Cargando…

Sub-cycle time resolution of multi-photon momentum transfer in strong-field ionization

During multi-photon ionization of an atom it is well understood how the involved photons transfer their energy to the ion and the photoelectron. However, the transfer of the photon linear momentum is still not fully understood. Here, we present a time-resolved measurement of linear momentum transfer...

Descripción completa

Detalles Bibliográficos
Autores principales: Willenberg, Benjamin, Maurer, Jochen, Mayer, Benedikt W., Keller, Ursula
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2019
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6895185/
https://www.ncbi.nlm.nih.gov/pubmed/31804473
http://dx.doi.org/10.1038/s41467-019-13409-6
_version_ 1783476542064558080
author Willenberg, Benjamin
Maurer, Jochen
Mayer, Benedikt W.
Keller, Ursula
author_facet Willenberg, Benjamin
Maurer, Jochen
Mayer, Benedikt W.
Keller, Ursula
author_sort Willenberg, Benjamin
collection PubMed
description During multi-photon ionization of an atom it is well understood how the involved photons transfer their energy to the ion and the photoelectron. However, the transfer of the photon linear momentum is still not fully understood. Here, we present a time-resolved measurement of linear momentum transfer along the laser pulse propagation direction. We can show that the linear momentum transfer to the photoelectron depends on the ionization time within the laser cycle using the attoclock technique. We can mostly explain the measured linear momentum transfer within a classical model for a free electron in a laser field. However, corrections are required due to the parent-ion interaction and due to the initial momentum when the electron enters the continuum. The parent-ion interaction induces a negative attosecond time delay between the appearance in the continuum of the electron with minimal linear momentum transfer and the point in time with maximum ionization rate.
format Online
Article
Text
id pubmed-6895185
institution National Center for Biotechnology Information
language English
publishDate 2019
publisher Nature Publishing Group UK
record_format MEDLINE/PubMed
spelling pubmed-68951852019-12-09 Sub-cycle time resolution of multi-photon momentum transfer in strong-field ionization Willenberg, Benjamin Maurer, Jochen Mayer, Benedikt W. Keller, Ursula Nat Commun Article During multi-photon ionization of an atom it is well understood how the involved photons transfer their energy to the ion and the photoelectron. However, the transfer of the photon linear momentum is still not fully understood. Here, we present a time-resolved measurement of linear momentum transfer along the laser pulse propagation direction. We can show that the linear momentum transfer to the photoelectron depends on the ionization time within the laser cycle using the attoclock technique. We can mostly explain the measured linear momentum transfer within a classical model for a free electron in a laser field. However, corrections are required due to the parent-ion interaction and due to the initial momentum when the electron enters the continuum. The parent-ion interaction induces a negative attosecond time delay between the appearance in the continuum of the electron with minimal linear momentum transfer and the point in time with maximum ionization rate. Nature Publishing Group UK 2019-12-05 /pmc/articles/PMC6895185/ /pubmed/31804473 http://dx.doi.org/10.1038/s41467-019-13409-6 Text en © The Author(s) 2019 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Willenberg, Benjamin
Maurer, Jochen
Mayer, Benedikt W.
Keller, Ursula
Sub-cycle time resolution of multi-photon momentum transfer in strong-field ionization
title Sub-cycle time resolution of multi-photon momentum transfer in strong-field ionization
title_full Sub-cycle time resolution of multi-photon momentum transfer in strong-field ionization
title_fullStr Sub-cycle time resolution of multi-photon momentum transfer in strong-field ionization
title_full_unstemmed Sub-cycle time resolution of multi-photon momentum transfer in strong-field ionization
title_short Sub-cycle time resolution of multi-photon momentum transfer in strong-field ionization
title_sort sub-cycle time resolution of multi-photon momentum transfer in strong-field ionization
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6895185/
https://www.ncbi.nlm.nih.gov/pubmed/31804473
http://dx.doi.org/10.1038/s41467-019-13409-6
work_keys_str_mv AT willenbergbenjamin subcycletimeresolutionofmultiphotonmomentumtransferinstrongfieldionization
AT maurerjochen subcycletimeresolutionofmultiphotonmomentumtransferinstrongfieldionization
AT mayerbenediktw subcycletimeresolutionofmultiphotonmomentumtransferinstrongfieldionization
AT kellerursula subcycletimeresolutionofmultiphotonmomentumtransferinstrongfieldionization