Cargando…
CdSe Quantum Dots/g-C(3)N(4) Heterostructure for Efficient H(2) Production under Visible Light Irradiation
[Image: see text] Novel photocatalysts -CdSe quantum dots (QDs)/g-C(3)N(4)- were successfully constructed. The structure, chemical composition, and optical properties of the prepared samples were investigated via a series of characterization techniques. The results indicated that CdSe QDs/g-C(3)N(4)...
Autores principales: | , , , , , |
---|---|
Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American Chemical Society
2018
|
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6643951/ https://www.ncbi.nlm.nih.gov/pubmed/31458373 http://dx.doi.org/10.1021/acsomega.8b02585 |
_version_ | 1783437184613744640 |
---|---|
author | Zhong, Yunqian Chen, Weiwei Yu, Shan Xie, Zhanghui Wei, Shiqian Zhou, Ying |
author_facet | Zhong, Yunqian Chen, Weiwei Yu, Shan Xie, Zhanghui Wei, Shiqian Zhou, Ying |
author_sort | Zhong, Yunqian |
collection | PubMed |
description | [Image: see text] Novel photocatalysts -CdSe quantum dots (QDs)/g-C(3)N(4)- were successfully constructed. The structure, chemical composition, and optical properties of the prepared samples were investigated via a series of characterization techniques. The results indicated that CdSe QDs/g-C(3)N(4) photocatalysts exhibited remarkably enhanced photocatalytic activity for visible-light-induced H(2) evolution compared to pristine g-C(3)N(4) and CdSe QDs and addition of 13.6 wt % CdSe QDs into the composite photocatalyst generated the highest H(2) production rate. The enhanced photocatalytic performance of CdSe QDs/g-C(3)N(4) can be attributed to the synergistic effects of excellent visible absorption and high charge separation efficiency from the heterostructure. This work could not only provide a facile method to fabricate semiconductor QDs-modified g-C(3)N(4) photocatalysts but also contribute to the design for heterostructures. |
format | Online Article Text |
id | pubmed-6643951 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2018 |
publisher | American Chemical Society |
record_format | MEDLINE/PubMed |
spelling | pubmed-66439512019-08-27 CdSe Quantum Dots/g-C(3)N(4) Heterostructure for Efficient H(2) Production under Visible Light Irradiation Zhong, Yunqian Chen, Weiwei Yu, Shan Xie, Zhanghui Wei, Shiqian Zhou, Ying ACS Omega [Image: see text] Novel photocatalysts -CdSe quantum dots (QDs)/g-C(3)N(4)- were successfully constructed. The structure, chemical composition, and optical properties of the prepared samples were investigated via a series of characterization techniques. The results indicated that CdSe QDs/g-C(3)N(4) photocatalysts exhibited remarkably enhanced photocatalytic activity for visible-light-induced H(2) evolution compared to pristine g-C(3)N(4) and CdSe QDs and addition of 13.6 wt % CdSe QDs into the composite photocatalyst generated the highest H(2) production rate. The enhanced photocatalytic performance of CdSe QDs/g-C(3)N(4) can be attributed to the synergistic effects of excellent visible absorption and high charge separation efficiency from the heterostructure. This work could not only provide a facile method to fabricate semiconductor QDs-modified g-C(3)N(4) photocatalysts but also contribute to the design for heterostructures. American Chemical Society 2018-12-19 /pmc/articles/PMC6643951/ /pubmed/31458373 http://dx.doi.org/10.1021/acsomega.8b02585 Text en Copyright © 2018 American Chemical Society This is an open access article published under an ACS AuthorChoice License (http://pubs.acs.org/page/policy/authorchoice_termsofuse.html) , which permits copying and redistribution of the article or any adaptations for non-commercial purposes. |
spellingShingle | Zhong, Yunqian Chen, Weiwei Yu, Shan Xie, Zhanghui Wei, Shiqian Zhou, Ying CdSe Quantum Dots/g-C(3)N(4) Heterostructure for Efficient H(2) Production under Visible Light Irradiation |
title | CdSe Quantum Dots/g-C(3)N(4) Heterostructure
for Efficient H(2) Production under Visible
Light Irradiation |
title_full | CdSe Quantum Dots/g-C(3)N(4) Heterostructure
for Efficient H(2) Production under Visible
Light Irradiation |
title_fullStr | CdSe Quantum Dots/g-C(3)N(4) Heterostructure
for Efficient H(2) Production under Visible
Light Irradiation |
title_full_unstemmed | CdSe Quantum Dots/g-C(3)N(4) Heterostructure
for Efficient H(2) Production under Visible
Light Irradiation |
title_short | CdSe Quantum Dots/g-C(3)N(4) Heterostructure
for Efficient H(2) Production under Visible
Light Irradiation |
title_sort | cdse quantum dots/g-c(3)n(4) heterostructure
for efficient h(2) production under visible
light irradiation |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6643951/ https://www.ncbi.nlm.nih.gov/pubmed/31458373 http://dx.doi.org/10.1021/acsomega.8b02585 |
work_keys_str_mv | AT zhongyunqian cdsequantumdotsgc3n4heterostructureforefficienth2productionundervisiblelightirradiation AT chenweiwei cdsequantumdotsgc3n4heterostructureforefficienth2productionundervisiblelightirradiation AT yushan cdsequantumdotsgc3n4heterostructureforefficienth2productionundervisiblelightirradiation AT xiezhanghui cdsequantumdotsgc3n4heterostructureforefficienth2productionundervisiblelightirradiation AT weishiqian cdsequantumdotsgc3n4heterostructureforefficienth2productionundervisiblelightirradiation AT zhouying cdsequantumdotsgc3n4heterostructureforefficienth2productionundervisiblelightirradiation |