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Propagating Precipitation Waves in Disordered Media
[Image: see text] The study presented in this paper investigates form changes of propagating waves generated through precipitation reactions in a gel matrix that possesses an inhomogeneous microstructure. The waves demonstrate form changes from a single ring-like pattern to multiple target-like wave...
Autores principales: | , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American Chemical Society
2017
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Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6645417/ https://www.ncbi.nlm.nih.gov/pubmed/31457353 http://dx.doi.org/10.1021/acsomega.7b01271 |
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author | Ban, Takahiko Kaji, Masaru Nagatsu, Yuichiro Tokuyama, Hideaki |
author_facet | Ban, Takahiko Kaji, Masaru Nagatsu, Yuichiro Tokuyama, Hideaki |
author_sort | Ban, Takahiko |
collection | PubMed |
description | [Image: see text] The study presented in this paper investigates form changes of propagating waves generated through precipitation reactions in a gel matrix that possesses an inhomogeneous microstructure. The waves demonstrate form changes from a single ring-like pattern to multiple target-like waves. Subsequently, the waves take up a spiral form and ultimately manifest themselves in the form of a turbulence pattern that intensifies with increasing fluctuations within the gel structure. An investigation into the dynamics of the precipitation waves reveals the existence of an anomalous diffusion. The effective diffusion coefficients are found to increase linearly with the quenching temperature. Further, it is revealed through the analysis of the anomalous diffusion dynamics that precipitation patterns could be adequately controlled by adjusting the permeability fluctuations within the gel structure. The findings of this study lead to a greater understanding of the spontaneous creation of precipitation patterns by a system driven by disorder. |
format | Online Article Text |
id | pubmed-6645417 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2017 |
publisher | American Chemical Society |
record_format | MEDLINE/PubMed |
spelling | pubmed-66454172019-08-27 Propagating Precipitation Waves in Disordered Media Ban, Takahiko Kaji, Masaru Nagatsu, Yuichiro Tokuyama, Hideaki ACS Omega [Image: see text] The study presented in this paper investigates form changes of propagating waves generated through precipitation reactions in a gel matrix that possesses an inhomogeneous microstructure. The waves demonstrate form changes from a single ring-like pattern to multiple target-like waves. Subsequently, the waves take up a spiral form and ultimately manifest themselves in the form of a turbulence pattern that intensifies with increasing fluctuations within the gel structure. An investigation into the dynamics of the precipitation waves reveals the existence of an anomalous diffusion. The effective diffusion coefficients are found to increase linearly with the quenching temperature. Further, it is revealed through the analysis of the anomalous diffusion dynamics that precipitation patterns could be adequately controlled by adjusting the permeability fluctuations within the gel structure. The findings of this study lead to a greater understanding of the spontaneous creation of precipitation patterns by a system driven by disorder. American Chemical Society 2017-11-16 /pmc/articles/PMC6645417/ /pubmed/31457353 http://dx.doi.org/10.1021/acsomega.7b01271 Text en Copyright © 2017 American Chemical Society This is an open access article published under an ACS AuthorChoice License (http://pubs.acs.org/page/policy/authorchoice_termsofuse.html) , which permits copying and redistribution of the article or any adaptations for non-commercial purposes. |
spellingShingle | Ban, Takahiko Kaji, Masaru Nagatsu, Yuichiro Tokuyama, Hideaki Propagating Precipitation Waves in Disordered Media |
title | Propagating Precipitation Waves in Disordered Media |
title_full | Propagating Precipitation Waves in Disordered Media |
title_fullStr | Propagating Precipitation Waves in Disordered Media |
title_full_unstemmed | Propagating Precipitation Waves in Disordered Media |
title_short | Propagating Precipitation Waves in Disordered Media |
title_sort | propagating precipitation waves in disordered media |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6645417/ https://www.ncbi.nlm.nih.gov/pubmed/31457353 http://dx.doi.org/10.1021/acsomega.7b01271 |
work_keys_str_mv | AT bantakahiko propagatingprecipitationwavesindisorderedmedia AT kajimasaru propagatingprecipitationwavesindisorderedmedia AT nagatsuyuichiro propagatingprecipitationwavesindisorderedmedia AT tokuyamahideaki propagatingprecipitationwavesindisorderedmedia |