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A skin-like two-dimensionally pixelized full-color quantum dot photodetector

Direct full-color photodetectors without sophisticated color filters and interferometric optics have attracted considerable attention for widespread applications. However, difficulties of combining various multispectral semiconductors and improving photon transfer efficiency for high-performance opt...

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Autores principales: Kim, Jaehyun, Kwon, Sung-Min, Kang, Yeo Kyung, Kim, Yong-Hoon, Lee, Myung-Jae, Han, Kwangjoon, Facchetti, Antonio, Kim, Myung-Gil, Park, Sung Kyu
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Association for the Advancement of Science 2019
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6874493/
https://www.ncbi.nlm.nih.gov/pubmed/31803836
http://dx.doi.org/10.1126/sciadv.aax8801
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author Kim, Jaehyun
Kwon, Sung-Min
Kang, Yeo Kyung
Kim, Yong-Hoon
Lee, Myung-Jae
Han, Kwangjoon
Facchetti, Antonio
Kim, Myung-Gil
Park, Sung Kyu
author_facet Kim, Jaehyun
Kwon, Sung-Min
Kang, Yeo Kyung
Kim, Yong-Hoon
Lee, Myung-Jae
Han, Kwangjoon
Facchetti, Antonio
Kim, Myung-Gil
Park, Sung Kyu
author_sort Kim, Jaehyun
collection PubMed
description Direct full-color photodetectors without sophisticated color filters and interferometric optics have attracted considerable attention for widespread applications. However, difficulties of combining various multispectral semiconductors and improving photon transfer efficiency for high-performance optoelectronic devices have impeded the translation of these platforms into practical realization. Here, we report a low-temperature (<150°C) fabricated two-dimensionally pixelized full-color photodetector by using monolithic integration of various-sized colloidal quantum dots (QDs) and amorphous indium-gallium-zinc-oxide semiconductors. By introducing trap-reduced chelating chalcometallate ligands, highly efficient charge carrier transport and photoresistor-free fine-patterning of QD layers were successfully realized, exhibiting extremely high photodetectivity (>4.2 × 10(17) Jones) and photoresponsivity (>8.3 × 10(3) A W(−1)) in a broad range of wavelengths (365 to 1310 nm). On the basis of these technologies, a wavelength discriminable phototransistor circuit array (>600 phototransistors) was implemented on a skin-like soft platform, which is expected to be a versatile and scalable approach for wide spectral image sensors and human-oriented biological devices.
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spelling pubmed-68744932019-12-04 A skin-like two-dimensionally pixelized full-color quantum dot photodetector Kim, Jaehyun Kwon, Sung-Min Kang, Yeo Kyung Kim, Yong-Hoon Lee, Myung-Jae Han, Kwangjoon Facchetti, Antonio Kim, Myung-Gil Park, Sung Kyu Sci Adv Research Articles Direct full-color photodetectors without sophisticated color filters and interferometric optics have attracted considerable attention for widespread applications. However, difficulties of combining various multispectral semiconductors and improving photon transfer efficiency for high-performance optoelectronic devices have impeded the translation of these platforms into practical realization. Here, we report a low-temperature (<150°C) fabricated two-dimensionally pixelized full-color photodetector by using monolithic integration of various-sized colloidal quantum dots (QDs) and amorphous indium-gallium-zinc-oxide semiconductors. By introducing trap-reduced chelating chalcometallate ligands, highly efficient charge carrier transport and photoresistor-free fine-patterning of QD layers were successfully realized, exhibiting extremely high photodetectivity (>4.2 × 10(17) Jones) and photoresponsivity (>8.3 × 10(3) A W(−1)) in a broad range of wavelengths (365 to 1310 nm). On the basis of these technologies, a wavelength discriminable phototransistor circuit array (>600 phototransistors) was implemented on a skin-like soft platform, which is expected to be a versatile and scalable approach for wide spectral image sensors and human-oriented biological devices. American Association for the Advancement of Science 2019-11-22 /pmc/articles/PMC6874493/ /pubmed/31803836 http://dx.doi.org/10.1126/sciadv.aax8801 Text en Copyright © 2019 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution NonCommercial License 4.0 (CC BY-NC). http://creativecommons.org/licenses/by-nc/4.0/ This is an open-access article distributed under the terms of the Creative Commons Attribution-NonCommercial license (http://creativecommons.org/licenses/by-nc/4.0/) , which permits use, distribution, and reproduction in any medium, so long as the resultant use is not for commercial advantage and provided the original work is properly cited.
spellingShingle Research Articles
Kim, Jaehyun
Kwon, Sung-Min
Kang, Yeo Kyung
Kim, Yong-Hoon
Lee, Myung-Jae
Han, Kwangjoon
Facchetti, Antonio
Kim, Myung-Gil
Park, Sung Kyu
A skin-like two-dimensionally pixelized full-color quantum dot photodetector
title A skin-like two-dimensionally pixelized full-color quantum dot photodetector
title_full A skin-like two-dimensionally pixelized full-color quantum dot photodetector
title_fullStr A skin-like two-dimensionally pixelized full-color quantum dot photodetector
title_full_unstemmed A skin-like two-dimensionally pixelized full-color quantum dot photodetector
title_short A skin-like two-dimensionally pixelized full-color quantum dot photodetector
title_sort skin-like two-dimensionally pixelized full-color quantum dot photodetector
topic Research Articles
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6874493/
https://www.ncbi.nlm.nih.gov/pubmed/31803836
http://dx.doi.org/10.1126/sciadv.aax8801
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