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Improving Water Permeability of Hydrophilic PVDF Membrane Prepared via Blending with Organic and Inorganic Additives for Humic Acid Separation
The removal of impurities from water or wastewater by the membrane filtration process has become more reliable due to good hydraulic performance and high permeate quality. The filterability of the membrane can be improved by having a material with a specific pore structure and good hydrophilic prope...
Autores principales: | , , , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
MDPI
2019
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6891752/ https://www.ncbi.nlm.nih.gov/pubmed/31766222 http://dx.doi.org/10.3390/molecules24224099 |
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author | Arahman, Nasrul Mulyati, Sri Fahrina, Afrillia Muchtar, Syawaliah Yusuf, Mukramah Takagi, Ryosuke Matsuyama, Hideto Nordin, Nik Abdul Hadi Bilad, Muhammad Roil |
author_facet | Arahman, Nasrul Mulyati, Sri Fahrina, Afrillia Muchtar, Syawaliah Yusuf, Mukramah Takagi, Ryosuke Matsuyama, Hideto Nordin, Nik Abdul Hadi Bilad, Muhammad Roil |
author_sort | Arahman, Nasrul |
collection | PubMed |
description | The removal of impurities from water or wastewater by the membrane filtration process has become more reliable due to good hydraulic performance and high permeate quality. The filterability of the membrane can be improved by having a material with a specific pore structure and good hydrophilic properties. This work aims at preparing a polyvinylidene fluoride (PVDF) membrane incorporated with phospholipid in the form of a 2-methacryloyloxyethyl phosphorylcholine, polymeric additive in the form of polyvinylpyrrolidone, and its combination with inorganic nanosilica from a renewable source derived from bagasse. The resulting membrane morphologies were analyzed by using scanning electron microscopy. Furthermore, atomic force microscopy was performed to analyze the membrane surface roughness. The chemical compositions of the resulting membranes were identified using Fourier transform infrared. A lab-scale cross-flow filtration system module was used to evaluate the membrane’s hydraulic and separation performance by the filtration of humic acid (HA) solution as the model contaminant. Results showed that the additives improved the membrane surface hydrophilicity. All modified membranes also showed up to five times higher water permeability than the pristine PVDF, thanks to the improved structure. Additionally, all membrane samples showed HA rejections of 75–90%. |
format | Online Article Text |
id | pubmed-6891752 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2019 |
publisher | MDPI |
record_format | MEDLINE/PubMed |
spelling | pubmed-68917522019-12-12 Improving Water Permeability of Hydrophilic PVDF Membrane Prepared via Blending with Organic and Inorganic Additives for Humic Acid Separation Arahman, Nasrul Mulyati, Sri Fahrina, Afrillia Muchtar, Syawaliah Yusuf, Mukramah Takagi, Ryosuke Matsuyama, Hideto Nordin, Nik Abdul Hadi Bilad, Muhammad Roil Molecules Article The removal of impurities from water or wastewater by the membrane filtration process has become more reliable due to good hydraulic performance and high permeate quality. The filterability of the membrane can be improved by having a material with a specific pore structure and good hydrophilic properties. This work aims at preparing a polyvinylidene fluoride (PVDF) membrane incorporated with phospholipid in the form of a 2-methacryloyloxyethyl phosphorylcholine, polymeric additive in the form of polyvinylpyrrolidone, and its combination with inorganic nanosilica from a renewable source derived from bagasse. The resulting membrane morphologies were analyzed by using scanning electron microscopy. Furthermore, atomic force microscopy was performed to analyze the membrane surface roughness. The chemical compositions of the resulting membranes were identified using Fourier transform infrared. A lab-scale cross-flow filtration system module was used to evaluate the membrane’s hydraulic and separation performance by the filtration of humic acid (HA) solution as the model contaminant. Results showed that the additives improved the membrane surface hydrophilicity. All modified membranes also showed up to five times higher water permeability than the pristine PVDF, thanks to the improved structure. Additionally, all membrane samples showed HA rejections of 75–90%. MDPI 2019-11-13 /pmc/articles/PMC6891752/ /pubmed/31766222 http://dx.doi.org/10.3390/molecules24224099 Text en © 2019 by the authors. Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (http://creativecommons.org/licenses/by/4.0/). |
spellingShingle | Article Arahman, Nasrul Mulyati, Sri Fahrina, Afrillia Muchtar, Syawaliah Yusuf, Mukramah Takagi, Ryosuke Matsuyama, Hideto Nordin, Nik Abdul Hadi Bilad, Muhammad Roil Improving Water Permeability of Hydrophilic PVDF Membrane Prepared via Blending with Organic and Inorganic Additives for Humic Acid Separation |
title | Improving Water Permeability of Hydrophilic PVDF Membrane Prepared via Blending with Organic and Inorganic Additives for Humic Acid Separation |
title_full | Improving Water Permeability of Hydrophilic PVDF Membrane Prepared via Blending with Organic and Inorganic Additives for Humic Acid Separation |
title_fullStr | Improving Water Permeability of Hydrophilic PVDF Membrane Prepared via Blending with Organic and Inorganic Additives for Humic Acid Separation |
title_full_unstemmed | Improving Water Permeability of Hydrophilic PVDF Membrane Prepared via Blending with Organic and Inorganic Additives for Humic Acid Separation |
title_short | Improving Water Permeability of Hydrophilic PVDF Membrane Prepared via Blending with Organic and Inorganic Additives for Humic Acid Separation |
title_sort | improving water permeability of hydrophilic pvdf membrane prepared via blending with organic and inorganic additives for humic acid separation |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6891752/ https://www.ncbi.nlm.nih.gov/pubmed/31766222 http://dx.doi.org/10.3390/molecules24224099 |
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