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Pinpointing nitrogen oxide emissions from space

Satellite observations of nitrogen dioxide (NO(2)) provide valuable information on the location and strength of NO(x) emissions, but spatial resolution is limited by horizontal transport and smearing of temporal averages due to changing wind fields. In this study, we map NO(x) emissions on high spat...

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Detalles Bibliográficos
Autores principales: Beirle, Steffen, Borger, Christian, Dörner, Steffen, Li, Ang, Hu, Zhaokun, Liu, Fei, Wang, Yang, Wagner, Thomas
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Association for the Advancement of Science 2019
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6853767/
https://www.ncbi.nlm.nih.gov/pubmed/31763456
http://dx.doi.org/10.1126/sciadv.aax9800
Descripción
Sumario:Satellite observations of nitrogen dioxide (NO(2)) provide valuable information on the location and strength of NO(x) emissions, but spatial resolution is limited by horizontal transport and smearing of temporal averages due to changing wind fields. In this study, we map NO(x) emissions on high spatial resolution from TROPOMI observations of NO(2) combined with wind fields based on the continuity equation. The divergence of horizontal fluxes proves to be highly sensitive for point sources like exhaust stacks. Thus, NO(x) emissions from individual power plants can be resolved and quantified even on top of considerably high urban pollution from the Saudi Arabian capital city Riyadh. This allows us to catalog NO(x) emissions from large point sources globally, as demonstrated for South Africa and Germany, with a detection limit of about 0.11 kg/s down to 0.03 kg/s for ideal conditions.