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Turing Patterns and Waves in Closed Two-Layer Gel Reactors

[Image: see text] Reaction–diffusion waves and stationary Turing patterns are observed in closed two-layer gel reactors, where the two compartments are initially filled with complementary sets of reactants of the chlorine dioxide–iodine–malonic acid–poly(vinyl alcohol) reaction. The asymmetrical loa...

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Autores principales: Dúzs, Brigitta, De Kepper, Patrick, Szalai, István
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2019
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6648942/
https://www.ncbi.nlm.nih.gov/pubmed/31459538
http://dx.doi.org/10.1021/acsomega.8b02997
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author Dúzs, Brigitta
De Kepper, Patrick
Szalai, István
author_facet Dúzs, Brigitta
De Kepper, Patrick
Szalai, István
author_sort Dúzs, Brigitta
collection PubMed
description [Image: see text] Reaction–diffusion waves and stationary Turing patterns are observed in closed two-layer gel reactors, where the two compartments are initially filled with complementary sets of reactants of the chlorine dioxide–iodine–malonic acid–poly(vinyl alcohol) reaction. The asymmetrical loading generates concentration gradients and the patterns form at the interface between the two parts. These easy-to-perform experiments allow us to study a wide range of dynamical phenomena without requiring a specific reactor design or the use of sophisticated equipment. To get complementary information on pattern formation in parallel and perpendicular to the direction of the concentration gradients, two geometrically different configurations of compartments are presented. We demonstrate that three variants of the initial distribution of the chemicals can be equally applied, and this flexibility provides a way to introduce additional reagents to perturb the dynamics of the systems. A noticeable increase in the wavelength of Turing patterns and in the period of waves has been induced by adding bromide ions. The interaction of Turing and Hopf modes has been observed as a result of not only the variation of the initial poly(vinyl alcohol) concentration but that of the gradients as well.
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spelling pubmed-66489422019-08-27 Turing Patterns and Waves in Closed Two-Layer Gel Reactors Dúzs, Brigitta De Kepper, Patrick Szalai, István ACS Omega [Image: see text] Reaction–diffusion waves and stationary Turing patterns are observed in closed two-layer gel reactors, where the two compartments are initially filled with complementary sets of reactants of the chlorine dioxide–iodine–malonic acid–poly(vinyl alcohol) reaction. The asymmetrical loading generates concentration gradients and the patterns form at the interface between the two parts. These easy-to-perform experiments allow us to study a wide range of dynamical phenomena without requiring a specific reactor design or the use of sophisticated equipment. To get complementary information on pattern formation in parallel and perpendicular to the direction of the concentration gradients, two geometrically different configurations of compartments are presented. We demonstrate that three variants of the initial distribution of the chemicals can be equally applied, and this flexibility provides a way to introduce additional reagents to perturb the dynamics of the systems. A noticeable increase in the wavelength of Turing patterns and in the period of waves has been induced by adding bromide ions. The interaction of Turing and Hopf modes has been observed as a result of not only the variation of the initial poly(vinyl alcohol) concentration but that of the gradients as well. American Chemical Society 2019-02-14 /pmc/articles/PMC6648942/ /pubmed/31459538 http://dx.doi.org/10.1021/acsomega.8b02997 Text en Copyright © 2019 American Chemical Society This is an open access article published under an ACS AuthorChoice License (http://pubs.acs.org/page/policy/authorchoice_termsofuse.html) , which permits copying and redistribution of the article or any adaptations for non-commercial purposes.
spellingShingle Dúzs, Brigitta
De Kepper, Patrick
Szalai, István
Turing Patterns and Waves in Closed Two-Layer Gel Reactors
title Turing Patterns and Waves in Closed Two-Layer Gel Reactors
title_full Turing Patterns and Waves in Closed Two-Layer Gel Reactors
title_fullStr Turing Patterns and Waves in Closed Two-Layer Gel Reactors
title_full_unstemmed Turing Patterns and Waves in Closed Two-Layer Gel Reactors
title_short Turing Patterns and Waves in Closed Two-Layer Gel Reactors
title_sort turing patterns and waves in closed two-layer gel reactors
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6648942/
https://www.ncbi.nlm.nih.gov/pubmed/31459538
http://dx.doi.org/10.1021/acsomega.8b02997
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