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Characterization and Validation of a-Si Magnetron-Sputtered Thin Films as Solid He Targets with High Stability for Nuclear Reactions

[Image: see text] In this work, we present our magnetron sputtering based methodology to produce amorphous silicon coatings with closed porosity, as a strategy to fabricate solid helium targets, in the form of supported or self-supported thin films, for nuclear reactions. We show how by changing the...

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Autores principales: Godinho, Vanda, Ferrer, Francisco Javier, Fernández, Begoña, Caballero-Hernández, Jaime, Gómez-Camacho, Joaquin, Fernández, Asunción
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2016
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6640798/
https://www.ncbi.nlm.nih.gov/pubmed/31457191
http://dx.doi.org/10.1021/acsomega.6b00270
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author Godinho, Vanda
Ferrer, Francisco Javier
Fernández, Begoña
Caballero-Hernández, Jaime
Gómez-Camacho, Joaquin
Fernández, Asunción
author_facet Godinho, Vanda
Ferrer, Francisco Javier
Fernández, Begoña
Caballero-Hernández, Jaime
Gómez-Camacho, Joaquin
Fernández, Asunción
author_sort Godinho, Vanda
collection PubMed
description [Image: see text] In this work, we present our magnetron sputtering based methodology to produce amorphous silicon coatings with closed porosity, as a strategy to fabricate solid helium targets, in the form of supported or self-supported thin films, for nuclear reactions. We show how by changing the He working pressure it is possible to obtain highly porous homogeneous structures incorporating different He amounts. These porous coatings (a-Si:He) are very reproducible from run to run, and the high He amount incorporated makes them excellent candidates for solid He targets. The possibility of producing self-supported films is illustrated here, and its potential use in inverse kinematics experiments with radioactive beams is shown through the dispersion in forward geometry of a stable (6)Li beam. Also the elastic scattering cross-sections for proton from helium were determined using an a-Si:He coating. The results agree well with the ones reported in the literature. These two examples validate our coatings as good candidates to be used as solid He targets in nuclear reactions. The stability of He inside the coatings, fundamental for its use as solid He targets, was investigated, both over time and after irradiation. The coatings proved to be very stable, and the amount of He inside the pores remains unaltered at least 2 years after deposition and after high irradiation fluence (5 × 10(17) particles/cm(2); with a dose rate of 5 × 10(12) particles/(cm(2) s)).
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spelling pubmed-66407982019-08-27 Characterization and Validation of a-Si Magnetron-Sputtered Thin Films as Solid He Targets with High Stability for Nuclear Reactions Godinho, Vanda Ferrer, Francisco Javier Fernández, Begoña Caballero-Hernández, Jaime Gómez-Camacho, Joaquin Fernández, Asunción ACS Omega [Image: see text] In this work, we present our magnetron sputtering based methodology to produce amorphous silicon coatings with closed porosity, as a strategy to fabricate solid helium targets, in the form of supported or self-supported thin films, for nuclear reactions. We show how by changing the He working pressure it is possible to obtain highly porous homogeneous structures incorporating different He amounts. These porous coatings (a-Si:He) are very reproducible from run to run, and the high He amount incorporated makes them excellent candidates for solid He targets. The possibility of producing self-supported films is illustrated here, and its potential use in inverse kinematics experiments with radioactive beams is shown through the dispersion in forward geometry of a stable (6)Li beam. Also the elastic scattering cross-sections for proton from helium were determined using an a-Si:He coating. The results agree well with the ones reported in the literature. These two examples validate our coatings as good candidates to be used as solid He targets in nuclear reactions. The stability of He inside the coatings, fundamental for its use as solid He targets, was investigated, both over time and after irradiation. The coatings proved to be very stable, and the amount of He inside the pores remains unaltered at least 2 years after deposition and after high irradiation fluence (5 × 10(17) particles/cm(2); with a dose rate of 5 × 10(12) particles/(cm(2) s)). American Chemical Society 2016-12-14 /pmc/articles/PMC6640798/ /pubmed/31457191 http://dx.doi.org/10.1021/acsomega.6b00270 Text en Copyright © 2016 American Chemical Society This is an open access article published under a Creative Commons Attribution (CC-BY) License (http://pubs.acs.org/page/policy/authorchoice_ccby_termsofuse.html) , which permits unrestricted use, distribution and reproduction in any medium, provided the author and source are cited.
spellingShingle Godinho, Vanda
Ferrer, Francisco Javier
Fernández, Begoña
Caballero-Hernández, Jaime
Gómez-Camacho, Joaquin
Fernández, Asunción
Characterization and Validation of a-Si Magnetron-Sputtered Thin Films as Solid He Targets with High Stability for Nuclear Reactions
title Characterization and Validation of a-Si Magnetron-Sputtered Thin Films as Solid He Targets with High Stability for Nuclear Reactions
title_full Characterization and Validation of a-Si Magnetron-Sputtered Thin Films as Solid He Targets with High Stability for Nuclear Reactions
title_fullStr Characterization and Validation of a-Si Magnetron-Sputtered Thin Films as Solid He Targets with High Stability for Nuclear Reactions
title_full_unstemmed Characterization and Validation of a-Si Magnetron-Sputtered Thin Films as Solid He Targets with High Stability for Nuclear Reactions
title_short Characterization and Validation of a-Si Magnetron-Sputtered Thin Films as Solid He Targets with High Stability for Nuclear Reactions
title_sort characterization and validation of a-si magnetron-sputtered thin films as solid he targets with high stability for nuclear reactions
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6640798/
https://www.ncbi.nlm.nih.gov/pubmed/31457191
http://dx.doi.org/10.1021/acsomega.6b00270
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