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A skin-like two-dimensionally pixelized full-color quantum dot photodetector
Direct full-color photodetectors without sophisticated color filters and interferometric optics have attracted considerable attention for widespread applications. However, difficulties of combining various multispectral semiconductors and improving photon transfer efficiency for high-performance opt...
Autores principales: | , , , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American Association for the Advancement of Science
2019
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6874493/ https://www.ncbi.nlm.nih.gov/pubmed/31803836 http://dx.doi.org/10.1126/sciadv.aax8801 |
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author | Kim, Jaehyun Kwon, Sung-Min Kang, Yeo Kyung Kim, Yong-Hoon Lee, Myung-Jae Han, Kwangjoon Facchetti, Antonio Kim, Myung-Gil Park, Sung Kyu |
author_facet | Kim, Jaehyun Kwon, Sung-Min Kang, Yeo Kyung Kim, Yong-Hoon Lee, Myung-Jae Han, Kwangjoon Facchetti, Antonio Kim, Myung-Gil Park, Sung Kyu |
author_sort | Kim, Jaehyun |
collection | PubMed |
description | Direct full-color photodetectors without sophisticated color filters and interferometric optics have attracted considerable attention for widespread applications. However, difficulties of combining various multispectral semiconductors and improving photon transfer efficiency for high-performance optoelectronic devices have impeded the translation of these platforms into practical realization. Here, we report a low-temperature (<150°C) fabricated two-dimensionally pixelized full-color photodetector by using monolithic integration of various-sized colloidal quantum dots (QDs) and amorphous indium-gallium-zinc-oxide semiconductors. By introducing trap-reduced chelating chalcometallate ligands, highly efficient charge carrier transport and photoresistor-free fine-patterning of QD layers were successfully realized, exhibiting extremely high photodetectivity (>4.2 × 10(17) Jones) and photoresponsivity (>8.3 × 10(3) A W(−1)) in a broad range of wavelengths (365 to 1310 nm). On the basis of these technologies, a wavelength discriminable phototransistor circuit array (>600 phototransistors) was implemented on a skin-like soft platform, which is expected to be a versatile and scalable approach for wide spectral image sensors and human-oriented biological devices. |
format | Online Article Text |
id | pubmed-6874493 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2019 |
publisher | American Association for the Advancement of Science |
record_format | MEDLINE/PubMed |
spelling | pubmed-68744932019-12-04 A skin-like two-dimensionally pixelized full-color quantum dot photodetector Kim, Jaehyun Kwon, Sung-Min Kang, Yeo Kyung Kim, Yong-Hoon Lee, Myung-Jae Han, Kwangjoon Facchetti, Antonio Kim, Myung-Gil Park, Sung Kyu Sci Adv Research Articles Direct full-color photodetectors without sophisticated color filters and interferometric optics have attracted considerable attention for widespread applications. However, difficulties of combining various multispectral semiconductors and improving photon transfer efficiency for high-performance optoelectronic devices have impeded the translation of these platforms into practical realization. Here, we report a low-temperature (<150°C) fabricated two-dimensionally pixelized full-color photodetector by using monolithic integration of various-sized colloidal quantum dots (QDs) and amorphous indium-gallium-zinc-oxide semiconductors. By introducing trap-reduced chelating chalcometallate ligands, highly efficient charge carrier transport and photoresistor-free fine-patterning of QD layers were successfully realized, exhibiting extremely high photodetectivity (>4.2 × 10(17) Jones) and photoresponsivity (>8.3 × 10(3) A W(−1)) in a broad range of wavelengths (365 to 1310 nm). On the basis of these technologies, a wavelength discriminable phototransistor circuit array (>600 phototransistors) was implemented on a skin-like soft platform, which is expected to be a versatile and scalable approach for wide spectral image sensors and human-oriented biological devices. American Association for the Advancement of Science 2019-11-22 /pmc/articles/PMC6874493/ /pubmed/31803836 http://dx.doi.org/10.1126/sciadv.aax8801 Text en Copyright © 2019 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution NonCommercial License 4.0 (CC BY-NC). http://creativecommons.org/licenses/by-nc/4.0/ This is an open-access article distributed under the terms of the Creative Commons Attribution-NonCommercial license (http://creativecommons.org/licenses/by-nc/4.0/) , which permits use, distribution, and reproduction in any medium, so long as the resultant use is not for commercial advantage and provided the original work is properly cited. |
spellingShingle | Research Articles Kim, Jaehyun Kwon, Sung-Min Kang, Yeo Kyung Kim, Yong-Hoon Lee, Myung-Jae Han, Kwangjoon Facchetti, Antonio Kim, Myung-Gil Park, Sung Kyu A skin-like two-dimensionally pixelized full-color quantum dot photodetector |
title | A skin-like two-dimensionally pixelized full-color quantum dot photodetector |
title_full | A skin-like two-dimensionally pixelized full-color quantum dot photodetector |
title_fullStr | A skin-like two-dimensionally pixelized full-color quantum dot photodetector |
title_full_unstemmed | A skin-like two-dimensionally pixelized full-color quantum dot photodetector |
title_short | A skin-like two-dimensionally pixelized full-color quantum dot photodetector |
title_sort | skin-like two-dimensionally pixelized full-color quantum dot photodetector |
topic | Research Articles |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6874493/ https://www.ncbi.nlm.nih.gov/pubmed/31803836 http://dx.doi.org/10.1126/sciadv.aax8801 |
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