Cargando…

Near-Field Manipulation in a Scanning Tunneling Microscope Junction with Plasmonic Fabry-Pérot Tips

[Image: see text] Near-field manipulation in plasmonic nanocavities can provide various applications in nanoscale science and technology. In particular, a gap plasmon in a scanning tunneling microscope (STM) junction is of key interest to nanoscale imaging and spectroscopy. Here we show that spectra...

Descripción completa

Detalles Bibliográficos
Autores principales: Böckmann, Hannes, Liu, Shuyi, Müller, Melanie, Hammud, Adnan, Wolf, Martin, Kumagai, Takashi
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2019
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6750903/
https://www.ncbi.nlm.nih.gov/pubmed/31070928
http://dx.doi.org/10.1021/acs.nanolett.9b00558
_version_ 1783452539812839424
author Böckmann, Hannes
Liu, Shuyi
Müller, Melanie
Hammud, Adnan
Wolf, Martin
Kumagai, Takashi
author_facet Böckmann, Hannes
Liu, Shuyi
Müller, Melanie
Hammud, Adnan
Wolf, Martin
Kumagai, Takashi
author_sort Böckmann, Hannes
collection PubMed
description [Image: see text] Near-field manipulation in plasmonic nanocavities can provide various applications in nanoscale science and technology. In particular, a gap plasmon in a scanning tunneling microscope (STM) junction is of key interest to nanoscale imaging and spectroscopy. Here we show that spectral features of a plasmonic STM junction can be manipulated by nanofabrication of Au tips using focused ion beam. An exemplary Fabry–Pérot type resonator of surface plasmons is demonstrated by producing the tip with a single groove on its shaft. Scanning tunneling luminescence spectra of the Fabry–Pérot tips exhibit spectral modulation resulting from interference between localized and propagating surface plasmon modes. In addition, the quality factor of the plasmonic Fabry–Pérot interference can be improved by optimizing the overall tip shape. Our approach paves the way for near-field imaging and spectroscopy with a high degree of accuracy.
format Online
Article
Text
id pubmed-6750903
institution National Center for Biotechnology Information
language English
publishDate 2019
publisher American Chemical Society
record_format MEDLINE/PubMed
spelling pubmed-67509032019-09-19 Near-Field Manipulation in a Scanning Tunneling Microscope Junction with Plasmonic Fabry-Pérot Tips Böckmann, Hannes Liu, Shuyi Müller, Melanie Hammud, Adnan Wolf, Martin Kumagai, Takashi Nano Lett [Image: see text] Near-field manipulation in plasmonic nanocavities can provide various applications in nanoscale science and technology. In particular, a gap plasmon in a scanning tunneling microscope (STM) junction is of key interest to nanoscale imaging and spectroscopy. Here we show that spectral features of a plasmonic STM junction can be manipulated by nanofabrication of Au tips using focused ion beam. An exemplary Fabry–Pérot type resonator of surface plasmons is demonstrated by producing the tip with a single groove on its shaft. Scanning tunneling luminescence spectra of the Fabry–Pérot tips exhibit spectral modulation resulting from interference between localized and propagating surface plasmon modes. In addition, the quality factor of the plasmonic Fabry–Pérot interference can be improved by optimizing the overall tip shape. Our approach paves the way for near-field imaging and spectroscopy with a high degree of accuracy. American Chemical Society 2019-05-09 2019-06-12 /pmc/articles/PMC6750903/ /pubmed/31070928 http://dx.doi.org/10.1021/acs.nanolett.9b00558 Text en Copyright © 2019 American Chemical Society This is an open access article published under a Creative Commons Attribution (CC-BY) License (http://pubs.acs.org/page/policy/authorchoice_ccby_termsofuse.html) , which permits unrestricted use, distribution and reproduction in any medium, provided the author and source are cited.
spellingShingle Böckmann, Hannes
Liu, Shuyi
Müller, Melanie
Hammud, Adnan
Wolf, Martin
Kumagai, Takashi
Near-Field Manipulation in a Scanning Tunneling Microscope Junction with Plasmonic Fabry-Pérot Tips
title Near-Field Manipulation in a Scanning Tunneling Microscope Junction with Plasmonic Fabry-Pérot Tips
title_full Near-Field Manipulation in a Scanning Tunneling Microscope Junction with Plasmonic Fabry-Pérot Tips
title_fullStr Near-Field Manipulation in a Scanning Tunneling Microscope Junction with Plasmonic Fabry-Pérot Tips
title_full_unstemmed Near-Field Manipulation in a Scanning Tunneling Microscope Junction with Plasmonic Fabry-Pérot Tips
title_short Near-Field Manipulation in a Scanning Tunneling Microscope Junction with Plasmonic Fabry-Pérot Tips
title_sort near-field manipulation in a scanning tunneling microscope junction with plasmonic fabry-pérot tips
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6750903/
https://www.ncbi.nlm.nih.gov/pubmed/31070928
http://dx.doi.org/10.1021/acs.nanolett.9b00558
work_keys_str_mv AT bockmannhannes nearfieldmanipulationinascanningtunnelingmicroscopejunctionwithplasmonicfabryperottips
AT liushuyi nearfieldmanipulationinascanningtunnelingmicroscopejunctionwithplasmonicfabryperottips
AT mullermelanie nearfieldmanipulationinascanningtunnelingmicroscopejunctionwithplasmonicfabryperottips
AT hammudadnan nearfieldmanipulationinascanningtunnelingmicroscopejunctionwithplasmonicfabryperottips
AT wolfmartin nearfieldmanipulationinascanningtunnelingmicroscopejunctionwithplasmonicfabryperottips
AT kumagaitakashi nearfieldmanipulationinascanningtunnelingmicroscopejunctionwithplasmonicfabryperottips