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Orbital-selective Kondo lattice and enigmatic f electrons emerging from inside the antiferromagnetic phase of a heavy fermion

Novel electronic phenomena frequently form in heavy-fermions because of the mutual localized and itinerant nature of f-electrons. On the magnetically ordered side of the heavy-fermion phase diagram, f-moments are expected to be localized and decoupled from the Fermi surface. It remains ambiguous whe...

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Autores principales: Giannakis, Ioannis, Leshen, Justin, Kavai, Mariam, Ran, Sheng, Kang, Chang-Jong, Saha, Shanta R., Zhao, Y., Xu, Z., Lynn, J. W., Miao, Lin, Wray, L. Andrew, Kotliar, Gabriel, Butch, Nicholas P., Aynajian, Pegor
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Association for the Advancement of Science 2019
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6799987/
https://www.ncbi.nlm.nih.gov/pubmed/31667341
http://dx.doi.org/10.1126/sciadv.aaw9061
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author Giannakis, Ioannis
Leshen, Justin
Kavai, Mariam
Ran, Sheng
Kang, Chang-Jong
Saha, Shanta R.
Zhao, Y.
Xu, Z.
Lynn, J. W.
Miao, Lin
Wray, L. Andrew
Kotliar, Gabriel
Butch, Nicholas P.
Aynajian, Pegor
author_facet Giannakis, Ioannis
Leshen, Justin
Kavai, Mariam
Ran, Sheng
Kang, Chang-Jong
Saha, Shanta R.
Zhao, Y.
Xu, Z.
Lynn, J. W.
Miao, Lin
Wray, L. Andrew
Kotliar, Gabriel
Butch, Nicholas P.
Aynajian, Pegor
author_sort Giannakis, Ioannis
collection PubMed
description Novel electronic phenomena frequently form in heavy-fermions because of the mutual localized and itinerant nature of f-electrons. On the magnetically ordered side of the heavy-fermion phase diagram, f-moments are expected to be localized and decoupled from the Fermi surface. It remains ambiguous whether Kondo lattice can develop inside the magnetically ordered phase. Using spectroscopic imaging with scanning tunneling microscope, complemented by neutron scattering, x-ray absorption spectroscopy, and dynamical mean field theory, we probe the electronic states in antiferromagnetic USb(2). We visualize a large gap in the antiferromagnetic phase within which Kondo hybridization develops below ~80 K. Our calculations indicate the antiferromagnetism and Kondo lattice to reside predominantly on different f-orbitals, promoting orbital selectivity as a new conception into how these phenomena coexist in heavy-fermions. Finally, at 45 K, we find a novel first order–like transition through abrupt emergence of nontrivial 5f-electronic states that may resemble the “hidden-order” phase of URu(2)Si(2).
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spelling pubmed-67999872019-10-30 Orbital-selective Kondo lattice and enigmatic f electrons emerging from inside the antiferromagnetic phase of a heavy fermion Giannakis, Ioannis Leshen, Justin Kavai, Mariam Ran, Sheng Kang, Chang-Jong Saha, Shanta R. Zhao, Y. Xu, Z. Lynn, J. W. Miao, Lin Wray, L. Andrew Kotliar, Gabriel Butch, Nicholas P. Aynajian, Pegor Sci Adv Research Articles Novel electronic phenomena frequently form in heavy-fermions because of the mutual localized and itinerant nature of f-electrons. On the magnetically ordered side of the heavy-fermion phase diagram, f-moments are expected to be localized and decoupled from the Fermi surface. It remains ambiguous whether Kondo lattice can develop inside the magnetically ordered phase. Using spectroscopic imaging with scanning tunneling microscope, complemented by neutron scattering, x-ray absorption spectroscopy, and dynamical mean field theory, we probe the electronic states in antiferromagnetic USb(2). We visualize a large gap in the antiferromagnetic phase within which Kondo hybridization develops below ~80 K. Our calculations indicate the antiferromagnetism and Kondo lattice to reside predominantly on different f-orbitals, promoting orbital selectivity as a new conception into how these phenomena coexist in heavy-fermions. Finally, at 45 K, we find a novel first order–like transition through abrupt emergence of nontrivial 5f-electronic states that may resemble the “hidden-order” phase of URu(2)Si(2). American Association for the Advancement of Science 2019-10-18 /pmc/articles/PMC6799987/ /pubmed/31667341 http://dx.doi.org/10.1126/sciadv.aaw9061 Text en Copyright © 2019 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution NonCommercial License 4.0 (CC BY-NC). http://creativecommons.org/licenses/by-nc/4.0/ This is an open-access article distributed under the terms of the Creative Commons Attribution-NonCommercial license (http://creativecommons.org/licenses/by-nc/4.0/) , which permits use, distribution, and reproduction in any medium, so long as the resultant use is not for commercial advantage and provided the original work is properly cited.
spellingShingle Research Articles
Giannakis, Ioannis
Leshen, Justin
Kavai, Mariam
Ran, Sheng
Kang, Chang-Jong
Saha, Shanta R.
Zhao, Y.
Xu, Z.
Lynn, J. W.
Miao, Lin
Wray, L. Andrew
Kotliar, Gabriel
Butch, Nicholas P.
Aynajian, Pegor
Orbital-selective Kondo lattice and enigmatic f electrons emerging from inside the antiferromagnetic phase of a heavy fermion
title Orbital-selective Kondo lattice and enigmatic f electrons emerging from inside the antiferromagnetic phase of a heavy fermion
title_full Orbital-selective Kondo lattice and enigmatic f electrons emerging from inside the antiferromagnetic phase of a heavy fermion
title_fullStr Orbital-selective Kondo lattice and enigmatic f electrons emerging from inside the antiferromagnetic phase of a heavy fermion
title_full_unstemmed Orbital-selective Kondo lattice and enigmatic f electrons emerging from inside the antiferromagnetic phase of a heavy fermion
title_short Orbital-selective Kondo lattice and enigmatic f electrons emerging from inside the antiferromagnetic phase of a heavy fermion
title_sort orbital-selective kondo lattice and enigmatic f electrons emerging from inside the antiferromagnetic phase of a heavy fermion
topic Research Articles
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6799987/
https://www.ncbi.nlm.nih.gov/pubmed/31667341
http://dx.doi.org/10.1126/sciadv.aaw9061
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