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Photoenhanced metastable c-axis electrodynamics in stripe-ordered cuprate La(1.885)Ba(0.115)CuO(4)

Quantum materials are amenable to nonequilibrium manipulation with light, enabling modification and control of macroscopic properties. Light-based augmentation of superconductivity is particularly intriguing. Copper-oxide superconductors exhibit complex interplay between spin order, charge order, an...

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Autores principales: Cremin, Kevin A., Zhang, Jingdi, Homes, Christopher C., Gu, G. D., Sun, Zhiyuan, Fogler, Michael M., Millis, Andrew J., Basov, D. N., Averitt, Richard D.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: National Academy of Sciences 2019
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6778182/
https://www.ncbi.nlm.nih.gov/pubmed/31527271
http://dx.doi.org/10.1073/pnas.1908368116
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author Cremin, Kevin A.
Zhang, Jingdi
Homes, Christopher C.
Gu, G. D.
Sun, Zhiyuan
Fogler, Michael M.
Millis, Andrew J.
Basov, D. N.
Averitt, Richard D.
author_facet Cremin, Kevin A.
Zhang, Jingdi
Homes, Christopher C.
Gu, G. D.
Sun, Zhiyuan
Fogler, Michael M.
Millis, Andrew J.
Basov, D. N.
Averitt, Richard D.
author_sort Cremin, Kevin A.
collection PubMed
description Quantum materials are amenable to nonequilibrium manipulation with light, enabling modification and control of macroscopic properties. Light-based augmentation of superconductivity is particularly intriguing. Copper-oxide superconductors exhibit complex interplay between spin order, charge order, and superconductivity, offering the prospect of enhanced coherence by altering the balance between competing orders. We utilize terahertz time-domain spectroscopy to monitor the c-axis Josephson plasma resonance (JPR) in La(2−x)Ba(x)CuO(4) (x = 0.115) as a direct probe of superconductivity dynamics following excitation with near-infrared pulses. Starting from the superconducting state, c-axis polarized excitation with a fluence of 100 μJ/cm(2) results in an increase of the far-infrared spectral weight by more than an order of magnitude as evidenced by a blueshift of the JPR, interpreted as resulting from nonthermal collapse of the charge order. The photoinduced signal persists well beyond our measurement window of 300 ps and exhibits signatures of spatial inhomogeneity. The electrodynamic response of this metastable state is consistent with enhanced superconducting fluctuations. Our results reveal that La(2−x)Ba(x)CuO(4) is highly sensitive to nonequilibrium excitation over a wide fluence range, providing an unambiguous example of photoinduced modification of order-parameter competition.
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spelling pubmed-67781822019-10-09 Photoenhanced metastable c-axis electrodynamics in stripe-ordered cuprate La(1.885)Ba(0.115)CuO(4) Cremin, Kevin A. Zhang, Jingdi Homes, Christopher C. Gu, G. D. Sun, Zhiyuan Fogler, Michael M. Millis, Andrew J. Basov, D. N. Averitt, Richard D. Proc Natl Acad Sci U S A Physical Sciences Quantum materials are amenable to nonequilibrium manipulation with light, enabling modification and control of macroscopic properties. Light-based augmentation of superconductivity is particularly intriguing. Copper-oxide superconductors exhibit complex interplay between spin order, charge order, and superconductivity, offering the prospect of enhanced coherence by altering the balance between competing orders. We utilize terahertz time-domain spectroscopy to monitor the c-axis Josephson plasma resonance (JPR) in La(2−x)Ba(x)CuO(4) (x = 0.115) as a direct probe of superconductivity dynamics following excitation with near-infrared pulses. Starting from the superconducting state, c-axis polarized excitation with a fluence of 100 μJ/cm(2) results in an increase of the far-infrared spectral weight by more than an order of magnitude as evidenced by a blueshift of the JPR, interpreted as resulting from nonthermal collapse of the charge order. The photoinduced signal persists well beyond our measurement window of 300 ps and exhibits signatures of spatial inhomogeneity. The electrodynamic response of this metastable state is consistent with enhanced superconducting fluctuations. Our results reveal that La(2−x)Ba(x)CuO(4) is highly sensitive to nonequilibrium excitation over a wide fluence range, providing an unambiguous example of photoinduced modification of order-parameter competition. National Academy of Sciences 2019-10-01 2019-09-16 /pmc/articles/PMC6778182/ /pubmed/31527271 http://dx.doi.org/10.1073/pnas.1908368116 Text en Copyright © 2019 the Author(s). Published by PNAS. https://creativecommons.org/licenses/by-nc-nd/4.0/ https://creativecommons.org/licenses/by-nc-nd/4.0/This open access article is distributed under Creative Commons Attribution-NonCommercial-NoDerivatives License 4.0 (CC BY-NC-ND) (https://creativecommons.org/licenses/by-nc-nd/4.0/) .
spellingShingle Physical Sciences
Cremin, Kevin A.
Zhang, Jingdi
Homes, Christopher C.
Gu, G. D.
Sun, Zhiyuan
Fogler, Michael M.
Millis, Andrew J.
Basov, D. N.
Averitt, Richard D.
Photoenhanced metastable c-axis electrodynamics in stripe-ordered cuprate La(1.885)Ba(0.115)CuO(4)
title Photoenhanced metastable c-axis electrodynamics in stripe-ordered cuprate La(1.885)Ba(0.115)CuO(4)
title_full Photoenhanced metastable c-axis electrodynamics in stripe-ordered cuprate La(1.885)Ba(0.115)CuO(4)
title_fullStr Photoenhanced metastable c-axis electrodynamics in stripe-ordered cuprate La(1.885)Ba(0.115)CuO(4)
title_full_unstemmed Photoenhanced metastable c-axis electrodynamics in stripe-ordered cuprate La(1.885)Ba(0.115)CuO(4)
title_short Photoenhanced metastable c-axis electrodynamics in stripe-ordered cuprate La(1.885)Ba(0.115)CuO(4)
title_sort photoenhanced metastable c-axis electrodynamics in stripe-ordered cuprate la(1.885)ba(0.115)cuo(4)
topic Physical Sciences
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6778182/
https://www.ncbi.nlm.nih.gov/pubmed/31527271
http://dx.doi.org/10.1073/pnas.1908368116
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