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Porous Carbon Networks Derived From Graphitic Carbon Nitride for Efficient Oxygen Reduction Reaction

Great efforts have been dedicated to finding economic and efficient oxygen reduction reaction (ORR) for fuel cell technology. Among various catalysts, N-doped carbon-based nanomaterials have attracted much attention due to low-cost, noble metal free, and good durability. Herein, we developed a facil...

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Detalles Bibliográficos
Autores principales: Li, Chenxia, Li, Xuesong, Sun, Xiaojuan, Zhang, Xueyu, Duan, Lianfeng, Yang, Xijia, Wang, Liying, Lü, Wei
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Springer US 2019
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6656852/
https://www.ncbi.nlm.nih.gov/pubmed/31342197
http://dx.doi.org/10.1186/s11671-019-3073-0
Descripción
Sumario:Great efforts have been dedicated to finding economic and efficient oxygen reduction reaction (ORR) for fuel cell technology. Among various catalysts, N-doped carbon-based nanomaterials have attracted much attention due to low-cost, noble metal free, and good durability. Herein, we developed a facile and economic strategy to prepare nitrogen-doped carbon networks for efficient ORR application. The g-C(3)N(4) is used as the template and N source, and dopamine is used as the carbon source. By simple hydrothermal treatment and sintering, N-doped carbon network structures with high specific surface area, effective ORR activity, and superior durability could be acquired. The present strategy is free of involving generally multistep, poisonous reagents, and complication of removing template for fabrication of 3D carbon structures. ELECTRONIC SUPPLEMENTARY MATERIAL: The online version of this article (10.1186/s11671-019-3073-0) contains supplementary material, which is available to authorized users.