Cargando…

Revising of the Purcell effect in periodic metal-dielectric structures: the role of absorption

Periodic metal-dielectric structures attract substantial interest since it was previously proposed that the spontaneous emission amplification rates (the Purcell factor) in such structures can reach enormous values up to 10(5). However, the role of absorption in real metals has not been thoroughly c...

Descripción completa

Detalles Bibliográficos
Autores principales: Morozov, Konstantin M., Ivanov, Konstantin A., de Sa Pereira, Daniel, Menelaou, Christopher, Monkman, Andrew P., Pozina, Galia, Kaliteevski, Mikhail A.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2019
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6610144/
https://www.ncbi.nlm.nih.gov/pubmed/31270385
http://dx.doi.org/10.1038/s41598-019-46071-5
_version_ 1783432449231945728
author Morozov, Konstantin M.
Ivanov, Konstantin A.
de Sa Pereira, Daniel
Menelaou, Christopher
Monkman, Andrew P.
Pozina, Galia
Kaliteevski, Mikhail A.
author_facet Morozov, Konstantin M.
Ivanov, Konstantin A.
de Sa Pereira, Daniel
Menelaou, Christopher
Monkman, Andrew P.
Pozina, Galia
Kaliteevski, Mikhail A.
author_sort Morozov, Konstantin M.
collection PubMed
description Periodic metal-dielectric structures attract substantial interest since it was previously proposed that the spontaneous emission amplification rates (the Purcell factor) in such structures can reach enormous values up to 10(5). However, the role of absorption in real metals has not been thoroughly considered. We provide a theoretical analysis showing that absorption leads to diminishing values of Purcell factor. We also suggest that using emitting organic compounds such as CBP (4,4-Bis(N-carbazolyl)-1,1-biphenyl) can lead to a moderate increase of about an order of magnitude in the Purcell factor. Defining the experimentally measured Purcell factor as a ratio between the excited state lifetimes in bare CBP and in periodic structure, this increase in the fabricated periodic structure is demonstrated through a 4–8 times decrease in excited state radiative lifetime compared to a bare organic material in a wide emission spectrum.
format Online
Article
Text
id pubmed-6610144
institution National Center for Biotechnology Information
language English
publishDate 2019
publisher Nature Publishing Group UK
record_format MEDLINE/PubMed
spelling pubmed-66101442019-07-14 Revising of the Purcell effect in periodic metal-dielectric structures: the role of absorption Morozov, Konstantin M. Ivanov, Konstantin A. de Sa Pereira, Daniel Menelaou, Christopher Monkman, Andrew P. Pozina, Galia Kaliteevski, Mikhail A. Sci Rep Article Periodic metal-dielectric structures attract substantial interest since it was previously proposed that the spontaneous emission amplification rates (the Purcell factor) in such structures can reach enormous values up to 10(5). However, the role of absorption in real metals has not been thoroughly considered. We provide a theoretical analysis showing that absorption leads to diminishing values of Purcell factor. We also suggest that using emitting organic compounds such as CBP (4,4-Bis(N-carbazolyl)-1,1-biphenyl) can lead to a moderate increase of about an order of magnitude in the Purcell factor. Defining the experimentally measured Purcell factor as a ratio between the excited state lifetimes in bare CBP and in periodic structure, this increase in the fabricated periodic structure is demonstrated through a 4–8 times decrease in excited state radiative lifetime compared to a bare organic material in a wide emission spectrum. Nature Publishing Group UK 2019-07-03 /pmc/articles/PMC6610144/ /pubmed/31270385 http://dx.doi.org/10.1038/s41598-019-46071-5 Text en © The Author(s) 2019 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Morozov, Konstantin M.
Ivanov, Konstantin A.
de Sa Pereira, Daniel
Menelaou, Christopher
Monkman, Andrew P.
Pozina, Galia
Kaliteevski, Mikhail A.
Revising of the Purcell effect in periodic metal-dielectric structures: the role of absorption
title Revising of the Purcell effect in periodic metal-dielectric structures: the role of absorption
title_full Revising of the Purcell effect in periodic metal-dielectric structures: the role of absorption
title_fullStr Revising of the Purcell effect in periodic metal-dielectric structures: the role of absorption
title_full_unstemmed Revising of the Purcell effect in periodic metal-dielectric structures: the role of absorption
title_short Revising of the Purcell effect in periodic metal-dielectric structures: the role of absorption
title_sort revising of the purcell effect in periodic metal-dielectric structures: the role of absorption
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6610144/
https://www.ncbi.nlm.nih.gov/pubmed/31270385
http://dx.doi.org/10.1038/s41598-019-46071-5
work_keys_str_mv AT morozovkonstantinm revisingofthepurcelleffectinperiodicmetaldielectricstructurestheroleofabsorption
AT ivanovkonstantina revisingofthepurcelleffectinperiodicmetaldielectricstructurestheroleofabsorption
AT desapereiradaniel revisingofthepurcelleffectinperiodicmetaldielectricstructurestheroleofabsorption
AT menelaouchristopher revisingofthepurcelleffectinperiodicmetaldielectricstructurestheroleofabsorption
AT monkmanandrewp revisingofthepurcelleffectinperiodicmetaldielectricstructurestheroleofabsorption
AT pozinagalia revisingofthepurcelleffectinperiodicmetaldielectricstructurestheroleofabsorption
AT kaliteevskimikhaila revisingofthepurcelleffectinperiodicmetaldielectricstructurestheroleofabsorption