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A hybrid organic–inorganic polariton LED

Polaritons are quasi-particles composed of a superposition of excitons and photons that can be created within a strongly coupled optical microcavity. Here, we describe a structure in which a strongly coupled microcavity containing an organic semiconductor is coupled to a second microcavity containin...

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Autores principales: Jayaprakash, Rahul, Georgiou, Kyriacos, Coulthard, Harriet, Askitopoulos, Alexis, Rajendran, Sai K., Coles, David M., Musser, Andrew J., Clark, Jenny, Samuel, Ifor D. W., Turnbull, Graham A., Lagoudakis, Pavlos G., Lidzey, David G.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2019
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6804868/
https://www.ncbi.nlm.nih.gov/pubmed/31666947
http://dx.doi.org/10.1038/s41377-019-0180-8
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author Jayaprakash, Rahul
Georgiou, Kyriacos
Coulthard, Harriet
Askitopoulos, Alexis
Rajendran, Sai K.
Coles, David M.
Musser, Andrew J.
Clark, Jenny
Samuel, Ifor D. W.
Turnbull, Graham A.
Lagoudakis, Pavlos G.
Lidzey, David G.
author_facet Jayaprakash, Rahul
Georgiou, Kyriacos
Coulthard, Harriet
Askitopoulos, Alexis
Rajendran, Sai K.
Coles, David M.
Musser, Andrew J.
Clark, Jenny
Samuel, Ifor D. W.
Turnbull, Graham A.
Lagoudakis, Pavlos G.
Lidzey, David G.
author_sort Jayaprakash, Rahul
collection PubMed
description Polaritons are quasi-particles composed of a superposition of excitons and photons that can be created within a strongly coupled optical microcavity. Here, we describe a structure in which a strongly coupled microcavity containing an organic semiconductor is coupled to a second microcavity containing a series of weakly coupled inorganic quantum wells. We show that optical hybridisation occurs between the optical modes of the two cavities, creating a delocalised polaritonic state. By electrically injecting electron–hole pairs into the inorganic quantum-well system, we are able to transfer energy between the cavities and populate organic-exciton polaritons. Our approach represents a new strategy to create highly efficient devices for emerging ‘polaritonic’ technologies.
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spelling pubmed-68048682019-10-30 A hybrid organic–inorganic polariton LED Jayaprakash, Rahul Georgiou, Kyriacos Coulthard, Harriet Askitopoulos, Alexis Rajendran, Sai K. Coles, David M. Musser, Andrew J. Clark, Jenny Samuel, Ifor D. W. Turnbull, Graham A. Lagoudakis, Pavlos G. Lidzey, David G. Light Sci Appl Article Polaritons are quasi-particles composed of a superposition of excitons and photons that can be created within a strongly coupled optical microcavity. Here, we describe a structure in which a strongly coupled microcavity containing an organic semiconductor is coupled to a second microcavity containing a series of weakly coupled inorganic quantum wells. We show that optical hybridisation occurs between the optical modes of the two cavities, creating a delocalised polaritonic state. By electrically injecting electron–hole pairs into the inorganic quantum-well system, we are able to transfer energy between the cavities and populate organic-exciton polaritons. Our approach represents a new strategy to create highly efficient devices for emerging ‘polaritonic’ technologies. Nature Publishing Group UK 2019-09-04 /pmc/articles/PMC6804868/ /pubmed/31666947 http://dx.doi.org/10.1038/s41377-019-0180-8 Text en © The Author(s) 2019 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Jayaprakash, Rahul
Georgiou, Kyriacos
Coulthard, Harriet
Askitopoulos, Alexis
Rajendran, Sai K.
Coles, David M.
Musser, Andrew J.
Clark, Jenny
Samuel, Ifor D. W.
Turnbull, Graham A.
Lagoudakis, Pavlos G.
Lidzey, David G.
A hybrid organic–inorganic polariton LED
title A hybrid organic–inorganic polariton LED
title_full A hybrid organic–inorganic polariton LED
title_fullStr A hybrid organic–inorganic polariton LED
title_full_unstemmed A hybrid organic–inorganic polariton LED
title_short A hybrid organic–inorganic polariton LED
title_sort hybrid organic–inorganic polariton led
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6804868/
https://www.ncbi.nlm.nih.gov/pubmed/31666947
http://dx.doi.org/10.1038/s41377-019-0180-8
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