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Valley-polarized exciton currents in a van der Waals heterostructure

Valleytronics is an appealing alternative to conventional charge-based electronics which aims at encoding data in the valley degree of freedom, i.e. the information over which extreme of the conduction or valence band carriers are occupying. The ability to create and control valley-currents in solid...

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Autores principales: Unuchek, Dmitrii, Ciarrocchi, Alberto, Avsar, Ahmet, Sun, Zhe, Watanabe, Kenji, Taniguchi, Takashi, Kis, Andras
Formato: Online Artículo Texto
Lenguaje:English
Publicado: 2019
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6897556/
https://www.ncbi.nlm.nih.gov/pubmed/31636411
http://dx.doi.org/10.1038/s41565-019-0559-y
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author Unuchek, Dmitrii
Ciarrocchi, Alberto
Avsar, Ahmet
Sun, Zhe
Watanabe, Kenji
Taniguchi, Takashi
Kis, Andras
author_facet Unuchek, Dmitrii
Ciarrocchi, Alberto
Avsar, Ahmet
Sun, Zhe
Watanabe, Kenji
Taniguchi, Takashi
Kis, Andras
author_sort Unuchek, Dmitrii
collection PubMed
description Valleytronics is an appealing alternative to conventional charge-based electronics which aims at encoding data in the valley degree of freedom, i.e. the information over which extreme of the conduction or valence band carriers are occupying. The ability to create and control valley-currents in solid state devices could therefore enable new paradigms for information processing. Transition metal dichalcogenides (TMDCs) are a promising platform for valleytronics, due to the presence of two inequivalent valleys with spin-valley locking(1) and a direct band gap(2,3), which allows optical initialization and readout of the valley-state(4,5). Recent progresses on the control of interlayer excitons in these materials(6–8) could offer an effective way to realize optoelectronic devices based on the valley degree of freedom. Here, we show the generation and transport over mesoscopic distances of valley-polarized excitons in a device based on a type-II TMDC heterostructure. Engineering of the interlayer coupling results in enhanced diffusion of valley-polarized excitons, which can be controlled and switched electrically. Furthermore, using electrostatic traps, we can increase exciton concentration by an order of magnitude, reaching densities in the order of 10(12) cm(-2), opening the route to achieving a coherent quantum state of valley-polarized excitons via Bose-Einstein condensation.
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spelling pubmed-68975562020-04-21 Valley-polarized exciton currents in a van der Waals heterostructure Unuchek, Dmitrii Ciarrocchi, Alberto Avsar, Ahmet Sun, Zhe Watanabe, Kenji Taniguchi, Takashi Kis, Andras Nat Nanotechnol Article Valleytronics is an appealing alternative to conventional charge-based electronics which aims at encoding data in the valley degree of freedom, i.e. the information over which extreme of the conduction or valence band carriers are occupying. The ability to create and control valley-currents in solid state devices could therefore enable new paradigms for information processing. Transition metal dichalcogenides (TMDCs) are a promising platform for valleytronics, due to the presence of two inequivalent valleys with spin-valley locking(1) and a direct band gap(2,3), which allows optical initialization and readout of the valley-state(4,5). Recent progresses on the control of interlayer excitons in these materials(6–8) could offer an effective way to realize optoelectronic devices based on the valley degree of freedom. Here, we show the generation and transport over mesoscopic distances of valley-polarized excitons in a device based on a type-II TMDC heterostructure. Engineering of the interlayer coupling results in enhanced diffusion of valley-polarized excitons, which can be controlled and switched electrically. Furthermore, using electrostatic traps, we can increase exciton concentration by an order of magnitude, reaching densities in the order of 10(12) cm(-2), opening the route to achieving a coherent quantum state of valley-polarized excitons via Bose-Einstein condensation. 2019-10-21 2019-12 /pmc/articles/PMC6897556/ /pubmed/31636411 http://dx.doi.org/10.1038/s41565-019-0559-y Text en http://www.nature.com/authors/editorial_policies/license.html#terms Users may view, print, copy, and download text and data-mine the content in such documents, for the purposes of academic research, subject always to the full Conditions of use:http://www.nature.com/authors/editorial_policies/license.html#terms
spellingShingle Article
Unuchek, Dmitrii
Ciarrocchi, Alberto
Avsar, Ahmet
Sun, Zhe
Watanabe, Kenji
Taniguchi, Takashi
Kis, Andras
Valley-polarized exciton currents in a van der Waals heterostructure
title Valley-polarized exciton currents in a van der Waals heterostructure
title_full Valley-polarized exciton currents in a van der Waals heterostructure
title_fullStr Valley-polarized exciton currents in a van der Waals heterostructure
title_full_unstemmed Valley-polarized exciton currents in a van der Waals heterostructure
title_short Valley-polarized exciton currents in a van der Waals heterostructure
title_sort valley-polarized exciton currents in a van der waals heterostructure
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6897556/
https://www.ncbi.nlm.nih.gov/pubmed/31636411
http://dx.doi.org/10.1038/s41565-019-0559-y
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