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Orbital-selective Kondo lattice and enigmatic f electrons emerging from inside the antiferromagnetic phase of a heavy fermion
Novel electronic phenomena frequently form in heavy-fermions because of the mutual localized and itinerant nature of f-electrons. On the magnetically ordered side of the heavy-fermion phase diagram, f-moments are expected to be localized and decoupled from the Fermi surface. It remains ambiguous whe...
Autores principales: | , , , , , , , , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American Association for the Advancement of Science
2019
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6799987/ https://www.ncbi.nlm.nih.gov/pubmed/31667341 http://dx.doi.org/10.1126/sciadv.aaw9061 |
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author | Giannakis, Ioannis Leshen, Justin Kavai, Mariam Ran, Sheng Kang, Chang-Jong Saha, Shanta R. Zhao, Y. Xu, Z. Lynn, J. W. Miao, Lin Wray, L. Andrew Kotliar, Gabriel Butch, Nicholas P. Aynajian, Pegor |
author_facet | Giannakis, Ioannis Leshen, Justin Kavai, Mariam Ran, Sheng Kang, Chang-Jong Saha, Shanta R. Zhao, Y. Xu, Z. Lynn, J. W. Miao, Lin Wray, L. Andrew Kotliar, Gabriel Butch, Nicholas P. Aynajian, Pegor |
author_sort | Giannakis, Ioannis |
collection | PubMed |
description | Novel electronic phenomena frequently form in heavy-fermions because of the mutual localized and itinerant nature of f-electrons. On the magnetically ordered side of the heavy-fermion phase diagram, f-moments are expected to be localized and decoupled from the Fermi surface. It remains ambiguous whether Kondo lattice can develop inside the magnetically ordered phase. Using spectroscopic imaging with scanning tunneling microscope, complemented by neutron scattering, x-ray absorption spectroscopy, and dynamical mean field theory, we probe the electronic states in antiferromagnetic USb(2). We visualize a large gap in the antiferromagnetic phase within which Kondo hybridization develops below ~80 K. Our calculations indicate the antiferromagnetism and Kondo lattice to reside predominantly on different f-orbitals, promoting orbital selectivity as a new conception into how these phenomena coexist in heavy-fermions. Finally, at 45 K, we find a novel first order–like transition through abrupt emergence of nontrivial 5f-electronic states that may resemble the “hidden-order” phase of URu(2)Si(2). |
format | Online Article Text |
id | pubmed-6799987 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2019 |
publisher | American Association for the Advancement of Science |
record_format | MEDLINE/PubMed |
spelling | pubmed-67999872019-10-30 Orbital-selective Kondo lattice and enigmatic f electrons emerging from inside the antiferromagnetic phase of a heavy fermion Giannakis, Ioannis Leshen, Justin Kavai, Mariam Ran, Sheng Kang, Chang-Jong Saha, Shanta R. Zhao, Y. Xu, Z. Lynn, J. W. Miao, Lin Wray, L. Andrew Kotliar, Gabriel Butch, Nicholas P. Aynajian, Pegor Sci Adv Research Articles Novel electronic phenomena frequently form in heavy-fermions because of the mutual localized and itinerant nature of f-electrons. On the magnetically ordered side of the heavy-fermion phase diagram, f-moments are expected to be localized and decoupled from the Fermi surface. It remains ambiguous whether Kondo lattice can develop inside the magnetically ordered phase. Using spectroscopic imaging with scanning tunneling microscope, complemented by neutron scattering, x-ray absorption spectroscopy, and dynamical mean field theory, we probe the electronic states in antiferromagnetic USb(2). We visualize a large gap in the antiferromagnetic phase within which Kondo hybridization develops below ~80 K. Our calculations indicate the antiferromagnetism and Kondo lattice to reside predominantly on different f-orbitals, promoting orbital selectivity as a new conception into how these phenomena coexist in heavy-fermions. Finally, at 45 K, we find a novel first order–like transition through abrupt emergence of nontrivial 5f-electronic states that may resemble the “hidden-order” phase of URu(2)Si(2). American Association for the Advancement of Science 2019-10-18 /pmc/articles/PMC6799987/ /pubmed/31667341 http://dx.doi.org/10.1126/sciadv.aaw9061 Text en Copyright © 2019 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution NonCommercial License 4.0 (CC BY-NC). http://creativecommons.org/licenses/by-nc/4.0/ This is an open-access article distributed under the terms of the Creative Commons Attribution-NonCommercial license (http://creativecommons.org/licenses/by-nc/4.0/) , which permits use, distribution, and reproduction in any medium, so long as the resultant use is not for commercial advantage and provided the original work is properly cited. |
spellingShingle | Research Articles Giannakis, Ioannis Leshen, Justin Kavai, Mariam Ran, Sheng Kang, Chang-Jong Saha, Shanta R. Zhao, Y. Xu, Z. Lynn, J. W. Miao, Lin Wray, L. Andrew Kotliar, Gabriel Butch, Nicholas P. Aynajian, Pegor Orbital-selective Kondo lattice and enigmatic f electrons emerging from inside the antiferromagnetic phase of a heavy fermion |
title | Orbital-selective Kondo lattice and enigmatic f electrons emerging from inside the antiferromagnetic phase of a heavy fermion |
title_full | Orbital-selective Kondo lattice and enigmatic f electrons emerging from inside the antiferromagnetic phase of a heavy fermion |
title_fullStr | Orbital-selective Kondo lattice and enigmatic f electrons emerging from inside the antiferromagnetic phase of a heavy fermion |
title_full_unstemmed | Orbital-selective Kondo lattice and enigmatic f electrons emerging from inside the antiferromagnetic phase of a heavy fermion |
title_short | Orbital-selective Kondo lattice and enigmatic f electrons emerging from inside the antiferromagnetic phase of a heavy fermion |
title_sort | orbital-selective kondo lattice and enigmatic f electrons emerging from inside the antiferromagnetic phase of a heavy fermion |
topic | Research Articles |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6799987/ https://www.ncbi.nlm.nih.gov/pubmed/31667341 http://dx.doi.org/10.1126/sciadv.aaw9061 |
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