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Evolution of native defects in ZnO nanorods irradiated with hydrogen ion

This work reports the study on the evolution of native defects in ZnO nanorods irradiated with hydrogen ion. ZnO nanorod arrays grown vertically on silicon substrates were irradiated by 180 keV H(+) ions to a total fluence of 8.50 × 10(15) ions/cm(2). The X-ray diffraction spectra, photoluminescence...

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Autores principales: Wu, Tengfei, Wang, Aiji, Zheng, Li, Wang, Guangfu, Tu, Qingyun, Lv, Bowen, Liu, Zilin, Wu, Zhenglong, Wang, Yinshu
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2019
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6874528/
https://www.ncbi.nlm.nih.gov/pubmed/31758068
http://dx.doi.org/10.1038/s41598-019-53951-3
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author Wu, Tengfei
Wang, Aiji
Zheng, Li
Wang, Guangfu
Tu, Qingyun
Lv, Bowen
Liu, Zilin
Wu, Zhenglong
Wang, Yinshu
author_facet Wu, Tengfei
Wang, Aiji
Zheng, Li
Wang, Guangfu
Tu, Qingyun
Lv, Bowen
Liu, Zilin
Wu, Zhenglong
Wang, Yinshu
author_sort Wu, Tengfei
collection PubMed
description This work reports the study on the evolution of native defects in ZnO nanorods irradiated with hydrogen ion. ZnO nanorod arrays grown vertically on silicon substrates were irradiated by 180 keV H(+) ions to a total fluence of 8.50 × 10(15) ions/cm(2). The X-ray diffraction spectra, photoluminescence spectra before and after irradiation and the real-time ionoluminescence spectra of the nanorod arrays during the irradiating process were measured. Formation and evolution of defects during H(+) ion irradiation and effects of irradiation on the crystal structure and optical property were studied. Blue shift of exciton emission, shrink of lattice c and improvement of the crystallinity of ZnO nanorods after irradiation were observed. Simple surface passivation of the nanorods could improve the radiation resistance. Formation and evolution of the defects during H(+) ion irradiation could be clarified into four stages and the related models are provided.
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spelling pubmed-68745282019-12-04 Evolution of native defects in ZnO nanorods irradiated with hydrogen ion Wu, Tengfei Wang, Aiji Zheng, Li Wang, Guangfu Tu, Qingyun Lv, Bowen Liu, Zilin Wu, Zhenglong Wang, Yinshu Sci Rep Article This work reports the study on the evolution of native defects in ZnO nanorods irradiated with hydrogen ion. ZnO nanorod arrays grown vertically on silicon substrates were irradiated by 180 keV H(+) ions to a total fluence of 8.50 × 10(15) ions/cm(2). The X-ray diffraction spectra, photoluminescence spectra before and after irradiation and the real-time ionoluminescence spectra of the nanorod arrays during the irradiating process were measured. Formation and evolution of defects during H(+) ion irradiation and effects of irradiation on the crystal structure and optical property were studied. Blue shift of exciton emission, shrink of lattice c and improvement of the crystallinity of ZnO nanorods after irradiation were observed. Simple surface passivation of the nanorods could improve the radiation resistance. Formation and evolution of the defects during H(+) ion irradiation could be clarified into four stages and the related models are provided. Nature Publishing Group UK 2019-11-22 /pmc/articles/PMC6874528/ /pubmed/31758068 http://dx.doi.org/10.1038/s41598-019-53951-3 Text en © The Author(s) 2019 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Wu, Tengfei
Wang, Aiji
Zheng, Li
Wang, Guangfu
Tu, Qingyun
Lv, Bowen
Liu, Zilin
Wu, Zhenglong
Wang, Yinshu
Evolution of native defects in ZnO nanorods irradiated with hydrogen ion
title Evolution of native defects in ZnO nanorods irradiated with hydrogen ion
title_full Evolution of native defects in ZnO nanorods irradiated with hydrogen ion
title_fullStr Evolution of native defects in ZnO nanorods irradiated with hydrogen ion
title_full_unstemmed Evolution of native defects in ZnO nanorods irradiated with hydrogen ion
title_short Evolution of native defects in ZnO nanorods irradiated with hydrogen ion
title_sort evolution of native defects in zno nanorods irradiated with hydrogen ion
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6874528/
https://www.ncbi.nlm.nih.gov/pubmed/31758068
http://dx.doi.org/10.1038/s41598-019-53951-3
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