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The role of transition dipole phase in atomic attosecond transient absorption from the multi-level model

Based on a multilevel model considering enough bound electronic states of atoms, we theoretically study the role of the transition dipole phase (TDP) in the attosecond transient absorption (ATA) spectrum of helium in intense laser fields. By solving the stationary Schrödinger equation with B-spline...

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Autores principales: Yuan, Guanglu, Jiang, Shicheng, Wang, Ziwen, Hua, Weijie, Yu, Chao, Jin, Cheng, Lu, Ruifeng
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Crystallographic Association 2019
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6796354/
https://www.ncbi.nlm.nih.gov/pubmed/31649962
http://dx.doi.org/10.1063/1.5124441
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author Yuan, Guanglu
Jiang, Shicheng
Wang, Ziwen
Hua, Weijie
Yu, Chao
Jin, Cheng
Lu, Ruifeng
author_facet Yuan, Guanglu
Jiang, Shicheng
Wang, Ziwen
Hua, Weijie
Yu, Chao
Jin, Cheng
Lu, Ruifeng
author_sort Yuan, Guanglu
collection PubMed
description Based on a multilevel model considering enough bound electronic states of atoms, we theoretically study the role of the transition dipole phase (TDP) in the attosecond transient absorption (ATA) spectrum of helium in intense laser fields. By solving the stationary Schrödinger equation with B-spline basis sets, we first calculate the transition dipole moments with well-defined phases between the bound states. Using the modified multilevel model, we reveal that the TDP plays an important role in determining the spectral structures if two or more paths populate the excited states from the ground state. Our multilevel model with the accurate TDP is convenient to address the origin of atomic ATA spectral structures by freely removing or adding specific electronic states and has been justified by comparing with the ATA spectra via directly solving the time-dependent Schrödinger equation. Hopefully, further incorporating macroscopic propagation into the model will provide indepth physical insights into experimental ATA spectra.
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spelling pubmed-67963542019-10-24 The role of transition dipole phase in atomic attosecond transient absorption from the multi-level model Yuan, Guanglu Jiang, Shicheng Wang, Ziwen Hua, Weijie Yu, Chao Jin, Cheng Lu, Ruifeng Struct Dyn ARTICLES Based on a multilevel model considering enough bound electronic states of atoms, we theoretically study the role of the transition dipole phase (TDP) in the attosecond transient absorption (ATA) spectrum of helium in intense laser fields. By solving the stationary Schrödinger equation with B-spline basis sets, we first calculate the transition dipole moments with well-defined phases between the bound states. Using the modified multilevel model, we reveal that the TDP plays an important role in determining the spectral structures if two or more paths populate the excited states from the ground state. Our multilevel model with the accurate TDP is convenient to address the origin of atomic ATA spectral structures by freely removing or adding specific electronic states and has been justified by comparing with the ATA spectra via directly solving the time-dependent Schrödinger equation. Hopefully, further incorporating macroscopic propagation into the model will provide indepth physical insights into experimental ATA spectra. American Crystallographic Association 2019-10-15 /pmc/articles/PMC6796354/ /pubmed/31649962 http://dx.doi.org/10.1063/1.5124441 Text en © 2019 Author(s). 2329-7778/2019/6(5)/054102/8 All article content, except where otherwise noted, is licensed under a Creative Commons Attribution (CC BY) license (http://creativecommons.org/licenses/by/4.0/).
spellingShingle ARTICLES
Yuan, Guanglu
Jiang, Shicheng
Wang, Ziwen
Hua, Weijie
Yu, Chao
Jin, Cheng
Lu, Ruifeng
The role of transition dipole phase in atomic attosecond transient absorption from the multi-level model
title The role of transition dipole phase in atomic attosecond transient absorption from the multi-level model
title_full The role of transition dipole phase in atomic attosecond transient absorption from the multi-level model
title_fullStr The role of transition dipole phase in atomic attosecond transient absorption from the multi-level model
title_full_unstemmed The role of transition dipole phase in atomic attosecond transient absorption from the multi-level model
title_short The role of transition dipole phase in atomic attosecond transient absorption from the multi-level model
title_sort role of transition dipole phase in atomic attosecond transient absorption from the multi-level model
topic ARTICLES
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6796354/
https://www.ncbi.nlm.nih.gov/pubmed/31649962
http://dx.doi.org/10.1063/1.5124441
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