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Double-sided slippery liquid-infused porous materials using conformable mesh

Often wetting is considered from the perspective of a single surface of a rigid substrate and its topographical properties such as roughness or texture. However, many substrates, such as membranes and meshes, have two useful surfaces. Such flexible substrates also offer the potential to be formed in...

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Autores principales: Geraldi, Nicasio R., Guan, Jian H., Dodd, Linzi E., Maiello, Pietro, Xu, Ben B., Wood, David, Newton, Michael I., Wells, Gary G., McHale, Glen
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2019
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6746700/
https://www.ncbi.nlm.nih.gov/pubmed/31527694
http://dx.doi.org/10.1038/s41598-019-49887-3
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author Geraldi, Nicasio R.
Guan, Jian H.
Dodd, Linzi E.
Maiello, Pietro
Xu, Ben B.
Wood, David
Newton, Michael I.
Wells, Gary G.
McHale, Glen
author_facet Geraldi, Nicasio R.
Guan, Jian H.
Dodd, Linzi E.
Maiello, Pietro
Xu, Ben B.
Wood, David
Newton, Michael I.
Wells, Gary G.
McHale, Glen
author_sort Geraldi, Nicasio R.
collection PubMed
description Often wetting is considered from the perspective of a single surface of a rigid substrate and its topographical properties such as roughness or texture. However, many substrates, such as membranes and meshes, have two useful surfaces. Such flexible substrates also offer the potential to be formed into structures with either a double-sided surface (e.g. by joining the ends of a mesh as a tape) or a single-sided surface (e.g. by ends with a half-twist). When a substrate possesses holes, it is also possible to consider how the spaces in the substrate may be connected or disconnected. This combination of flexibility, holes and connectedness can therefore be used to introduce topological concepts, which are distinct from simple topography. Here, we present a method to create a Slippery Liquid-Infused Porous Surface (SLIPS) coating on flexible conformable doubled-sided meshes and for coating complex geometries. By considering the flexibility and connectedness of a mesh with the surface properties of SLIPS, we show it is possible to create double-sided SLIPS materials with high droplet mobility and droplet control on both faces. We also exemplify the importance of flexibility using a mesh-based SLIPS pipe capable of withstanding laminar and turbulent flows for 180 and 90 minutes, respectively. Finally, we discuss how ideas of topology introduced by the SLIPS mesh might be extended to create completely new types of SLIPS systems, such as Mobius strips and auxetic metamaterials.
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spelling pubmed-67467002019-09-27 Double-sided slippery liquid-infused porous materials using conformable mesh Geraldi, Nicasio R. Guan, Jian H. Dodd, Linzi E. Maiello, Pietro Xu, Ben B. Wood, David Newton, Michael I. Wells, Gary G. McHale, Glen Sci Rep Article Often wetting is considered from the perspective of a single surface of a rigid substrate and its topographical properties such as roughness or texture. However, many substrates, such as membranes and meshes, have two useful surfaces. Such flexible substrates also offer the potential to be formed into structures with either a double-sided surface (e.g. by joining the ends of a mesh as a tape) or a single-sided surface (e.g. by ends with a half-twist). When a substrate possesses holes, it is also possible to consider how the spaces in the substrate may be connected or disconnected. This combination of flexibility, holes and connectedness can therefore be used to introduce topological concepts, which are distinct from simple topography. Here, we present a method to create a Slippery Liquid-Infused Porous Surface (SLIPS) coating on flexible conformable doubled-sided meshes and for coating complex geometries. By considering the flexibility and connectedness of a mesh with the surface properties of SLIPS, we show it is possible to create double-sided SLIPS materials with high droplet mobility and droplet control on both faces. We also exemplify the importance of flexibility using a mesh-based SLIPS pipe capable of withstanding laminar and turbulent flows for 180 and 90 minutes, respectively. Finally, we discuss how ideas of topology introduced by the SLIPS mesh might be extended to create completely new types of SLIPS systems, such as Mobius strips and auxetic metamaterials. Nature Publishing Group UK 2019-09-16 /pmc/articles/PMC6746700/ /pubmed/31527694 http://dx.doi.org/10.1038/s41598-019-49887-3 Text en © The Author(s) 2019 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Geraldi, Nicasio R.
Guan, Jian H.
Dodd, Linzi E.
Maiello, Pietro
Xu, Ben B.
Wood, David
Newton, Michael I.
Wells, Gary G.
McHale, Glen
Double-sided slippery liquid-infused porous materials using conformable mesh
title Double-sided slippery liquid-infused porous materials using conformable mesh
title_full Double-sided slippery liquid-infused porous materials using conformable mesh
title_fullStr Double-sided slippery liquid-infused porous materials using conformable mesh
title_full_unstemmed Double-sided slippery liquid-infused porous materials using conformable mesh
title_short Double-sided slippery liquid-infused porous materials using conformable mesh
title_sort double-sided slippery liquid-infused porous materials using conformable mesh
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6746700/
https://www.ncbi.nlm.nih.gov/pubmed/31527694
http://dx.doi.org/10.1038/s41598-019-49887-3
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