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Modeling and Selection of RF Thermal Plasma Hot-Wall Torch for Large-Scale Production of Nanopowders

Fouling is a great problem that significantly affects the continuous operation for large-scale radio-frequency (RF) thermal plasma synthesizing nanopowders. In order to eliminate or weaken the phenomenon, numerical simulations based on FLUENT software were founded to investigate the effect of operat...

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Autores principales: Bai, Liuyang, He, Jiaping, Ouyang, Yuge, Liu, Wenfu, Liu, Huichao, Yao, Haizi, Li, Zengshuai, Song, Jun, Wang, Yinling, Yuan, Fangli
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2019
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6651854/
https://www.ncbi.nlm.nih.gov/pubmed/31277239
http://dx.doi.org/10.3390/ma12132141
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author Bai, Liuyang
He, Jiaping
Ouyang, Yuge
Liu, Wenfu
Liu, Huichao
Yao, Haizi
Li, Zengshuai
Song, Jun
Wang, Yinling
Yuan, Fangli
author_facet Bai, Liuyang
He, Jiaping
Ouyang, Yuge
Liu, Wenfu
Liu, Huichao
Yao, Haizi
Li, Zengshuai
Song, Jun
Wang, Yinling
Yuan, Fangli
author_sort Bai, Liuyang
collection PubMed
description Fouling is a great problem that significantly affects the continuous operation for large-scale radio-frequency (RF) thermal plasma synthesizing nanopowders. In order to eliminate or weaken the phenomenon, numerical simulations based on FLUENT software were founded to investigate the effect of operation parameters, including feeding style of central gas and sheath gas, on plasma torches. It is shown that the tangential feeding style of central gas brings serious negative axial velocity regions, which always forces the synthesized nanopowders to “back-mix”, and further leads to the fouling of the quartz tube. Moreover, it is shown that sheath gas should be tangentially fed into the plasma reactor to further eliminate the gas stream’s back-mixing. However, when this feeding style is applied, although the negative axial velocity region is decreased, the plasma gas and kinetic energy of the vapor phase near the wall of the plasma reactor are less and lower, respectively; as a result, that plasma flame is more difficult to be arced. A new plasma arcing method by way of feeding gun instead of torch wall was proposed and put in use. The fouling problem has been well solved and plasma arcing is well ensured, and as a result, the experiment on large-scale production of nanopowders can be carried out for 8 h without any interruption, and synthesized Si and Al(2)O(3) nanopowders exhibit good dispersion and sphericity.
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spelling pubmed-66518542019-08-08 Modeling and Selection of RF Thermal Plasma Hot-Wall Torch for Large-Scale Production of Nanopowders Bai, Liuyang He, Jiaping Ouyang, Yuge Liu, Wenfu Liu, Huichao Yao, Haizi Li, Zengshuai Song, Jun Wang, Yinling Yuan, Fangli Materials (Basel) Article Fouling is a great problem that significantly affects the continuous operation for large-scale radio-frequency (RF) thermal plasma synthesizing nanopowders. In order to eliminate or weaken the phenomenon, numerical simulations based on FLUENT software were founded to investigate the effect of operation parameters, including feeding style of central gas and sheath gas, on plasma torches. It is shown that the tangential feeding style of central gas brings serious negative axial velocity regions, which always forces the synthesized nanopowders to “back-mix”, and further leads to the fouling of the quartz tube. Moreover, it is shown that sheath gas should be tangentially fed into the plasma reactor to further eliminate the gas stream’s back-mixing. However, when this feeding style is applied, although the negative axial velocity region is decreased, the plasma gas and kinetic energy of the vapor phase near the wall of the plasma reactor are less and lower, respectively; as a result, that plasma flame is more difficult to be arced. A new plasma arcing method by way of feeding gun instead of torch wall was proposed and put in use. The fouling problem has been well solved and plasma arcing is well ensured, and as a result, the experiment on large-scale production of nanopowders can be carried out for 8 h without any interruption, and synthesized Si and Al(2)O(3) nanopowders exhibit good dispersion and sphericity. MDPI 2019-07-03 /pmc/articles/PMC6651854/ /pubmed/31277239 http://dx.doi.org/10.3390/ma12132141 Text en © 2019 by the authors. Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (http://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Bai, Liuyang
He, Jiaping
Ouyang, Yuge
Liu, Wenfu
Liu, Huichao
Yao, Haizi
Li, Zengshuai
Song, Jun
Wang, Yinling
Yuan, Fangli
Modeling and Selection of RF Thermal Plasma Hot-Wall Torch for Large-Scale Production of Nanopowders
title Modeling and Selection of RF Thermal Plasma Hot-Wall Torch for Large-Scale Production of Nanopowders
title_full Modeling and Selection of RF Thermal Plasma Hot-Wall Torch for Large-Scale Production of Nanopowders
title_fullStr Modeling and Selection of RF Thermal Plasma Hot-Wall Torch for Large-Scale Production of Nanopowders
title_full_unstemmed Modeling and Selection of RF Thermal Plasma Hot-Wall Torch for Large-Scale Production of Nanopowders
title_short Modeling and Selection of RF Thermal Plasma Hot-Wall Torch for Large-Scale Production of Nanopowders
title_sort modeling and selection of rf thermal plasma hot-wall torch for large-scale production of nanopowders
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6651854/
https://www.ncbi.nlm.nih.gov/pubmed/31277239
http://dx.doi.org/10.3390/ma12132141
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