Facile Preparation and Enhanced Catalytic Properties of Self-Assembled Pd Nanoparticle-Loaded Nanocomposite Films Synthesized via the Electrospun Approach

[Image: see text] In recent years, people pay more attention to environmental pollution and the treatment of sewage has become the focus of recent research. Palladium nanoparticles have good catalytic properties but are easy to agglomerate. Therefore, we used the electrospinning technology to prepare a uniform composite nanofiber film based on polyacrylic acid (PAA) and polyvinyl alcohol (PVA), which demonstrated that they are good carriers of palladium nanoparticles to make the nanoparticles well dispersed. Furthermore, carbon nanotubes (CNTs) were added to increase the specific surface area of the composite nanofiber film and improve its mechanical properties. The successfully synthesized PAA/PVA/CNT-COOH@palladium nanoparticle (PdNP) composite fiber films were characterized by scanning electron microscopy, transmission electron microscopy, and thermogravimetry analysis. p-Nitrophenol and 2-nitroaniline were utilized as typical pollutants to further evaluate the catalytic performance of PAA/PVA/CNT-COOH@PdNP composite fiber films. The PAA/PVA/CNT-COOH@PdNP composite fiber films exhibited enhanced catalytic performance and could be reused for eight consecutive cycles. This work provided new clues for the preparation and application of composite electrospun film materials.