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Dynamic Enhancement of Nitric Oxide Radioluminescence with Nitrogen Purge

Remote detection of alpha radiation is commonly realised by collecting the light, the radioluminescence, that is produced when alpha particles are stopped in air. Radioluminescence of nitric oxide (NO) is primarily emitted between 200 nm and 300 nm, which makes it possible to use it for remote detec...

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Autores principales: Kerst, Thomas, Toivonen, Juha
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2019
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6761183/
https://www.ncbi.nlm.nih.gov/pubmed/31554918
http://dx.doi.org/10.1038/s41598-019-50396-6
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author Kerst, Thomas
Toivonen, Juha
author_facet Kerst, Thomas
Toivonen, Juha
author_sort Kerst, Thomas
collection PubMed
description Remote detection of alpha radiation is commonly realised by collecting the light, the radioluminescence, that is produced when alpha particles are stopped in air. Radioluminescence of nitric oxide (NO) is primarily emitted between 200 nm and 300 nm, which makes it possible to use it for remote detection under daylight conditions. Quenching by ambient oxygen and water vapour, however, makes it generally difficult to effectively create NO radioluminescence. We present the detection of intense NO radioluminescence in ambient air under standard indoor lighting conditions using a nitrogen purge. The nitrogen contained NO impurities that were intrinsic to the gas and had not explicitly been added. We study the mechanisms that govern the NO radioluminescence production and introduce a model to describe the dynamics of the process. The level of NO contained in the gas was found to determine how successful a purge can be. We conclude by discussing possible applications of the technique in nitrogen-flushed gloveboxes at nuclear facilities where NO concentration of 100 ppb–1 ppm would be sufficient for efficient optical alpha radiation detection in standard lighting conditions.
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spelling pubmed-67611832019-11-12 Dynamic Enhancement of Nitric Oxide Radioluminescence with Nitrogen Purge Kerst, Thomas Toivonen, Juha Sci Rep Article Remote detection of alpha radiation is commonly realised by collecting the light, the radioluminescence, that is produced when alpha particles are stopped in air. Radioluminescence of nitric oxide (NO) is primarily emitted between 200 nm and 300 nm, which makes it possible to use it for remote detection under daylight conditions. Quenching by ambient oxygen and water vapour, however, makes it generally difficult to effectively create NO radioluminescence. We present the detection of intense NO radioluminescence in ambient air under standard indoor lighting conditions using a nitrogen purge. The nitrogen contained NO impurities that were intrinsic to the gas and had not explicitly been added. We study the mechanisms that govern the NO radioluminescence production and introduce a model to describe the dynamics of the process. The level of NO contained in the gas was found to determine how successful a purge can be. We conclude by discussing possible applications of the technique in nitrogen-flushed gloveboxes at nuclear facilities where NO concentration of 100 ppb–1 ppm would be sufficient for efficient optical alpha radiation detection in standard lighting conditions. Nature Publishing Group UK 2019-09-25 /pmc/articles/PMC6761183/ /pubmed/31554918 http://dx.doi.org/10.1038/s41598-019-50396-6 Text en © The Author(s) 2019 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Kerst, Thomas
Toivonen, Juha
Dynamic Enhancement of Nitric Oxide Radioluminescence with Nitrogen Purge
title Dynamic Enhancement of Nitric Oxide Radioluminescence with Nitrogen Purge
title_full Dynamic Enhancement of Nitric Oxide Radioluminescence with Nitrogen Purge
title_fullStr Dynamic Enhancement of Nitric Oxide Radioluminescence with Nitrogen Purge
title_full_unstemmed Dynamic Enhancement of Nitric Oxide Radioluminescence with Nitrogen Purge
title_short Dynamic Enhancement of Nitric Oxide Radioluminescence with Nitrogen Purge
title_sort dynamic enhancement of nitric oxide radioluminescence with nitrogen purge
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6761183/
https://www.ncbi.nlm.nih.gov/pubmed/31554918
http://dx.doi.org/10.1038/s41598-019-50396-6
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