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Millimetre-long transport of photogenerated carriers in topological insulators
Excitons are spin integer particles that are predicted to condense into a coherent quantum state at sufficiently low temperature. Here by using photocurrent imaging we report experimental evidence of formation and efficient transport of non-equilibrium excitons in Bi(2-x)Sb(x)Se(3) nanoribbons. The...
Autores principales: | , , , , , , , , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group UK
2019
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6915787/ https://www.ncbi.nlm.nih.gov/pubmed/31844140 http://dx.doi.org/10.1038/s41467-019-13711-3 |
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author | Hou, Yasen Wang, Rui Xiao, Rui McClintock, Luke Clark Travaglini, Henry Paulus Francia, John Fetsch, Harry Erten, Onur Savrasov, Sergey Y. Wang, Baigeng Rossi, Antonio Vishik, Inna Rotenberg, Eli Yu, Dong |
author_facet | Hou, Yasen Wang, Rui Xiao, Rui McClintock, Luke Clark Travaglini, Henry Paulus Francia, John Fetsch, Harry Erten, Onur Savrasov, Sergey Y. Wang, Baigeng Rossi, Antonio Vishik, Inna Rotenberg, Eli Yu, Dong |
author_sort | Hou, Yasen |
collection | PubMed |
description | Excitons are spin integer particles that are predicted to condense into a coherent quantum state at sufficiently low temperature. Here by using photocurrent imaging we report experimental evidence of formation and efficient transport of non-equilibrium excitons in Bi(2-x)Sb(x)Se(3) nanoribbons. The photocurrent distributions are independent of electric field, indicating that photoexcited electrons and holes form excitons. Remarkably, these excitons can transport over hundreds of micrometers along the topological insulator (TI) nanoribbons before recombination at up to 40 K. The macroscopic transport distance, combined with short carrier lifetime obtained from transient photocurrent measurements, indicates an exciton diffusion coefficient at least 36 m(2) s(−1), which corresponds to a mobility of 6 × 10(4) m(2) V(−1) s(−1) at 7 K and is four order of magnitude higher than the value reported for free carriers in TIs. The observation of highly dissipationless exciton transport implies the formation of superfluid-like exciton condensate at the surface of TIs. |
format | Online Article Text |
id | pubmed-6915787 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2019 |
publisher | Nature Publishing Group UK |
record_format | MEDLINE/PubMed |
spelling | pubmed-69157872019-12-18 Millimetre-long transport of photogenerated carriers in topological insulators Hou, Yasen Wang, Rui Xiao, Rui McClintock, Luke Clark Travaglini, Henry Paulus Francia, John Fetsch, Harry Erten, Onur Savrasov, Sergey Y. Wang, Baigeng Rossi, Antonio Vishik, Inna Rotenberg, Eli Yu, Dong Nat Commun Article Excitons are spin integer particles that are predicted to condense into a coherent quantum state at sufficiently low temperature. Here by using photocurrent imaging we report experimental evidence of formation and efficient transport of non-equilibrium excitons in Bi(2-x)Sb(x)Se(3) nanoribbons. The photocurrent distributions are independent of electric field, indicating that photoexcited electrons and holes form excitons. Remarkably, these excitons can transport over hundreds of micrometers along the topological insulator (TI) nanoribbons before recombination at up to 40 K. The macroscopic transport distance, combined with short carrier lifetime obtained from transient photocurrent measurements, indicates an exciton diffusion coefficient at least 36 m(2) s(−1), which corresponds to a mobility of 6 × 10(4) m(2) V(−1) s(−1) at 7 K and is four order of magnitude higher than the value reported for free carriers in TIs. The observation of highly dissipationless exciton transport implies the formation of superfluid-like exciton condensate at the surface of TIs. Nature Publishing Group UK 2019-12-16 /pmc/articles/PMC6915787/ /pubmed/31844140 http://dx.doi.org/10.1038/s41467-019-13711-3 Text en © The Author(s) 2019 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/. |
spellingShingle | Article Hou, Yasen Wang, Rui Xiao, Rui McClintock, Luke Clark Travaglini, Henry Paulus Francia, John Fetsch, Harry Erten, Onur Savrasov, Sergey Y. Wang, Baigeng Rossi, Antonio Vishik, Inna Rotenberg, Eli Yu, Dong Millimetre-long transport of photogenerated carriers in topological insulators |
title | Millimetre-long transport of photogenerated carriers in topological insulators |
title_full | Millimetre-long transport of photogenerated carriers in topological insulators |
title_fullStr | Millimetre-long transport of photogenerated carriers in topological insulators |
title_full_unstemmed | Millimetre-long transport of photogenerated carriers in topological insulators |
title_short | Millimetre-long transport of photogenerated carriers in topological insulators |
title_sort | millimetre-long transport of photogenerated carriers in topological insulators |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6915787/ https://www.ncbi.nlm.nih.gov/pubmed/31844140 http://dx.doi.org/10.1038/s41467-019-13711-3 |
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