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In situ observation of picosecond polaron self-localisation in α-Fe(2)O(3) photoelectrochemical cells
Hematite (α-Fe(2)O(3)) is the most studied artificial oxygen-evolving photo-anode and yet its efficiency limitations and their origin remain unknown. A sub-picosecond reorganisation of the hematite structure has been proposed as the mechanism which dictates carrier lifetimes, energetics and the ulti...
Autores principales: | Pastor, Ernest, Park, Ji-Sang, Steier, Ludmilla, Kim, Sunghyun, Grätzel, Michael, Durrant, James R., Walsh, Aron, Bakulin, Artem A. |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group UK
2019
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6722133/ https://www.ncbi.nlm.nih.gov/pubmed/31481691 http://dx.doi.org/10.1038/s41467-019-11767-9 |
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