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Millimetre-long transport of photogenerated carriers in topological insulators

Excitons are spin integer particles that are predicted to condense into a coherent quantum state at sufficiently low temperature. Here by using photocurrent imaging we report experimental evidence of formation and efficient transport of non-equilibrium excitons in Bi(2-x)Sb(x)Se(3) nanoribbons. The...

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Autores principales: Hou, Yasen, Wang, Rui, Xiao, Rui, McClintock, Luke, Clark Travaglini, Henry, Paulus Francia, John, Fetsch, Harry, Erten, Onur, Savrasov, Sergey Y., Wang, Baigeng, Rossi, Antonio, Vishik, Inna, Rotenberg, Eli, Yu, Dong
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2019
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6915787/
https://www.ncbi.nlm.nih.gov/pubmed/31844140
http://dx.doi.org/10.1038/s41467-019-13711-3
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author Hou, Yasen
Wang, Rui
Xiao, Rui
McClintock, Luke
Clark Travaglini, Henry
Paulus Francia, John
Fetsch, Harry
Erten, Onur
Savrasov, Sergey Y.
Wang, Baigeng
Rossi, Antonio
Vishik, Inna
Rotenberg, Eli
Yu, Dong
author_facet Hou, Yasen
Wang, Rui
Xiao, Rui
McClintock, Luke
Clark Travaglini, Henry
Paulus Francia, John
Fetsch, Harry
Erten, Onur
Savrasov, Sergey Y.
Wang, Baigeng
Rossi, Antonio
Vishik, Inna
Rotenberg, Eli
Yu, Dong
author_sort Hou, Yasen
collection PubMed
description Excitons are spin integer particles that are predicted to condense into a coherent quantum state at sufficiently low temperature. Here by using photocurrent imaging we report experimental evidence of formation and efficient transport of non-equilibrium excitons in Bi(2-x)Sb(x)Se(3) nanoribbons. The photocurrent distributions are independent of electric field, indicating that photoexcited electrons and holes form excitons. Remarkably, these excitons can transport over hundreds of micrometers along the topological insulator (TI) nanoribbons before recombination at up to 40 K. The macroscopic transport distance, combined with short carrier lifetime obtained from transient photocurrent measurements, indicates an exciton diffusion coefficient at least 36 m(2) s(−1), which corresponds to a mobility of 6 × 10(4) m(2) V(−1) s(−1) at 7 K and is four order of magnitude higher than the value reported for free carriers in TIs. The observation of highly dissipationless exciton transport implies the formation of superfluid-like exciton condensate at the surface of TIs.
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spelling pubmed-69157872019-12-18 Millimetre-long transport of photogenerated carriers in topological insulators Hou, Yasen Wang, Rui Xiao, Rui McClintock, Luke Clark Travaglini, Henry Paulus Francia, John Fetsch, Harry Erten, Onur Savrasov, Sergey Y. Wang, Baigeng Rossi, Antonio Vishik, Inna Rotenberg, Eli Yu, Dong Nat Commun Article Excitons are spin integer particles that are predicted to condense into a coherent quantum state at sufficiently low temperature. Here by using photocurrent imaging we report experimental evidence of formation and efficient transport of non-equilibrium excitons in Bi(2-x)Sb(x)Se(3) nanoribbons. The photocurrent distributions are independent of electric field, indicating that photoexcited electrons and holes form excitons. Remarkably, these excitons can transport over hundreds of micrometers along the topological insulator (TI) nanoribbons before recombination at up to 40 K. The macroscopic transport distance, combined with short carrier lifetime obtained from transient photocurrent measurements, indicates an exciton diffusion coefficient at least 36 m(2) s(−1), which corresponds to a mobility of 6 × 10(4) m(2) V(−1) s(−1) at 7 K and is four order of magnitude higher than the value reported for free carriers in TIs. The observation of highly dissipationless exciton transport implies the formation of superfluid-like exciton condensate at the surface of TIs. Nature Publishing Group UK 2019-12-16 /pmc/articles/PMC6915787/ /pubmed/31844140 http://dx.doi.org/10.1038/s41467-019-13711-3 Text en © The Author(s) 2019 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Hou, Yasen
Wang, Rui
Xiao, Rui
McClintock, Luke
Clark Travaglini, Henry
Paulus Francia, John
Fetsch, Harry
Erten, Onur
Savrasov, Sergey Y.
Wang, Baigeng
Rossi, Antonio
Vishik, Inna
Rotenberg, Eli
Yu, Dong
Millimetre-long transport of photogenerated carriers in topological insulators
title Millimetre-long transport of photogenerated carriers in topological insulators
title_full Millimetre-long transport of photogenerated carriers in topological insulators
title_fullStr Millimetre-long transport of photogenerated carriers in topological insulators
title_full_unstemmed Millimetre-long transport of photogenerated carriers in topological insulators
title_short Millimetre-long transport of photogenerated carriers in topological insulators
title_sort millimetre-long transport of photogenerated carriers in topological insulators
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6915787/
https://www.ncbi.nlm.nih.gov/pubmed/31844140
http://dx.doi.org/10.1038/s41467-019-13711-3
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