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A skin-like two-dimensionally pixelized full-color quantum dot photodetector

Direct full-color photodetectors without sophisticated color filters and interferometric optics have attracted considerable attention for widespread applications. However, difficulties of combining various multispectral semiconductors and improving photon transfer efficiency for high-performance opt...

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Detalles Bibliográficos
Autores principales: Kim, Jaehyun, Kwon, Sung-Min, Kang, Yeo Kyung, Kim, Yong-Hoon, Lee, Myung-Jae, Han, Kwangjoon, Facchetti, Antonio, Kim, Myung-Gil, Park, Sung Kyu
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Association for the Advancement of Science 2019
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6874493/
https://www.ncbi.nlm.nih.gov/pubmed/31803836
http://dx.doi.org/10.1126/sciadv.aax8801
Descripción
Sumario:Direct full-color photodetectors without sophisticated color filters and interferometric optics have attracted considerable attention for widespread applications. However, difficulties of combining various multispectral semiconductors and improving photon transfer efficiency for high-performance optoelectronic devices have impeded the translation of these platforms into practical realization. Here, we report a low-temperature (<150°C) fabricated two-dimensionally pixelized full-color photodetector by using monolithic integration of various-sized colloidal quantum dots (QDs) and amorphous indium-gallium-zinc-oxide semiconductors. By introducing trap-reduced chelating chalcometallate ligands, highly efficient charge carrier transport and photoresistor-free fine-patterning of QD layers were successfully realized, exhibiting extremely high photodetectivity (>4.2 × 10(17) Jones) and photoresponsivity (>8.3 × 10(3) A W(−1)) in a broad range of wavelengths (365 to 1310 nm). On the basis of these technologies, a wavelength discriminable phototransistor circuit array (>600 phototransistors) was implemented on a skin-like soft platform, which is expected to be a versatile and scalable approach for wide spectral image sensors and human-oriented biological devices.