmed-66101442019-07-14 Revising of the Purcell effect in periodic metal-dielectric structures: the role of absorption Morozov, Konstantin M. Ivanov, Konstantin A. de Sa Pereira, Daniel Menelaou, Christopher Monkman, Andrew P. Pozina, Galia Kaliteevski, Mikhail A. Sci Rep Article Periodic metal-dielectric structures attract substantial interest since it was previously proposed that the spontaneous emission amplification rates (the Purcell factor) in such structures can reach enormous values up to 10(5). However, the role of absorption in real metals has not been thoroughly considered. We provide a theoretical analysis showing that absorption leads to diminishing values of Purcell factor. We also suggest that using emitting organic compounds such as CBP (4,4-Bis(N-carbazolyl)-1,1-biphenyl) can lead to a moderate increase of about an order of magnitude in the Purcell factor. Defining the experimentally measured Purcell factor as a ratio between the excited state lifetimes in bare CBP and in periodic structure, this increase in the fabricated periodic structure is demonstrated through a 4–8 times decrease in excited state radiative lifetime compared to a bare organic material in a wide emission spectrum. Nature Publishing Group UK 2019-07-03 /pmc/articles/PMC6610144/ /pubmed/31270385 http://dx.doi.org/10.1038/s41598-019-46071-5 Text en © The Author(s) 2019 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/. |
spellingShingle | Article Morozov, Konstantin M. Ivanov, Konstantin A. de Sa Pereira, Daniel Menelaou, Christopher Monkman, Andrew P. Pozina, Galia Kaliteevski, Mikhail A. Revising of the Purcell effect in periodic metal-dielectric structures: the role of absorption |
title | Revising of the Purcell effect in periodic metal-dielectric structures: the role of absorption |
title_full | Revising of the Purcell effect in periodic metal-dielectric structures: the role of absorption |
title_fullStr | Revising of the Purcell effect in periodic metal-dielectric structures: the role of absorption |
title_full_unstemmed | Revising of the Purcell effect in periodic metal-dielectric structures: the role of absorption |
title_short | Revising of the Purcell effect in periodic metal-dielectric structures: the role of absorption |
title_sort | revising of the purcell effect in periodic metal-dielectric structures: the role of absorption |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6610144/ https://www.ncbi.nlm.nih.gov/pubmed/31270385 http://dx.doi.org/10.1038/s41598-019-46071-5 |
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