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CdSe Quantum Dots/g-C(3)N(4) Heterostructure for Efficient H(2) Production under Visible Light Irradiation

[Image: see text] Novel photocatalysts -CdSe quantum dots (QDs)/g-C(3)N(4)- were successfully constructed. The structure, chemical composition, and optical properties of the prepared samples were investigated via a series of characterization techniques. The results indicated that CdSe QDs/g-C(3)N(4)...

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Autores principales: Zhong, Yunqian, Chen, Weiwei, Yu, Shan, Xie, Zhanghui, Wei, Shiqian, Zhou, Ying
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2018
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6643951/
https://www.ncbi.nlm.nih.gov/pubmed/31458373
http://dx.doi.org/10.1021/acsomega.8b02585
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author Zhong, Yunqian
Chen, Weiwei
Yu, Shan
Xie, Zhanghui
Wei, Shiqian
Zhou, Ying
author_facet Zhong, Yunqian
Chen, Weiwei
Yu, Shan
Xie, Zhanghui
Wei, Shiqian
Zhou, Ying
author_sort Zhong, Yunqian
collection PubMed
description [Image: see text] Novel photocatalysts -CdSe quantum dots (QDs)/g-C(3)N(4)- were successfully constructed. The structure, chemical composition, and optical properties of the prepared samples were investigated via a series of characterization techniques. The results indicated that CdSe QDs/g-C(3)N(4) photocatalysts exhibited remarkably enhanced photocatalytic activity for visible-light-induced H(2) evolution compared to pristine g-C(3)N(4) and CdSe QDs and addition of 13.6 wt % CdSe QDs into the composite photocatalyst generated the highest H(2) production rate. The enhanced photocatalytic performance of CdSe QDs/g-C(3)N(4) can be attributed to the synergistic effects of excellent visible absorption and high charge separation efficiency from the heterostructure. This work could not only provide a facile method to fabricate semiconductor QDs-modified g-C(3)N(4) photocatalysts but also contribute to the design for heterostructures.
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spelling pubmed-66439512019-08-27 CdSe Quantum Dots/g-C(3)N(4) Heterostructure for Efficient H(2) Production under Visible Light Irradiation Zhong, Yunqian Chen, Weiwei Yu, Shan Xie, Zhanghui Wei, Shiqian Zhou, Ying ACS Omega [Image: see text] Novel photocatalysts -CdSe quantum dots (QDs)/g-C(3)N(4)- were successfully constructed. The structure, chemical composition, and optical properties of the prepared samples were investigated via a series of characterization techniques. The results indicated that CdSe QDs/g-C(3)N(4) photocatalysts exhibited remarkably enhanced photocatalytic activity for visible-light-induced H(2) evolution compared to pristine g-C(3)N(4) and CdSe QDs and addition of 13.6 wt % CdSe QDs into the composite photocatalyst generated the highest H(2) production rate. The enhanced photocatalytic performance of CdSe QDs/g-C(3)N(4) can be attributed to the synergistic effects of excellent visible absorption and high charge separation efficiency from the heterostructure. This work could not only provide a facile method to fabricate semiconductor QDs-modified g-C(3)N(4) photocatalysts but also contribute to the design for heterostructures. American Chemical Society 2018-12-19 /pmc/articles/PMC6643951/ /pubmed/31458373 http://dx.doi.org/10.1021/acsomega.8b02585 Text en Copyright © 2018 American Chemical Society This is an open access article published under an ACS AuthorChoice License (http://pubs.acs.org/page/policy/authorchoice_termsofuse.html) , which permits copying and redistribution of the article or any adaptations for non-commercial purposes.
spellingShingle Zhong, Yunqian
Chen, Weiwei
Yu, Shan
Xie, Zhanghui
Wei, Shiqian
Zhou, Ying
CdSe Quantum Dots/g-C(3)N(4) Heterostructure for Efficient H(2) Production under Visible Light Irradiation
title CdSe Quantum Dots/g-C(3)N(4) Heterostructure for Efficient H(2) Production under Visible Light Irradiation
title_full CdSe Quantum Dots/g-C(3)N(4) Heterostructure for Efficient H(2) Production under Visible Light Irradiation
title_fullStr CdSe Quantum Dots/g-C(3)N(4) Heterostructure for Efficient H(2) Production under Visible Light Irradiation
title_full_unstemmed CdSe Quantum Dots/g-C(3)N(4) Heterostructure for Efficient H(2) Production under Visible Light Irradiation
title_short CdSe Quantum Dots/g-C(3)N(4) Heterostructure for Efficient H(2) Production under Visible Light Irradiation
title_sort cdse quantum dots/g-c(3)n(4) heterostructure for efficient h(2) production under visible light irradiation
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6643951/
https://www.ncbi.nlm.nih.gov/pubmed/31458373
http://dx.doi.org/10.1021/acsomega.8b02585
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