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Ultrafast time-resolved x-ray scattering reveals diffusive charge order dynamics in La(2–x)Ba(x)CuO(4)

Charge order is universal among high-T(c) cuprates, but its relation to superconductivity is unclear. While static order competes with superconductivity, dynamic order may be favorable and even contribute to Cooper pairing. Using time-resolved resonant soft x-ray scattering at a free-electron laser,...

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Autores principales: Mitrano, Matteo, Lee, Sangjun, Husain, Ali A., Delacretaz, Luca, Zhu, Minhui, de la Peña Munoz, Gilberto, Sun, Stella X.-L., Joe, Young Il, Reid, Alexander H., Wandel, Scott F., Coslovich, Giacomo, Schlotter, William, van Driel, Tim, Schneeloch, John, Gu, G. D., Hartnoll, Sean, Goldenfeld, Nigel, Abbamonte, Peter
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Association for the Advancement of Science 2019
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6697434/
https://www.ncbi.nlm.nih.gov/pubmed/31453340
http://dx.doi.org/10.1126/sciadv.aax3346
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author Mitrano, Matteo
Lee, Sangjun
Husain, Ali A.
Delacretaz, Luca
Zhu, Minhui
de la Peña Munoz, Gilberto
Sun, Stella X.-L.
Joe, Young Il
Reid, Alexander H.
Wandel, Scott F.
Coslovich, Giacomo
Schlotter, William
van Driel, Tim
Schneeloch, John
Gu, G. D.
Hartnoll, Sean
Goldenfeld, Nigel
Abbamonte, Peter
author_facet Mitrano, Matteo
Lee, Sangjun
Husain, Ali A.
Delacretaz, Luca
Zhu, Minhui
de la Peña Munoz, Gilberto
Sun, Stella X.-L.
Joe, Young Il
Reid, Alexander H.
Wandel, Scott F.
Coslovich, Giacomo
Schlotter, William
van Driel, Tim
Schneeloch, John
Gu, G. D.
Hartnoll, Sean
Goldenfeld, Nigel
Abbamonte, Peter
author_sort Mitrano, Matteo
collection PubMed
description Charge order is universal among high-T(c) cuprates, but its relation to superconductivity is unclear. While static order competes with superconductivity, dynamic order may be favorable and even contribute to Cooper pairing. Using time-resolved resonant soft x-ray scattering at a free-electron laser, we show that the charge order in prototypical La(2−x)Ba(x)CuO(4) exhibits transverse fluctuations at picosecond time scales. These sub–millielectron volt excitations propagate by Brownian-like diffusion and have an energy scale remarkably close to the superconducting T(c). At sub–millielectron volt energy scales, the dynamics are governed by universal scaling laws defined by the propagation of topological defects. Our results show that charge order in La(2−x)Ba(x)CuO(4) exhibits dynamics favorable to the in-plane superconducting tunneling and establish time-resolved x-rays as a means to study excitations at energy scales inaccessible to conventional scattering techniques.
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spelling pubmed-66974342019-08-26 Ultrafast time-resolved x-ray scattering reveals diffusive charge order dynamics in La(2–x)Ba(x)CuO(4) Mitrano, Matteo Lee, Sangjun Husain, Ali A. Delacretaz, Luca Zhu, Minhui de la Peña Munoz, Gilberto Sun, Stella X.-L. Joe, Young Il Reid, Alexander H. Wandel, Scott F. Coslovich, Giacomo Schlotter, William van Driel, Tim Schneeloch, John Gu, G. D. Hartnoll, Sean Goldenfeld, Nigel Abbamonte, Peter Sci Adv Research Articles Charge order is universal among high-T(c) cuprates, but its relation to superconductivity is unclear. While static order competes with superconductivity, dynamic order may be favorable and even contribute to Cooper pairing. Using time-resolved resonant soft x-ray scattering at a free-electron laser, we show that the charge order in prototypical La(2−x)Ba(x)CuO(4) exhibits transverse fluctuations at picosecond time scales. These sub–millielectron volt excitations propagate by Brownian-like diffusion and have an energy scale remarkably close to the superconducting T(c). At sub–millielectron volt energy scales, the dynamics are governed by universal scaling laws defined by the propagation of topological defects. Our results show that charge order in La(2−x)Ba(x)CuO(4) exhibits dynamics favorable to the in-plane superconducting tunneling and establish time-resolved x-rays as a means to study excitations at energy scales inaccessible to conventional scattering techniques. American Association for the Advancement of Science 2019-08-16 /pmc/articles/PMC6697434/ /pubmed/31453340 http://dx.doi.org/10.1126/sciadv.aax3346 Text en Copyright © 2019 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution NonCommercial License 4.0 (CC BY-NC). http://creativecommons.org/licenses/by-nc/4.0/ This is an open-access article distributed under the terms of the Creative Commons Attribution-NonCommercial license (http://creativecommons.org/licenses/by-nc/4.0/) , which permits use, distribution, and reproduction in any medium, so long as the resultant use is not for commercial advantage and provided the original work is properly cited.
spellingShingle Research Articles
Mitrano, Matteo
Lee, Sangjun
Husain, Ali A.
Delacretaz, Luca
Zhu, Minhui
de la Peña Munoz, Gilberto
Sun, Stella X.-L.
Joe, Young Il
Reid, Alexander H.
Wandel, Scott F.
Coslovich, Giacomo
Schlotter, William
van Driel, Tim
Schneeloch, John
Gu, G. D.
Hartnoll, Sean
Goldenfeld, Nigel
Abbamonte, Peter
Ultrafast time-resolved x-ray scattering reveals diffusive charge order dynamics in La(2–x)Ba(x)CuO(4)
title Ultrafast time-resolved x-ray scattering reveals diffusive charge order dynamics in La(2–x)Ba(x)CuO(4)
title_full Ultrafast time-resolved x-ray scattering reveals diffusive charge order dynamics in La(2–x)Ba(x)CuO(4)
title_fullStr Ultrafast time-resolved x-ray scattering reveals diffusive charge order dynamics in La(2–x)Ba(x)CuO(4)
title_full_unstemmed Ultrafast time-resolved x-ray scattering reveals diffusive charge order dynamics in La(2–x)Ba(x)CuO(4)
title_short Ultrafast time-resolved x-ray scattering reveals diffusive charge order dynamics in La(2–x)Ba(x)CuO(4)
title_sort ultrafast time-resolved x-ray scattering reveals diffusive charge order dynamics in la(2–x)ba(x)cuo(4)
topic Research Articles
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6697434/
https://www.ncbi.nlm.nih.gov/pubmed/31453340
http://dx.doi.org/10.1126/sciadv.aax3346
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